Effective degradation of rhodamine B by electro-Fenton process, using ferromagnetic nanoparticles loaded on modified graphite felt electrode as reusable catalyst: in neutral pH condition and without external aeration
Polytetrafluoroethylene/ferromagnetic nanoparticle/carbon black (PTFE/MNP/CB)-modified graphite felt (GF) was successfully applied as cathode for the mineralization of rhodamine B (RhB) in electro-Fenton (EF) process. The modified cathode showed high decolorization efficiency for RhB solution even i...
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| Veröffentlicht in: | Environmental science and pollution research international 2016-08, Vol.23 (15), p.15471-15482 |
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| creator | Tian, Jiangnan Zhao, Jixiang Olajuyin, Ayobami Matthew Sharshar, Moustafa Mohamed Mu, Tingzhen Yang, Maohua Xing, Jianmin |
| description | Polytetrafluoroethylene/ferromagnetic nanoparticle/carbon black (PTFE/MNP/CB)-modified graphite felt (GF) was successfully applied as cathode for the mineralization of rhodamine B (RhB) in electro-Fenton (EF) process. The modified cathode showed high decolorization efficiency for RhB solution even in neutral pH condition and without external aeration, achieving nearly complete decolorization and 89.52 % total organic carbon (TOC) removal after 270-min oxidation with the MNP load 1.2 g at 50 A/m
2
. Moreover, the operational parameters (current density, MNP load, initial pH, and airflow rate) were optimized. After that, adsorption isotherm was also conducted to compare the absorption quantity of CB and carbon nanotube (CNT). Then, the surface morphologies of MNPs were characterized by transmission electron microscope (TEM), energy-dispersive X-ray detector (EDX), and Fourier transform infrared spectroscopy (FTIR); and the modified cathode was characterized by SEM and contact angle. Finally, the stability and reusability of modified cathode were tested. Result uncovered that the PTFE/MNP/CB-modified cathode has the potential for industrial application and the solution after treatment was easily biodegradable. |
| doi_str_mv | 10.1007/s11356-016-6721-2 |
| format | Article |
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2
. Moreover, the operational parameters (current density, MNP load, initial pH, and airflow rate) were optimized. After that, adsorption isotherm was also conducted to compare the absorption quantity of CB and carbon nanotube (CNT). Then, the surface morphologies of MNPs were characterized by transmission electron microscope (TEM), energy-dispersive X-ray detector (EDX), and Fourier transform infrared spectroscopy (FTIR); and the modified cathode was characterized by SEM and contact angle. Finally, the stability and reusability of modified cathode were tested. Result uncovered that the PTFE/MNP/CB-modified cathode has the potential for industrial application and the solution after treatment was easily biodegradable.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-016-6721-2</identifier><identifier>PMID: 27117155</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Adsorption ; Aeration ; Air flow ; Aquatic Pollution ; Aqueous solutions ; Atmospheric Protection/Air Quality Control/Air Pollution ; Biodegradation ; Black carbon ; Carbon ; Carbon black ; Catalysis ; Catalysts ; Contact angle ; Decolorization ; Earth and Environmental Science ; Ecotoxicology ; Electrochemical Techniques - methods ; Electrodes ; Electrons ; Engineering ; Environment ; Environmental Chemistry ; Environmental Health ; Fourier transforms ; Graphite ; Graphite - chemistry ; Hydrogen Peroxide - chemistry ; Hydrogen-Ion Concentration ; Industrial applications ; Infrared spectroscopy ; Iron - chemistry ; Load distribution ; Magnetite Nanoparticles - chemistry ; Mineralization ; Nanoparticles ; Organic carbon ; Organic loading ; Oxidation ; Oxidation-Reduction ; pH effects ; Polytetrafluoroethylene ; Research Article ; Rhodamine ; Rhodamines - analysis ; Total organic carbon ; Waste Water Technology ; Water Management ; Water Pollutants, Chemical - analysis ; Water Pollution Control ; Water Purification - methods</subject><ispartof>Environmental science and pollution research international, 2016-08, Vol.23 (15), p.15471-15482</ispartof><rights>Springer-Verlag Berlin Heidelberg 2016</rights><rights>Environmental Science and Pollution Research is a copyright of Springer, 2016.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c442t-d67f7ba610287e09ec6ebe816b5ede942276221cf911c7318a198fcaeccf310a3</citedby><cites>FETCH-LOGICAL-c442t-d67f7ba610287e09ec6ebe816b5ede942276221cf911c7318a198fcaeccf310a3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-016-6721-2$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-016-6721-2$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/27117155$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Tian, Jiangnan</creatorcontrib><creatorcontrib>Zhao, Jixiang</creatorcontrib><creatorcontrib>Olajuyin, Ayobami Matthew</creatorcontrib><creatorcontrib>Sharshar, Moustafa Mohamed</creatorcontrib><creatorcontrib>Mu, Tingzhen</creatorcontrib><creatorcontrib>Yang, Maohua</creatorcontrib><creatorcontrib>Xing, Jianmin</creatorcontrib><title>Effective degradation of rhodamine B by electro-Fenton process, using ferromagnetic nanoparticles loaded on modified graphite felt electrode as reusable catalyst: in neutral pH condition and without external aeration</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>Polytetrafluoroethylene/ferromagnetic nanoparticle/carbon black (PTFE/MNP/CB)-modified graphite felt (GF) was successfully applied as cathode for the mineralization of rhodamine B (RhB) in electro-Fenton (EF) process. The modified cathode showed high decolorization efficiency for RhB solution even in neutral pH condition and without external aeration, achieving nearly complete decolorization and 89.52 % total organic carbon (TOC) removal after 270-min oxidation with the MNP load 1.2 g at 50 A/m
2
. Moreover, the operational parameters (current density, MNP load, initial pH, and airflow rate) were optimized. After that, adsorption isotherm was also conducted to compare the absorption quantity of CB and carbon nanotube (CNT). Then, the surface morphologies of MNPs were characterized by transmission electron microscope (TEM), energy-dispersive X-ray detector (EDX), and Fourier transform infrared spectroscopy (FTIR); and the modified cathode was characterized by SEM and contact angle. Finally, the stability and reusability of modified cathode were tested. Result uncovered that the PTFE/MNP/CB-modified cathode has the potential for industrial application and the solution after treatment was easily biodegradable.</description><subject>Adsorption</subject><subject>Aeration</subject><subject>Air flow</subject><subject>Aquatic Pollution</subject><subject>Aqueous solutions</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Biodegradation</subject><subject>Black carbon</subject><subject>Carbon</subject><subject>Carbon black</subject><subject>Catalysis</subject><subject>Catalysts</subject><subject>Contact angle</subject><subject>Decolorization</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Electrochemical Techniques - methods</subject><subject>Electrodes</subject><subject>Electrons</subject><subject>Engineering</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Fourier transforms</subject><subject>Graphite</subject><subject>Graphite - 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Academic</collection><jtitle>Environmental science and pollution research international</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Tian, Jiangnan</au><au>Zhao, Jixiang</au><au>Olajuyin, Ayobami Matthew</au><au>Sharshar, Moustafa Mohamed</au><au>Mu, Tingzhen</au><au>Yang, Maohua</au><au>Xing, Jianmin</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Effective degradation of rhodamine B by electro-Fenton process, using ferromagnetic nanoparticles loaded on modified graphite felt electrode as reusable catalyst: in neutral pH condition and without external aeration</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2016-08-01</date><risdate>2016</risdate><volume>23</volume><issue>15</issue><spage>15471</spage><epage>15482</epage><pages>15471-15482</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>Polytetrafluoroethylene/ferromagnetic nanoparticle/carbon black (PTFE/MNP/CB)-modified graphite felt (GF) was successfully applied as cathode for the mineralization of rhodamine B (RhB) in electro-Fenton (EF) process. The modified cathode showed high decolorization efficiency for RhB solution even in neutral pH condition and without external aeration, achieving nearly complete decolorization and 89.52 % total organic carbon (TOC) removal after 270-min oxidation with the MNP load 1.2 g at 50 A/m
2
. Moreover, the operational parameters (current density, MNP load, initial pH, and airflow rate) were optimized. After that, adsorption isotherm was also conducted to compare the absorption quantity of CB and carbon nanotube (CNT). Then, the surface morphologies of MNPs were characterized by transmission electron microscope (TEM), energy-dispersive X-ray detector (EDX), and Fourier transform infrared spectroscopy (FTIR); and the modified cathode was characterized by SEM and contact angle. Finally, the stability and reusability of modified cathode were tested. Result uncovered that the PTFE/MNP/CB-modified cathode has the potential for industrial application and the solution after treatment was easily biodegradable.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>27117155</pmid><doi>10.1007/s11356-016-6721-2</doi><tpages>12</tpages></addata></record> |
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| subjects | Adsorption Aeration Air flow Aquatic Pollution Aqueous solutions Atmospheric Protection/Air Quality Control/Air Pollution Biodegradation Black carbon Carbon Carbon black Catalysis Catalysts Contact angle Decolorization Earth and Environmental Science Ecotoxicology Electrochemical Techniques - methods Electrodes Electrons Engineering Environment Environmental Chemistry Environmental Health Fourier transforms Graphite Graphite - chemistry Hydrogen Peroxide - chemistry Hydrogen-Ion Concentration Industrial applications Infrared spectroscopy Iron - chemistry Load distribution Magnetite Nanoparticles - chemistry Mineralization Nanoparticles Organic carbon Organic loading Oxidation Oxidation-Reduction pH effects Polytetrafluoroethylene Research Article Rhodamine Rhodamines - analysis Total organic carbon Waste Water Technology Water Management Water Pollutants, Chemical - analysis Water Pollution Control Water Purification - methods |
| title | Effective degradation of rhodamine B by electro-Fenton process, using ferromagnetic nanoparticles loaded on modified graphite felt electrode as reusable catalyst: in neutral pH condition and without external aeration |
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