Relationship between laser-induced gratings and vibrational properties of Eu-doped glasses
Four-wave-mixing techniques have been shown previously to produce permanent refractive index gratings in Eu-doped glasses by resonant excitation of the Eu/sup 3+/ ions. A variety of glass hosts were studied and it was found that permanent holographic gratings could be established in some of these bu...
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| Veröffentlicht in: | Phys. Rev. B: Condens. Matter; (United States) 1987-03, Vol.35 (8), p.4109-4112 |
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| container_title | Phys. Rev. B: Condens. Matter; (United States) |
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| creator | DURVILLE, F. M BEHRENS, E. G POWELL, R. C |
| description | Four-wave-mixing techniques have been shown previously to produce permanent refractive index gratings in Eu-doped glasses by resonant excitation of the Eu/sup 3+/ ions. A variety of glass hosts were studied and it was found that permanent holographic gratings could be established in some of these but not in others. We report here an extension of our previous work which includes investigations of new materials, attempts to form gratings with different excitation wavelengths, and a comparison of the Raman and resonant Raman spectra of glasses which do and do not exhibit permanent holographic gratings. It was found that direct excitation into the /sup 5/D/sub 0/ level did not produce permanent gratings. It was also found that glasses which do exhibit permanent gratings have high-frequency vibrational modes which couple strongly to the Eu/sup 3+/ ions. These results help to verify the model proposed previously to explain the origin of the holographic grating in terms of structural changes caused by thermal effects arising from radiationless relaxation through high-frequency local modes. |
| doi_str_mv | 10.1103/PhysRevB.35.4109 |
| format | Article |
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M ; BEHRENS, E. G ; POWELL, R. C</creator><creatorcontrib>DURVILLE, F. M ; BEHRENS, E. G ; POWELL, R. C ; Department of Physics, Oklahoma State University, Stillwater, Oklahoma 74078-0444</creatorcontrib><description>Four-wave-mixing techniques have been shown previously to produce permanent refractive index gratings in Eu-doped glasses by resonant excitation of the Eu/sup 3+/ ions. A variety of glass hosts were studied and it was found that permanent holographic gratings could be established in some of these but not in others. We report here an extension of our previous work which includes investigations of new materials, attempts to form gratings with different excitation wavelengths, and a comparison of the Raman and resonant Raman spectra of glasses which do and do not exhibit permanent holographic gratings. It was found that direct excitation into the /sup 5/D/sub 0/ level did not produce permanent gratings. It was also found that glasses which do exhibit permanent gratings have high-frequency vibrational modes which couple strongly to the Eu/sup 3+/ ions. These results help to verify the model proposed previously to explain the origin of the holographic grating in terms of structural changes caused by thermal effects arising from radiationless relaxation through high-frequency local modes.</description><identifier>ISSN: 0163-1829</identifier><identifier>EISSN: 1095-3795</identifier><identifier>DOI: 10.1103/PhysRevB.35.4109</identifier><identifier>PMID: 9941945</identifier><identifier>CODEN: PRBMDO</identifier><language>eng</language><publisher>Woodbury, NY: American Physical Society</publisher><subject>ALLOYS ; CHARGED PARTICLES ; Condensed matter: electronic structure, electrical, magnetic, and optical properties ; DOPED MATERIALS ; ENERGY-LEVEL TRANSITIONS ; EUROPIUM ADDITIONS ; EUROPIUM ALLOYS ; EUROPIUM IONS ; Exact sciences and technology ; EXCITATION ; GLASS ; GRATINGS ; Infrared and raman spectra and scattering ; IONS ; LASERS ; LATTICE VIBRATIONS ; MATERIALS ; MATERIALS SCIENCE ; OPTICAL PROPERTIES ; Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation ; PHYSICAL PROPERTIES ; Physics ; RARE EARTH ADDITIONS ; RARE EARTH ALLOYS 360602 -- Other Materials-- Structure & Phase Studies ; REFRACTIVITY ; RELAXATION ; RESONANCE ; TEMPERATURE EFFECTS</subject><ispartof>Phys. 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M</creatorcontrib><creatorcontrib>BEHRENS, E. G</creatorcontrib><creatorcontrib>POWELL, R. C</creatorcontrib><creatorcontrib>Department of Physics, Oklahoma State University, Stillwater, Oklahoma 74078-0444</creatorcontrib><title>Relationship between laser-induced gratings and vibrational properties of Eu-doped glasses</title><title>Phys. Rev. B: Condens. Matter; (United States)</title><addtitle>Phys Rev B Condens Matter</addtitle><description>Four-wave-mixing techniques have been shown previously to produce permanent refractive index gratings in Eu-doped glasses by resonant excitation of the Eu/sup 3+/ ions. A variety of glass hosts were studied and it was found that permanent holographic gratings could be established in some of these but not in others. We report here an extension of our previous work which includes investigations of new materials, attempts to form gratings with different excitation wavelengths, and a comparison of the Raman and resonant Raman spectra of glasses which do and do not exhibit permanent holographic gratings. It was found that direct excitation into the /sup 5/D/sub 0/ level did not produce permanent gratings. It was also found that glasses which do exhibit permanent gratings have high-frequency vibrational modes which couple strongly to the Eu/sup 3+/ ions. These results help to verify the model proposed previously to explain the origin of the holographic grating in terms of structural changes caused by thermal effects arising from radiationless relaxation through high-frequency local modes.</description><subject>ALLOYS</subject><subject>CHARGED PARTICLES</subject><subject>Condensed matter: electronic structure, electrical, magnetic, and optical properties</subject><subject>DOPED MATERIALS</subject><subject>ENERGY-LEVEL TRANSITIONS</subject><subject>EUROPIUM ADDITIONS</subject><subject>EUROPIUM ALLOYS</subject><subject>EUROPIUM IONS</subject><subject>Exact sciences and technology</subject><subject>EXCITATION</subject><subject>GLASS</subject><subject>GRATINGS</subject><subject>Infrared and raman spectra and scattering</subject><subject>IONS</subject><subject>LASERS</subject><subject>LATTICE VIBRATIONS</subject><subject>MATERIALS</subject><subject>MATERIALS SCIENCE</subject><subject>OPTICAL PROPERTIES</subject><subject>Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation</subject><subject>PHYSICAL PROPERTIES</subject><subject>Physics</subject><subject>RARE EARTH ADDITIONS</subject><subject>RARE EARTH ALLOYS 360602 -- Other Materials-- Structure & Phase Studies</subject><subject>REFRACTIVITY</subject><subject>RELAXATION</subject><subject>RESONANCE</subject><subject>TEMPERATURE EFFECTS</subject><issn>0163-1829</issn><issn>1095-3795</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>1987</creationdate><recordtype>article</recordtype><recordid>eNo9kM1v1DAQxa2KqiyFOxekCHHgksWOP5I5lqq0SJWKKrhwsRxn3DXKOltPUtT_Hre7dA4zGs3vPY0eY-8FXwvB5Zcfm0e6xYeva6nXSnA4YqvSdS1b0K_Yigsja9E18Jq9IfrDSzUGTtgJgBKg9Ir9vsXRzXFKtIm7qsf5L2KqRkeY65iGxeNQ3eVCpDuqXBqqh9jnZ4Ebq12edpjniFRNobpY6qHshS9yQnrLjoMbCd8d5in79e3i5_lVfX1z-f387Lr2UjdzHVTfcBeCBKmGoOSgUA4dh7YTQYdOgFfSqL5rVAPAlfBC-AYMl2haAOnlKfu4951ojpZ8nNFv_JQS-tmaTnCudYE-76Hy8_2CNNttJI_j6BJOC1nRaRAtGCMKyveozxNRxmB3OW5dfrSC26fU7f_UrdT2KfUi-XBwX_otDi-CQ8zl_ulwd-TdGLJLPtIL1qrOtArkP_s3i14</recordid><startdate>19870315</startdate><enddate>19870315</enddate><creator>DURVILLE, F. M</creator><creator>BEHRENS, E. G</creator><creator>POWELL, R. C</creator><general>American Physical Society</general><general>American Institute of Physics</general><scope>IQODW</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>OTOTI</scope></search><sort><creationdate>19870315</creationdate><title>Relationship between laser-induced gratings and vibrational properties of Eu-doped glasses</title><author>DURVILLE, F. M ; BEHRENS, E. G ; POWELL, R. C</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c352t-f4b20aff3934df43d4e3d809781f5f819c4364b824299041c11c29603e67993c3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>1987</creationdate><topic>ALLOYS</topic><topic>CHARGED PARTICLES</topic><topic>Condensed matter: electronic structure, electrical, magnetic, and optical properties</topic><topic>DOPED MATERIALS</topic><topic>ENERGY-LEVEL TRANSITIONS</topic><topic>EUROPIUM ADDITIONS</topic><topic>EUROPIUM ALLOYS</topic><topic>EUROPIUM IONS</topic><topic>Exact sciences and technology</topic><topic>EXCITATION</topic><topic>GLASS</topic><topic>GRATINGS</topic><topic>Infrared and raman spectra and scattering</topic><topic>IONS</topic><topic>LASERS</topic><topic>LATTICE VIBRATIONS</topic><topic>MATERIALS</topic><topic>MATERIALS SCIENCE</topic><topic>OPTICAL PROPERTIES</topic><topic>Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation</topic><topic>PHYSICAL PROPERTIES</topic><topic>Physics</topic><topic>RARE EARTH ADDITIONS</topic><topic>RARE EARTH ALLOYS 360602 -- Other Materials-- Structure & Phase Studies</topic><topic>REFRACTIVITY</topic><topic>RELAXATION</topic><topic>RESONANCE</topic><topic>TEMPERATURE EFFECTS</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>DURVILLE, F. M</creatorcontrib><creatorcontrib>BEHRENS, E. G</creatorcontrib><creatorcontrib>POWELL, R. C</creatorcontrib><creatorcontrib>Department of Physics, Oklahoma State University, Stillwater, Oklahoma 74078-0444</creatorcontrib><collection>Pascal-Francis</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>OSTI.GOV</collection><jtitle>Phys. Rev. B: Condens. Matter; (United States)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>DURVILLE, F. M</au><au>BEHRENS, E. G</au><au>POWELL, R. C</au><aucorp>Department of Physics, Oklahoma State University, Stillwater, Oklahoma 74078-0444</aucorp><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Relationship between laser-induced gratings and vibrational properties of Eu-doped glasses</atitle><jtitle>Phys. Rev. B: Condens. Matter; (United States)</jtitle><addtitle>Phys Rev B Condens Matter</addtitle><date>1987-03-15</date><risdate>1987</risdate><volume>35</volume><issue>8</issue><spage>4109</spage><epage>4112</epage><pages>4109-4112</pages><issn>0163-1829</issn><eissn>1095-3795</eissn><coden>PRBMDO</coden><abstract>Four-wave-mixing techniques have been shown previously to produce permanent refractive index gratings in Eu-doped glasses by resonant excitation of the Eu/sup 3+/ ions. A variety of glass hosts were studied and it was found that permanent holographic gratings could be established in some of these but not in others. We report here an extension of our previous work which includes investigations of new materials, attempts to form gratings with different excitation wavelengths, and a comparison of the Raman and resonant Raman spectra of glasses which do and do not exhibit permanent holographic gratings. It was found that direct excitation into the /sup 5/D/sub 0/ level did not produce permanent gratings. It was also found that glasses which do exhibit permanent gratings have high-frequency vibrational modes which couple strongly to the Eu/sup 3+/ ions. These results help to verify the model proposed previously to explain the origin of the holographic grating in terms of structural changes caused by thermal effects arising from radiationless relaxation through high-frequency local modes.</abstract><cop>Woodbury, NY</cop><pub>American Physical Society</pub><pmid>9941945</pmid><doi>10.1103/PhysRevB.35.4109</doi><tpages>4</tpages></addata></record> |
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| subjects | ALLOYS CHARGED PARTICLES Condensed matter: electronic structure, electrical, magnetic, and optical properties DOPED MATERIALS ENERGY-LEVEL TRANSITIONS EUROPIUM ADDITIONS EUROPIUM ALLOYS EUROPIUM IONS Exact sciences and technology EXCITATION GLASS GRATINGS Infrared and raman spectra and scattering IONS LASERS LATTICE VIBRATIONS MATERIALS MATERIALS SCIENCE OPTICAL PROPERTIES Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation PHYSICAL PROPERTIES Physics RARE EARTH ADDITIONS RARE EARTH ALLOYS 360602 -- Other Materials-- Structure & Phase Studies REFRACTIVITY RELAXATION RESONANCE TEMPERATURE EFFECTS |
| title | Relationship between laser-induced gratings and vibrational properties of Eu-doped glasses |
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