Overcoming the Interface Losses in Planar Heterojunction Perovskite-Based Solar Cells

A scalable, hysteresis‐free and planar architecture perovskite solar cell is presented, employing a flame spray synthesized low‐temperature processed NiO (LT‐NiO) as hole‐transporting layer yielding efficiencies close to 18%. Importantly, it is found that LT‐NiO boosts the limits of open‐circuit vol...

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Veröffentlicht in:Advanced materials (Weinheim) 2016-07, Vol.28 (25), p.5112-5120
Hauptverfasser: Hou, Yi, Chen, Wei, Baran, Derya, Stubhan, Tobias, Luechinger, Norman A., Hartmeier, Benjamin, Richter, Moses, Min, Jie, Chen, Shi, Quiroz, Cesar Omar Ramirez, Li, Ning, Zhang, Hong, Heumueller, Thomas, Matt, Gebhard J., Osvet, Andres, Forberich, Karen, Zhang, Zhi-Guo, Li, Yongfang, Winter, Benjamin, Schweizer, Peter, Spiecker, Erdmann, Brabec, Christoph J.
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container_end_page 5120
container_issue 25
container_start_page 5112
container_title Advanced materials (Weinheim)
container_volume 28
creator Hou, Yi
Chen, Wei
Baran, Derya
Stubhan, Tobias
Luechinger, Norman A.
Hartmeier, Benjamin
Richter, Moses
Min, Jie
Chen, Shi
Quiroz, Cesar Omar Ramirez
Li, Ning
Zhang, Hong
Heumueller, Thomas
Matt, Gebhard J.
Osvet, Andres
Forberich, Karen
Zhang, Zhi-Guo
Li, Yongfang
Winter, Benjamin
Schweizer, Peter
Spiecker, Erdmann
Brabec, Christoph J.
description A scalable, hysteresis‐free and planar architecture perovskite solar cell is presented, employing a flame spray synthesized low‐temperature processed NiO (LT‐NiO) as hole‐transporting layer yielding efficiencies close to 18%. Importantly, it is found that LT‐NiO boosts the limits of open‐circuit voltages toward an impressive non‐radiative voltage loss of 0.226 V only, whereas PEDOT:PSS suffers from significant large non‐radiative recombination losses.
doi_str_mv 10.1002/adma.201504168
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source Wiley Online Library Journals Frontfile Complete
subjects Architecture (computers)
Electric potential
Heterojunctions
low temperature processing
nickel oxide
non-radiative voltage loss
perovskite solar cells
Photovoltaic cells
Solar cells
Sprayers
Sprays
Voltage
title Overcoming the Interface Losses in Planar Heterojunction Perovskite-Based Solar Cells
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