A conceptual framework for mixing structures in individual aerosol particles

This study investigated the particle size‐ and age‐dependent mixing structures of individual particles in clean and polluted air. Aerosols were classified into eight components: sea salt, mineral dust, fly ash, metal, soot, sulfates, nitrates, and organic matter (OM). Based on our aerosol classifica...

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Veröffentlicht in:Journal of geophysical research. Atmospheres 2016-11, Vol.121 (22), p.13,784-13,798
Hauptverfasser: Li, Weijun, Sun, Jiaxing, Xu, Liang, Shi, Zongbo, Riemer, Nicole, Sun, Yele, Fu, Pingqing, Zhang, Jianchao, Lin, Yangting, Wang, Xinfeng, Shao, Longyi, Chen, Jianmin, Zhang, Xiaoye, Wang, Zifa, Wang, Wenxing
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Sprache:eng
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Zusammenfassung:This study investigated the particle size‐ and age‐dependent mixing structures of individual particles in clean and polluted air. Aerosols were classified into eight components: sea salt, mineral dust, fly ash, metal, soot, sulfates, nitrates, and organic matter (OM). Based on our aerosol classification, a particle that consists of two or more aerosol components can be defined as an internally mixed particle. Otherwise, it is considered to be an externally mixed particle. Within the internally mixed particle class, we identified four heterogeneous mixing structures: core‐shell, dumbbell, OM coating, and dispersed OM, as well as one homogeneous‐like mixing structure. Homogeneous‐like mixing mainly occurred in fine particles (
ISSN:2169-897X
2169-8996
DOI:10.1002/2016JD025252