Application of a biosorbent to soil: a potential method for controlling water pollution by pesticides
Different strategies are now being optimized to prevent water from agricultural areas being contaminated by pesticides. The aim of this work was to optimize the adsorption of non-polar (tebuconazole, triadimenol) and polar (cymoxanil, pirimicarb) pesticides by soils after applying the biosorbent spe...
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| Veröffentlicht in: | Environmental science and pollution research international 2016-05, Vol.23 (9), p.9192-9203 |
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| creator | Álvarez-Martín, Alba Rodríguez-Cruz, M. Sonia Andrades, M. Soledad Sánchez-Martín, María J. |
| description | Different strategies are now being optimized to prevent water from agricultural areas being contaminated by pesticides. The aim of this work was to optimize the adsorption of non-polar (tebuconazole, triadimenol) and polar (cymoxanil, pirimicarb) pesticides by soils after applying the biosorbent spent mushroom substrate (SMS) at different rates. The adsorption isotherms of pesticides by three soils and SMS-amended soils were obtained and the adsorption constants were calculated. The distribution coefficients (
K
d
) increased 1.40–23.1 times (tebuconazole), 1.08–23.7 times (triadimenol), 1.31–42.1 times (cymoxanil), and 0.55–23.8 times (pirimicarb) for soils amended with biosorbent at rates between 2 and 75 %. Increasing the SMS rates led to a constant increase in adsorption efficiency for non-polar pesticides but not for polar pesticides, due to the increase in the organic carbon (OC) content of soils as indicated by
K
OC
values. The OC content of SMS-amended soils accounted for more than 90 % of the adsorption variability of non-polar pesticides, but it accounted for only 56.3 % for polar pesticides. The estimated adsorption of SMS-amended soils determined from the individual adsorption of soils and SMS was more consistent with real experimental values for non-polar pesticides than for polar pesticides. The results revealed the use of SMS as a tool to optimize pesticide adsorption by soils in dealing with specific contamination problems involving these compounds. |
| doi_str_mv | 10.1007/s11356-016-6132-4 |
| format | Article |
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K
d
) increased 1.40–23.1 times (tebuconazole), 1.08–23.7 times (triadimenol), 1.31–42.1 times (cymoxanil), and 0.55–23.8 times (pirimicarb) for soils amended with biosorbent at rates between 2 and 75 %. Increasing the SMS rates led to a constant increase in adsorption efficiency for non-polar pesticides but not for polar pesticides, due to the increase in the organic carbon (OC) content of soils as indicated by
K
OC
values. The OC content of SMS-amended soils accounted for more than 90 % of the adsorption variability of non-polar pesticides, but it accounted for only 56.3 % for polar pesticides. The estimated adsorption of SMS-amended soils determined from the individual adsorption of soils and SMS was more consistent with real experimental values for non-polar pesticides than for polar pesticides. The results revealed the use of SMS as a tool to optimize pesticide adsorption by soils in dealing with specific contamination problems involving these compounds.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-016-6132-4</identifier><identifier>PMID: 26832876</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Adsorption ; Agaricales - chemistry ; Agricultural pollution ; Agriculture ; Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; biosorbents ; Carbon ; cymoxanil ; Earth and Environmental Science ; Ecotoxicology ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Fungicides ; Insecticides ; Mushrooms ; Organic carbon ; Organic soils ; Pesticides ; Pesticides - analysis ; pirimicarb ; Research Article ; Soil - chemistry ; Soil adsorption ; Soil amendment ; Soil contamination ; Soil Pollutants - analysis ; Soil pollution ; spent mushroom compost ; Studies ; Tebuconazole ; Triadimenol ; Triazoles ; Waste Water Technology ; Water Management ; Water pollution ; Water Pollution - prevention & control ; Water Pollution Control ; Wineries & vineyards</subject><ispartof>Environmental science and pollution research international, 2016-05, Vol.23 (9), p.9192-9203</ispartof><rights>Springer-Verlag Berlin Heidelberg 2016</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c518t-a60742a5a690833246ffe7f538c1ec91d153f0f44fafcfb55769341e613136d83</citedby><cites>FETCH-LOGICAL-c518t-a60742a5a690833246ffe7f538c1ec91d153f0f44fafcfb55769341e613136d83</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-016-6132-4$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-016-6132-4$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/26832876$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Álvarez-Martín, Alba</creatorcontrib><creatorcontrib>Rodríguez-Cruz, M. Sonia</creatorcontrib><creatorcontrib>Andrades, M. Soledad</creatorcontrib><creatorcontrib>Sánchez-Martín, María J.</creatorcontrib><title>Application of a biosorbent to soil: a potential method for controlling water pollution by pesticides</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>Different strategies are now being optimized to prevent water from agricultural areas being contaminated by pesticides. The aim of this work was to optimize the adsorption of non-polar (tebuconazole, triadimenol) and polar (cymoxanil, pirimicarb) pesticides by soils after applying the biosorbent spent mushroom substrate (SMS) at different rates. The adsorption isotherms of pesticides by three soils and SMS-amended soils were obtained and the adsorption constants were calculated. The distribution coefficients (
K
d
) increased 1.40–23.1 times (tebuconazole), 1.08–23.7 times (triadimenol), 1.31–42.1 times (cymoxanil), and 0.55–23.8 times (pirimicarb) for soils amended with biosorbent at rates between 2 and 75 %. Increasing the SMS rates led to a constant increase in adsorption efficiency for non-polar pesticides but not for polar pesticides, due to the increase in the organic carbon (OC) content of soils as indicated by
K
OC
values. The OC content of SMS-amended soils accounted for more than 90 % of the adsorption variability of non-polar pesticides, but it accounted for only 56.3 % for polar pesticides. The estimated adsorption of SMS-amended soils determined from the individual adsorption of soils and SMS was more consistent with real experimental values for non-polar pesticides than for polar pesticides. The results revealed the use of SMS as a tool to optimize pesticide adsorption by soils in dealing with specific contamination problems involving these compounds.</description><subject>Adsorption</subject><subject>Agaricales - chemistry</subject><subject>Agricultural pollution</subject><subject>Agriculture</subject><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>biosorbents</subject><subject>Carbon</subject><subject>cymoxanil</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Fungicides</subject><subject>Insecticides</subject><subject>Mushrooms</subject><subject>Organic carbon</subject><subject>Organic soils</subject><subject>Pesticides</subject><subject>Pesticides - analysis</subject><subject>pirimicarb</subject><subject>Research Article</subject><subject>Soil - chemistry</subject><subject>Soil adsorption</subject><subject>Soil amendment</subject><subject>Soil contamination</subject><subject>Soil Pollutants - analysis</subject><subject>Soil pollution</subject><subject>spent mushroom compost</subject><subject>Studies</subject><subject>Tebuconazole</subject><subject>Triadimenol</subject><subject>Triazoles</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water pollution</subject><subject>Water Pollution - prevention & control</subject><subject>Water Pollution Control</subject><subject>Wineries & vineyards</subject><issn>0944-1344</issn><issn>1614-7499</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2016</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><sourceid>BENPR</sourceid><recordid>eNqNkU9rVTEQxYMo9rX6AdxIwI2bq5mb_-5K0SoU3Og65OYmNSXv5prkIv32zeurIoLQ1cDMb85w5iD0Csg7IES-rwCUi4GAGATQcWBP0A4EsEEyrZ-iHdGMDUAZO0Gntd4QMhI9yufoZBSKjkqKHfLn65qisy3mBeeALZ5irrlMfmm4ZVxzTB96d82td6JNeO_bjzzjkAt2eWklpxSXa_zLNl86ltJ2rzXd4tXXFl2cfX2BngWbqn_5UM_Q908fv118Hq6-Xn65OL8aHAfVBiuIZKPlVmiiKB2ZCMHLwKly4J2GGTgNJDAWbHBh4lwKTRn4bh6omBU9Q2-PumvJP7d-3uxjdT4lu_i8VQOKCtGN60egUh_ep-RjUMUl44SLjr75B73JW1m653sKBOfiIAhHypVca_HBrCXubbk1QMwhWXNM1vRkzSFZw_rO6wflbdr7-c_G7yg7MB6B2kfLtS9_nf6v6h102q0D</recordid><startdate>20160501</startdate><enddate>20160501</enddate><creator>Álvarez-Martín, Alba</creator><creator>Rodríguez-Cruz, M. 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Sonia</au><au>Andrades, M. Soledad</au><au>Sánchez-Martín, María J.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Application of a biosorbent to soil: a potential method for controlling water pollution by pesticides</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2016-05-01</date><risdate>2016</risdate><volume>23</volume><issue>9</issue><spage>9192</spage><epage>9203</epage><pages>9192-9203</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>Different strategies are now being optimized to prevent water from agricultural areas being contaminated by pesticides. The aim of this work was to optimize the adsorption of non-polar (tebuconazole, triadimenol) and polar (cymoxanil, pirimicarb) pesticides by soils after applying the biosorbent spent mushroom substrate (SMS) at different rates. The adsorption isotherms of pesticides by three soils and SMS-amended soils were obtained and the adsorption constants were calculated. The distribution coefficients (
K
d
) increased 1.40–23.1 times (tebuconazole), 1.08–23.7 times (triadimenol), 1.31–42.1 times (cymoxanil), and 0.55–23.8 times (pirimicarb) for soils amended with biosorbent at rates between 2 and 75 %. Increasing the SMS rates led to a constant increase in adsorption efficiency for non-polar pesticides but not for polar pesticides, due to the increase in the organic carbon (OC) content of soils as indicated by
K
OC
values. The OC content of SMS-amended soils accounted for more than 90 % of the adsorption variability of non-polar pesticides, but it accounted for only 56.3 % for polar pesticides. The estimated adsorption of SMS-amended soils determined from the individual adsorption of soils and SMS was more consistent with real experimental values for non-polar pesticides than for polar pesticides. The results revealed the use of SMS as a tool to optimize pesticide adsorption by soils in dealing with specific contamination problems involving these compounds.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>26832876</pmid><doi>10.1007/s11356-016-6132-4</doi><tpages>12</tpages><oa>free_for_read</oa></addata></record> |
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| ispartof | Environmental science and pollution research international, 2016-05, Vol.23 (9), p.9192-9203 |
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| source | MEDLINE; Springer Nature - Complete Springer Journals |
| subjects | Adsorption Agaricales - chemistry Agricultural pollution Agriculture Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution biosorbents Carbon cymoxanil Earth and Environmental Science Ecotoxicology Environment Environmental Chemistry Environmental Health Environmental science Fungicides Insecticides Mushrooms Organic carbon Organic soils Pesticides Pesticides - analysis pirimicarb Research Article Soil - chemistry Soil adsorption Soil amendment Soil contamination Soil Pollutants - analysis Soil pollution spent mushroom compost Studies Tebuconazole Triadimenol Triazoles Waste Water Technology Water Management Water pollution Water Pollution - prevention & control Water Pollution Control Wineries & vineyards |
| title | Application of a biosorbent to soil: a potential method for controlling water pollution by pesticides |
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