Femtosecond Stimulated Raman Exposes the Role of Vibrational Coherence in Condensed-Phase Photoreactivity

Femtosecond spectroscopy has revealed coherent wave packet motion time and time again, but the question as to whether these coherences are necessary for reactivity or merely a consequence of the experiment has remained open. For diatomic systems in the gas phase, such as sodium iodide, the dimension...

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Veröffentlicht in:	Accounts of chemical research 2016-04, Vol.49 (4), p.616-625
Hauptverfasser:	Hoffman, David P, Mathies, Richard A
Format:	Artikel
Sprache:	eng
Schlagworte:	Anharmonicity Coherence Condensing Coupling Dynamical systems Dynamics Excitation Internal conversion
Online-Zugang:	Volltext
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