Molecular Dynamics of Flexible Polar Cations in a Variable Confined Space: Toward Exceptional Two-Step Nonlinear Optical Switches

Molecular Dynamics of Flexible Polar Cations in a Variable Confined Space: Toward Exceptional Two-Step Nonlinear Optical Switches

The changeable molecular dynamics of flexible polar cations in the variable confined space between inorganic chains brings about a new type of two‐step nonlinear optical (NLO) switch with genuine “off–on–off” second harmonic generation (SHG) conversion between one NLO‐active state and two NLO‐inacti...

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Veröffentlicht in:Advanced materials (Weinheim) 2016-07, Vol.28 (28), p.5886-5890
Hauptverfasser: Xu, Wei-Jian, He, Chun-Ting, Ji, Cheng-Min, Chen, Shao-Li, Huang, Rui-Kang, Lin, Rui-Biao, Xue, Wei, Luo, Jun-Hua, Zhang, Wei-Xiong, Chen, Xiao-Ming
Format: Artikel
Sprache:eng
Schlagworte:
Cations
Confined environments
Conversion
ferroelectrics
flexible polar cations
Molecular dynamics
nonlinear optical switches
Nonlinearity
Optical switching
phase transitions
Second harmonic generation
Switches
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Zusammenfassung:The changeable molecular dynamics of flexible polar cations in the variable confined space between inorganic chains brings about a new type of two‐step nonlinear optical (NLO) switch with genuine “off–on–off” second harmonic generation (SHG) conversion between one NLO‐active state and two NLO‐inactive states.
ISSN:0935-9648
1521-4095
DOI:10.1002/adma.201600895