Preparation of platinum catalysts supported on functionalized graphene and the electrocatalytic properties for ethanol oxidation in direct ethanol fuel cell
In this work, we develop a facile method under mild conditions to synthesize 2-aminoethanesulfonic acid (taurine)-functionalized-graphene (T-fGN) and to prepare Pt catalysts supported on T-fGN through a self-assembly route. The structure, morphologies and electrochemical properties of T-fGN and Pt/T...
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| Veröffentlicht in: | Journal of materials science. Materials in electronics 2016-06, Vol.27 (6), p.6208-6215 |
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| container_title | Journal of materials science. Materials in electronics |
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| creator | Li, Yanhong Han, Lu An, Baigang Wang, Yiyong Wang, Lin Yin, Xitao Lu, Jinlin |
| description | In this work, we develop a facile method under mild conditions to synthesize 2-aminoethanesulfonic acid (taurine)-functionalized-graphene (T-fGN) and to prepare Pt catalysts supported on T-fGN through a self-assembly route. The structure, morphologies and electrochemical properties of T-fGN and Pt/T-fGN were examined by atomic force microscope, X-ray photoelectron spectroscopy, Fourier transform infrared spectroscopy and different electrochemical techniques. The electrocatalytic properties of Pt/T-fGN were investigated for ethanol oxidation reaction (EOR) in comparison to Pt supported on Vulcan XC-72 (Pt/VC). The results indicate that the as-prepared Pt/T-fGN catalyst possesses a much higher electrocatalytic activity, faster reaction kinetics and a better stability for EOR than Pt/VC. |
| doi_str_mv | 10.1007/s10854-016-4551-0 |
| format | Article |
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The structure, morphologies and electrochemical properties of T-fGN and Pt/T-fGN were examined by atomic force microscope, X-ray photoelectron spectroscopy, Fourier transform infrared spectroscopy and different electrochemical techniques. The electrocatalytic properties of Pt/T-fGN were investigated for ethanol oxidation reaction (EOR) in comparison to Pt supported on Vulcan XC-72 (Pt/VC). The results indicate that the as-prepared Pt/T-fGN catalyst possesses a much higher electrocatalytic activity, faster reaction kinetics and a better stability for EOR than Pt/VC.</description><identifier>ISSN: 0957-4522</identifier><identifier>EISSN: 1573-482X</identifier><identifier>DOI: 10.1007/s10854-016-4551-0</identifier><language>eng</language><publisher>New York: Springer US</publisher><subject>Catalysis ; Catalysts ; Characterization and Evaluation of Materials ; Chemistry and Materials Science ; Ethanol ; Ethyl alcohol ; Graphene ; Materials Science ; Optical and Electronic Materials ; Oxidation ; Platinum ; Self assembly</subject><ispartof>Journal of materials science. 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Materials in electronics</title><addtitle>J Mater Sci: Mater Electron</addtitle><description>In this work, we develop a facile method under mild conditions to synthesize 2-aminoethanesulfonic acid (taurine)-functionalized-graphene (T-fGN) and to prepare Pt catalysts supported on T-fGN through a self-assembly route. The structure, morphologies and electrochemical properties of T-fGN and Pt/T-fGN were examined by atomic force microscope, X-ray photoelectron spectroscopy, Fourier transform infrared spectroscopy and different electrochemical techniques. The electrocatalytic properties of Pt/T-fGN were investigated for ethanol oxidation reaction (EOR) in comparison to Pt supported on Vulcan XC-72 (Pt/VC). The results indicate that the as-prepared Pt/T-fGN catalyst possesses a much higher electrocatalytic activity, faster reaction kinetics and a better stability for EOR than Pt/VC.</description><subject>Catalysis</subject><subject>Catalysts</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemistry and Materials Science</subject><subject>Ethanol</subject><subject>Ethyl alcohol</subject><subject>Graphene</subject><subject>Materials Science</subject><subject>Optical and Electronic Materials</subject><subject>Oxidation</subject><subject>Platinum</subject><subject>Self assembly</subject><issn>0957-4522</issn><issn>1573-482X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2016</creationdate><recordtype>article</recordtype><sourceid>AFKRA</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><recordid>eNp1kc9qFTEUxoNY8Fp9AHcBN27G5s8kk1lK0SoUdGHBXchkTnpTcpMxyYDts_iwzTBSRHCVQ87v-87hfAi9oeQ9JWS4KJQo0XeEyq4XgnbkGTpQMfCuV-zHc3Qgoxhah7EX6GUpd4QQ2XN1QL-_ZVhMNtWniJPDS2hlXE_YmmrCfakFl3VZUq4w44a4NdqNNcE_tJ_bbJYjRMAmzrgeAUMAW3Pa1dVbvOS0QK4eCnYpY6hHE1PA6Zef96E-4tnnpnrquRUCthDCK3TmTCjw-s97jm4-ffx--bm7_nr15fLDdWe5krVjo3TOzmYiXBpBnSUDo8CncRKz4paogUgQXAzM0pHxfuQOgE7KUDvNUjB-jt7tvm3ZnyuUqk--bAuYCGktmioqCWVjTxr69h_0Lq25naNRg5LtwpT1jaI7ZXMqJYPTS_Ynk-81JXrLS-956ZaX3vLSmzPbNaWx8RbyX87_FT0CdgOcTQ</recordid><startdate>20160601</startdate><enddate>20160601</enddate><creator>Li, Yanhong</creator><creator>Han, Lu</creator><creator>An, Baigang</creator><creator>Wang, Yiyong</creator><creator>Wang, Lin</creator><creator>Yin, Xitao</creator><creator>Lu, Jinlin</creator><general>Springer US</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7SR</scope><scope>8BQ</scope><scope>8FD</scope><scope>8FE</scope><scope>8FG</scope><scope>ABJCF</scope><scope>AFKRA</scope><scope>ARAPS</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>F28</scope><scope>FR3</scope><scope>HCIFZ</scope><scope>JG9</scope><scope>KB.</scope><scope>L7M</scope><scope>P5Z</scope><scope>P62</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>S0W</scope></search><sort><creationdate>20160601</creationdate><title>Preparation of platinum catalysts supported on functionalized graphene and the electrocatalytic properties for ethanol oxidation in direct ethanol fuel cell</title><author>Li, Yanhong ; Han, Lu ; An, Baigang ; Wang, Yiyong ; Wang, Lin ; Yin, Xitao ; Lu, Jinlin</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c386t-296ffcdab036a51fc0721e3b9b5d83c08706e53572c1923493fee1b8a1cbd6523</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2016</creationdate><topic>Catalysis</topic><topic>Catalysts</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemistry and Materials Science</topic><topic>Ethanol</topic><topic>Ethyl alcohol</topic><topic>Graphene</topic><topic>Materials Science</topic><topic>Optical and Electronic Materials</topic><topic>Oxidation</topic><topic>Platinum</topic><topic>Self assembly</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Li, Yanhong</creatorcontrib><creatorcontrib>Han, Lu</creatorcontrib><creatorcontrib>An, Baigang</creatorcontrib><creatorcontrib>Wang, Yiyong</creatorcontrib><creatorcontrib>Wang, Lin</creatorcontrib><creatorcontrib>Yin, Xitao</creatorcontrib><creatorcontrib>Lu, Jinlin</creatorcontrib><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>Materials Science & Engineering Collection</collection><collection>ProQuest Central UK/Ireland</collection><collection>Advanced Technologies & Aerospace Collection</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central</collection><collection>ANTE: Abstracts in New Technology & Engineering</collection><collection>Engineering Research Database</collection><collection>SciTech Premium Collection (Proquest) (PQ_SDU_P3)</collection><collection>Materials Research Database</collection><collection>ProQuest Materials Science Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>ProQuest Advanced Technologies & Aerospace Database</collection><collection>ProQuest Advanced Technologies & Aerospace Collection</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>DELNET Engineering & Technology Collection</collection><jtitle>Journal of materials science. Materials in electronics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Li, Yanhong</au><au>Han, Lu</au><au>An, Baigang</au><au>Wang, Yiyong</au><au>Wang, Lin</au><au>Yin, Xitao</au><au>Lu, Jinlin</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Preparation of platinum catalysts supported on functionalized graphene and the electrocatalytic properties for ethanol oxidation in direct ethanol fuel cell</atitle><jtitle>Journal of materials science. Materials in electronics</jtitle><stitle>J Mater Sci: Mater Electron</stitle><date>2016-06-01</date><risdate>2016</risdate><volume>27</volume><issue>6</issue><spage>6208</spage><epage>6215</epage><pages>6208-6215</pages><issn>0957-4522</issn><eissn>1573-482X</eissn><abstract>In this work, we develop a facile method under mild conditions to synthesize 2-aminoethanesulfonic acid (taurine)-functionalized-graphene (T-fGN) and to prepare Pt catalysts supported on T-fGN through a self-assembly route. The structure, morphologies and electrochemical properties of T-fGN and Pt/T-fGN were examined by atomic force microscope, X-ray photoelectron spectroscopy, Fourier transform infrared spectroscopy and different electrochemical techniques. The electrocatalytic properties of Pt/T-fGN were investigated for ethanol oxidation reaction (EOR) in comparison to Pt supported on Vulcan XC-72 (Pt/VC). The results indicate that the as-prepared Pt/T-fGN catalyst possesses a much higher electrocatalytic activity, faster reaction kinetics and a better stability for EOR than Pt/VC.</abstract><cop>New York</cop><pub>Springer US</pub><doi>10.1007/s10854-016-4551-0</doi><tpages>8</tpages></addata></record> |
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| subjects | Catalysis Catalysts Characterization and Evaluation of Materials Chemistry and Materials Science Ethanol Ethyl alcohol Graphene Materials Science Optical and Electronic Materials Oxidation Platinum Self assembly |
| title | Preparation of platinum catalysts supported on functionalized graphene and the electrocatalytic properties for ethanol oxidation in direct ethanol fuel cell |
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