Integrated Photoelectrochemical Solar Energy Conversion and Organic Redox Flow Battery Devices
Building on regenerative photoelectrochemical solar cells and emerging electrochemical redox flow batteries (RFBs), more efficient, scalable, compact, and cost‐effective hybrid energy conversion and storage devices could be realized. An integrated photoelectrochemical solar energy conversion and ele...
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| Veröffentlicht in: | Angewandte Chemie 2016-10, Vol.128 (42), p.13298-13302 |
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| creator | Li, Wenjie Fu, Hui-Chun Li, Linsen Cabán-Acevedo, Miguel He, Jr-Hau Jin, Song |
| description | Building on regenerative photoelectrochemical solar cells and emerging electrochemical redox flow batteries (RFBs), more efficient, scalable, compact, and cost‐effective hybrid energy conversion and storage devices could be realized. An integrated photoelectrochemical solar energy conversion and electrochemical storage device is developed by integrating regenerative silicon solar cells and 9,10‐anthraquinone‐2,7‐disulfonic acid (AQDS)/1,2‐benzoquinone‐3,5‐disulfonic acid (BQDS) RFBs. The device can be directly charged by solar light without external bias, and discharged like normal RFBs with an energy storage density of 1.15 Wh L−1 and a solar‐to‐output electricity efficiency (SOEE) of 1.7 % over many cycles. The concept exploits a previously undeveloped design connecting two major energy technologies and promises a general approach for storing solar energy electrochemically with high theoretical storage capacity and efficiency.
Fließend gespeichert: Ein integrierter Energiespeicher nutzt Siliciumsolarzellen und organische Redoxflussbatterien. Der Prototyp enthält eine p+nn+‐Si/TiO2/Pt‐Photokathode und eine n+np+‐Si/TiO2/Pt‐Photoanode. Durch seine Leistungsfähigkeit könnte er einen allgemeinen, effizienten und kostengünstigen Weg für die elektrochemische Zwischenspeicherung von Sonnenenergie öffnen. |
| doi_str_mv | 10.1002/ange.201606986 |
| format | Article |
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Fließend gespeichert: Ein integrierter Energiespeicher nutzt Siliciumsolarzellen und organische Redoxflussbatterien. Der Prototyp enthält eine p+nn+‐Si/TiO2/Pt‐Photokathode und eine n+np+‐Si/TiO2/Pt‐Photoanode. Durch seine Leistungsfähigkeit könnte er einen allgemeinen, effizienten und kostengünstigen Weg für die elektrochemische Zwischenspeicherung von Sonnenenergie öffnen.</description><identifier>ISSN: 0044-8249</identifier><identifier>EISSN: 1521-3757</identifier><identifier>DOI: 10.1002/ange.201606986</identifier><language>eng</language><publisher>Weinheim: Blackwell Publishing Ltd</publisher><subject>Anthraquinone ; Batteries ; Benzoquinone ; Bias ; Buildings ; Chemistry ; Chinone ; Density ; Design ; Devices ; Direct power generation ; Electricity ; Electrochemistry ; Energy conversion ; Energy conversion efficiency ; Energy management ; Energy storage ; Energy technology ; Flow ; Integrierte Funktionseinheiten ; Light effects ; Photoelektrochemie ; Photovoltaic cells ; Quinones ; Rechargeable batteries ; Redoxflussbatterien ; Regenerative ; Silicon ; Solar cells ; Solar energy ; Solar energy conversion ; Solarenergie ; Storage capacity</subject><ispartof>Angewandte Chemie, 2016-10, Vol.128 (42), p.13298-13302</ispartof><rights>2016 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim</rights><rights>2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c2336-8177c9db5356aa7952fdbd7e4ad5f7ede1a140ea78d386780c3b4e9e69e0d68d3</citedby><cites>FETCH-LOGICAL-c2336-8177c9db5356aa7952fdbd7e4ad5f7ede1a140ea78d386780c3b4e9e69e0d68d3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1002%2Fange.201606986$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1002%2Fange.201606986$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>314,780,784,1417,27924,27925,45574,45575</link.rule.ids></links><search><creatorcontrib>Li, Wenjie</creatorcontrib><creatorcontrib>Fu, Hui-Chun</creatorcontrib><creatorcontrib>Li, Linsen</creatorcontrib><creatorcontrib>Cabán-Acevedo, Miguel</creatorcontrib><creatorcontrib>He, Jr-Hau</creatorcontrib><creatorcontrib>Jin, Song</creatorcontrib><title>Integrated Photoelectrochemical Solar Energy Conversion and Organic Redox Flow Battery Devices</title><title>Angewandte Chemie</title><addtitle>Angew. Chem</addtitle><description>Building on regenerative photoelectrochemical solar cells and emerging electrochemical redox flow batteries (RFBs), more efficient, scalable, compact, and cost‐effective hybrid energy conversion and storage devices could be realized. An integrated photoelectrochemical solar energy conversion and electrochemical storage device is developed by integrating regenerative silicon solar cells and 9,10‐anthraquinone‐2,7‐disulfonic acid (AQDS)/1,2‐benzoquinone‐3,5‐disulfonic acid (BQDS) RFBs. The device can be directly charged by solar light without external bias, and discharged like normal RFBs with an energy storage density of 1.15 Wh L−1 and a solar‐to‐output electricity efficiency (SOEE) of 1.7 % over many cycles. The concept exploits a previously undeveloped design connecting two major energy technologies and promises a general approach for storing solar energy electrochemically with high theoretical storage capacity and efficiency.
Fließend gespeichert: Ein integrierter Energiespeicher nutzt Siliciumsolarzellen und organische Redoxflussbatterien. Der Prototyp enthält eine p+nn+‐Si/TiO2/Pt‐Photokathode und eine n+np+‐Si/TiO2/Pt‐Photoanode. Durch seine Leistungsfähigkeit könnte er einen allgemeinen, effizienten und kostengünstigen Weg für die elektrochemische Zwischenspeicherung von Sonnenenergie öffnen.</description><subject>Anthraquinone</subject><subject>Batteries</subject><subject>Benzoquinone</subject><subject>Bias</subject><subject>Buildings</subject><subject>Chemistry</subject><subject>Chinone</subject><subject>Density</subject><subject>Design</subject><subject>Devices</subject><subject>Direct power generation</subject><subject>Electricity</subject><subject>Electrochemistry</subject><subject>Energy conversion</subject><subject>Energy conversion efficiency</subject><subject>Energy management</subject><subject>Energy storage</subject><subject>Energy technology</subject><subject>Flow</subject><subject>Integrierte Funktionseinheiten</subject><subject>Light effects</subject><subject>Photoelektrochemie</subject><subject>Photovoltaic cells</subject><subject>Quinones</subject><subject>Rechargeable batteries</subject><subject>Redoxflussbatterien</subject><subject>Regenerative</subject><subject>Silicon</subject><subject>Solar cells</subject><subject>Solar energy</subject><subject>Solar energy conversion</subject><subject>Solarenergie</subject><subject>Storage capacity</subject><issn>0044-8249</issn><issn>1521-3757</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2016</creationdate><recordtype>article</recordtype><recordid>eNqFkU1LAzEQhoMoWD-ungNevGxNdvOxOWqtVRQVq-jJkCbTurpNarJV--_dUhHx4mlgeJ5heF-E9ijpUkLyQ-Mn0M0JFUSoUqyhDuU5zQrJ5TrqEMJYVuZMbaKtlF4IISKXqoOezn0Dk2gacPjmOTQBarBNDPYZppU1NR6G2kTc9xAnC9wL_h1iqoLHxjt8HSfGVxbfgguf-LQOH_jYNA3EBT6B98pC2kEbY1Mn2P2e2-j-tH_XO8surwfnvaPLzOZFIbKSSmmVG_GCC2Ok4vnYjZwEZhwfS3BADWUEjCxdUQpZEluMGCgQCogT7XIbHazuzmJ4m0Nq9LRKFuraeAjzpGnJuFQFl7RF9_-gL2EeffudpooIVjJKl1R3RdkYUoow1rNYTU1caEr0Mm69jFv_xN0KaiV8VDUs_qH10dWg_9vNVm6VGvj8cU181UK2BeqHq4F-PL54UHx4q4fFF9S-k_U</recordid><startdate>20161010</startdate><enddate>20161010</enddate><creator>Li, Wenjie</creator><creator>Fu, Hui-Chun</creator><creator>Li, Linsen</creator><creator>Cabán-Acevedo, Miguel</creator><creator>He, Jr-Hau</creator><creator>Jin, Song</creator><general>Blackwell Publishing Ltd</general><general>Wiley Subscription Services, Inc</general><scope>BSCLL</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope></search><sort><creationdate>20161010</creationdate><title>Integrated Photoelectrochemical Solar Energy Conversion and Organic Redox Flow Battery Devices</title><author>Li, Wenjie ; Fu, Hui-Chun ; Li, Linsen ; Cabán-Acevedo, Miguel ; He, Jr-Hau ; Jin, Song</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c2336-8177c9db5356aa7952fdbd7e4ad5f7ede1a140ea78d386780c3b4e9e69e0d68d3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2016</creationdate><topic>Anthraquinone</topic><topic>Batteries</topic><topic>Benzoquinone</topic><topic>Bias</topic><topic>Buildings</topic><topic>Chemistry</topic><topic>Chinone</topic><topic>Density</topic><topic>Design</topic><topic>Devices</topic><topic>Direct power generation</topic><topic>Electricity</topic><topic>Electrochemistry</topic><topic>Energy conversion</topic><topic>Energy conversion efficiency</topic><topic>Energy management</topic><topic>Energy storage</topic><topic>Energy technology</topic><topic>Flow</topic><topic>Integrierte Funktionseinheiten</topic><topic>Light effects</topic><topic>Photoelektrochemie</topic><topic>Photovoltaic cells</topic><topic>Quinones</topic><topic>Rechargeable batteries</topic><topic>Redoxflussbatterien</topic><topic>Regenerative</topic><topic>Silicon</topic><topic>Solar cells</topic><topic>Solar energy</topic><topic>Solar energy conversion</topic><topic>Solarenergie</topic><topic>Storage capacity</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Li, Wenjie</creatorcontrib><creatorcontrib>Fu, Hui-Chun</creatorcontrib><creatorcontrib>Li, Linsen</creatorcontrib><creatorcontrib>Cabán-Acevedo, Miguel</creatorcontrib><creatorcontrib>He, Jr-Hau</creatorcontrib><creatorcontrib>Jin, Song</creatorcontrib><collection>Istex</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Angewandte Chemie</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Li, Wenjie</au><au>Fu, Hui-Chun</au><au>Li, Linsen</au><au>Cabán-Acevedo, Miguel</au><au>He, Jr-Hau</au><au>Jin, Song</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Integrated Photoelectrochemical Solar Energy Conversion and Organic Redox Flow Battery Devices</atitle><jtitle>Angewandte Chemie</jtitle><addtitle>Angew. Chem</addtitle><date>2016-10-10</date><risdate>2016</risdate><volume>128</volume><issue>42</issue><spage>13298</spage><epage>13302</epage><pages>13298-13302</pages><issn>0044-8249</issn><eissn>1521-3757</eissn><abstract>Building on regenerative photoelectrochemical solar cells and emerging electrochemical redox flow batteries (RFBs), more efficient, scalable, compact, and cost‐effective hybrid energy conversion and storage devices could be realized. An integrated photoelectrochemical solar energy conversion and electrochemical storage device is developed by integrating regenerative silicon solar cells and 9,10‐anthraquinone‐2,7‐disulfonic acid (AQDS)/1,2‐benzoquinone‐3,5‐disulfonic acid (BQDS) RFBs. The device can be directly charged by solar light without external bias, and discharged like normal RFBs with an energy storage density of 1.15 Wh L−1 and a solar‐to‐output electricity efficiency (SOEE) of 1.7 % over many cycles. The concept exploits a previously undeveloped design connecting two major energy technologies and promises a general approach for storing solar energy electrochemically with high theoretical storage capacity and efficiency.
Fließend gespeichert: Ein integrierter Energiespeicher nutzt Siliciumsolarzellen und organische Redoxflussbatterien. Der Prototyp enthält eine p+nn+‐Si/TiO2/Pt‐Photokathode und eine n+np+‐Si/TiO2/Pt‐Photoanode. Durch seine Leistungsfähigkeit könnte er einen allgemeinen, effizienten und kostengünstigen Weg für die elektrochemische Zwischenspeicherung von Sonnenenergie öffnen.</abstract><cop>Weinheim</cop><pub>Blackwell Publishing Ltd</pub><doi>10.1002/ange.201606986</doi><tpages>5</tpages></addata></record> |
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| subjects | Anthraquinone Batteries Benzoquinone Bias Buildings Chemistry Chinone Density Design Devices Direct power generation Electricity Electrochemistry Energy conversion Energy conversion efficiency Energy management Energy storage Energy technology Flow Integrierte Funktionseinheiten Light effects Photoelektrochemie Photovoltaic cells Quinones Rechargeable batteries Redoxflussbatterien Regenerative Silicon Solar cells Solar energy Solar energy conversion Solarenergie Storage capacity |
| title | Integrated Photoelectrochemical Solar Energy Conversion and Organic Redox Flow Battery Devices |
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