A Comparative Study on Activated Carbons Derived from a Broad Range of Agro-industrial Wastes in Removal of Large-Molecular-Size Organic Pollutants in Aqueous Phase
Microporous–mesoporous activated carbons from five different types of agro-industrial wastes were produced using chemical activation with ZnCl 2 and carbonization at mild conditions of 600 °C, comprehensively characterized and investigated for removal of methylene blue (MB) in aqueous solution, a mo...
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| Veröffentlicht in: | Water, air, and soil pollution air, and soil pollution, 2015-07, Vol.226 (7), p.1-15, Article 214 |
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| creator | Cruz, G. J. F. Matějová, L. Pirilä, M. Ainassaari, K. Canepa, C. A. Solis, J. Cruz, J.F. Šolcová, O. Keiski, R. L. |
| description | Microporous–mesoporous activated carbons from five different types of agro-industrial wastes were produced using chemical activation with ZnCl
2
and carbonization at mild conditions of 600 °C, comprehensively characterized and investigated for removal of methylene blue (MB) in aqueous solution, a model large-molecular-size organic pollutant. The external part of the mango pit (mango seed husk) was used for the production of activated carbon (AC) for the first time. Despite that the raw agro-materials exhibited significantly different porosity, all activated carbons produced possessed well-developed microporous–mesoporous structures showing high surface areas and micropore volumes. Further, it was revealed that the pore size distribution of raw agro-material is a more important property in development of microporous–mesoporous structure of produced ACs than their overall porosity. All activated carbons produced adsorbed MB, reaching in most cases 100 % removal from the aqueous phase. Adsorption data were fitted well to a pseudo-second-order kinetic model. For MB adsorption, the mesoporosity and the ratio of micropores accessible for MB were the key factors since there exists the size-selectivity effect on MB adsorption due to MB molecular dimensions. The molecular dimensions of MB were estimated via DFT calculations to 1.66 × 0.82 × 0.54 nm, and this parameter was correlated with determined micropore size distributions of activated carbons. |
| doi_str_mv | 10.1007/s11270-015-2474-7 |
| format | Article |
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2
and carbonization at mild conditions of 600 °C, comprehensively characterized and investigated for removal of methylene blue (MB) in aqueous solution, a model large-molecular-size organic pollutant. The external part of the mango pit (mango seed husk) was used for the production of activated carbon (AC) for the first time. Despite that the raw agro-materials exhibited significantly different porosity, all activated carbons produced possessed well-developed microporous–mesoporous structures showing high surface areas and micropore volumes. Further, it was revealed that the pore size distribution of raw agro-material is a more important property in development of microporous–mesoporous structure of produced ACs than their overall porosity. All activated carbons produced adsorbed MB, reaching in most cases 100 % removal from the aqueous phase. Adsorption data were fitted well to a pseudo-second-order kinetic model. For MB adsorption, the mesoporosity and the ratio of micropores accessible for MB were the key factors since there exists the size-selectivity effect on MB adsorption due to MB molecular dimensions. The molecular dimensions of MB were estimated via DFT calculations to 1.66 × 0.82 × 0.54 nm, and this parameter was correlated with determined micropore size distributions of activated carbons.</description><identifier>ISSN: 0049-6979</identifier><identifier>EISSN: 1573-2932</identifier><identifier>DOI: 10.1007/s11270-015-2474-7</identifier><language>eng</language><publisher>Cham: Springer International Publishing</publisher><subject>Activated carbon ; Adsorption ; Agricultural pollution ; Agricultural production ; Agricultural wastes ; Analysis ; Atmospheric Protection/Air Quality Control/Air Pollution ; Biomass ; Bioremediation ; Climate Change/Climate Change Impacts ; Cocoa ; Coffee ; Comparative studies ; Earth and Environmental Science ; Environment ; Environmental monitoring ; Hydrogeology ; Industrial wastes ; Mangifera indica ; Methylene blue ; Pollutants ; Pore size ; Porosity ; Raw materials ; Size distribution ; Soil Science & Conservation ; Studies ; Water Quality/Water Pollution</subject><ispartof>Water, air, and soil pollution, 2015-07, Vol.226 (7), p.1-15, Article 214</ispartof><rights>Springer International Publishing Switzerland 2015</rights><rights>COPYRIGHT 2015 Springer</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c388t-70652920c724c00805aa3014ab2535db179a618be35670ada3e315505fcd949b3</citedby><cites>FETCH-LOGICAL-c388t-70652920c724c00805aa3014ab2535db179a618be35670ada3e315505fcd949b3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11270-015-2474-7$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11270-015-2474-7$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,777,781,27905,27906,41469,42538,51300</link.rule.ids></links><search><creatorcontrib>Cruz, G. J. F.</creatorcontrib><creatorcontrib>Matějová, L.</creatorcontrib><creatorcontrib>Pirilä, M.</creatorcontrib><creatorcontrib>Ainassaari, K.</creatorcontrib><creatorcontrib>Canepa, C. A.</creatorcontrib><creatorcontrib>Solis, J.</creatorcontrib><creatorcontrib>Cruz, J.F.</creatorcontrib><creatorcontrib>Šolcová, O.</creatorcontrib><creatorcontrib>Keiski, R. L.</creatorcontrib><title>A Comparative Study on Activated Carbons Derived from a Broad Range of Agro-industrial Wastes in Removal of Large-Molecular-Size Organic Pollutants in Aqueous Phase</title><title>Water, air, and soil pollution</title><addtitle>Water Air Soil Pollut</addtitle><description>Microporous–mesoporous activated carbons from five different types of agro-industrial wastes were produced using chemical activation with ZnCl
2
and carbonization at mild conditions of 600 °C, comprehensively characterized and investigated for removal of methylene blue (MB) in aqueous solution, a model large-molecular-size organic pollutant. The external part of the mango pit (mango seed husk) was used for the production of activated carbon (AC) for the first time. Despite that the raw agro-materials exhibited significantly different porosity, all activated carbons produced possessed well-developed microporous–mesoporous structures showing high surface areas and micropore volumes. Further, it was revealed that the pore size distribution of raw agro-material is a more important property in development of microporous–mesoporous structure of produced ACs than their overall porosity. All activated carbons produced adsorbed MB, reaching in most cases 100 % removal from the aqueous phase. Adsorption data were fitted well to a pseudo-second-order kinetic model. For MB adsorption, the mesoporosity and the ratio of micropores accessible for MB were the key factors since there exists the size-selectivity effect on MB adsorption due to MB molecular dimensions. The molecular dimensions of MB were estimated via DFT calculations to 1.66 × 0.82 × 0.54 nm, and this parameter was correlated with determined micropore size distributions of activated carbons.</description><subject>Activated carbon</subject><subject>Adsorption</subject><subject>Agricultural pollution</subject><subject>Agricultural production</subject><subject>Agricultural wastes</subject><subject>Analysis</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Biomass</subject><subject>Bioremediation</subject><subject>Climate Change/Climate Change Impacts</subject><subject>Cocoa</subject><subject>Coffee</subject><subject>Comparative studies</subject><subject>Earth and Environmental Science</subject><subject>Environment</subject><subject>Environmental monitoring</subject><subject>Hydrogeology</subject><subject>Industrial wastes</subject><subject>Mangifera indica</subject><subject>Methylene blue</subject><subject>Pollutants</subject><subject>Pore size</subject><subject>Porosity</subject><subject>Raw materials</subject><subject>Size distribution</subject><subject>Soil Science & Conservation</subject><subject>Studies</subject><subject>Water Quality/Water Pollution</subject><issn>0049-6979</issn><issn>1573-2932</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2015</creationdate><recordtype>article</recordtype><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNp1kU-P1CAYhxujiePqB_BG4sULuy-lDHCs4581GbObXY1H8pbSyqaFEdpN1s_jB5VxPBgT4UB48zzwS35V9ZLBOQOQF5mxWgIFJmjdyIbKR9WGCclprXn9uNoANJputdRPq2c530FZWslN9bMluzgfMOHi7x25Xdb-gcRAWlvuuLie7DB1MWTy1qVC9GRIcSZI3qSIPbnBMDoSB9KOKVIf-jUvyeNEvmJeXCY-kBs3x_syKdAe0-jopzg5u06Y6K3_4chVGjF4S67jNK0LhuW31X5fXVwzuf6G2T2vngw4Zffiz3lWfXn_7vPuku6vPnzctXtquVILlbAVta7ByrqxAAoEIgfWYFcLLvqOSY1bpjrHxVYC9sgdZ0KAGGyvG93xs-r16d1DiuX_vJjZZ-umCcMxjGEKlAQppCzoq3_Qu7imUNIZJmXNQSmhCnV-okacnPFhiEtCW3bvZm9jcIMv87bhnDVaaSgCOwk2xZyTG8wh-RnTg2FgjkWbU9GmFG2ORZtjlPrk5MKWOtJfUf4r_QKHWqqw</recordid><startdate>20150701</startdate><enddate>20150701</enddate><creator>Cruz, G. J. F.</creator><creator>Matějová, L.</creator><creator>Pirilä, M.</creator><creator>Ainassaari, K.</creator><creator>Canepa, C. A.</creator><creator>Solis, J.</creator><creator>Cruz, J.F.</creator><creator>Šolcová, O.</creator><creator>Keiski, R. 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J. F. ; Matějová, L. ; Pirilä, M. ; Ainassaari, K. ; Canepa, C. A. ; Solis, J. ; Cruz, J.F. ; Šolcová, O. ; Keiski, R. 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J. F.</creatorcontrib><creatorcontrib>Matějová, L.</creatorcontrib><creatorcontrib>Pirilä, M.</creatorcontrib><creatorcontrib>Ainassaari, K.</creatorcontrib><creatorcontrib>Canepa, C. A.</creatorcontrib><creatorcontrib>Solis, J.</creatorcontrib><creatorcontrib>Cruz, J.F.</creatorcontrib><creatorcontrib>Šolcová, O.</creatorcontrib><creatorcontrib>Keiski, R. 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J. F.</au><au>Matějová, L.</au><au>Pirilä, M.</au><au>Ainassaari, K.</au><au>Canepa, C. A.</au><au>Solis, J.</au><au>Cruz, J.F.</au><au>Šolcová, O.</au><au>Keiski, R. L.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>A Comparative Study on Activated Carbons Derived from a Broad Range of Agro-industrial Wastes in Removal of Large-Molecular-Size Organic Pollutants in Aqueous Phase</atitle><jtitle>Water, air, and soil pollution</jtitle><stitle>Water Air Soil Pollut</stitle><date>2015-07-01</date><risdate>2015</risdate><volume>226</volume><issue>7</issue><spage>1</spage><epage>15</epage><pages>1-15</pages><artnum>214</artnum><issn>0049-6979</issn><eissn>1573-2932</eissn><abstract>Microporous–mesoporous activated carbons from five different types of agro-industrial wastes were produced using chemical activation with ZnCl
2
and carbonization at mild conditions of 600 °C, comprehensively characterized and investigated for removal of methylene blue (MB) in aqueous solution, a model large-molecular-size organic pollutant. The external part of the mango pit (mango seed husk) was used for the production of activated carbon (AC) for the first time. Despite that the raw agro-materials exhibited significantly different porosity, all activated carbons produced possessed well-developed microporous–mesoporous structures showing high surface areas and micropore volumes. Further, it was revealed that the pore size distribution of raw agro-material is a more important property in development of microporous–mesoporous structure of produced ACs than their overall porosity. All activated carbons produced adsorbed MB, reaching in most cases 100 % removal from the aqueous phase. Adsorption data were fitted well to a pseudo-second-order kinetic model. For MB adsorption, the mesoporosity and the ratio of micropores accessible for MB were the key factors since there exists the size-selectivity effect on MB adsorption due to MB molecular dimensions. The molecular dimensions of MB were estimated via DFT calculations to 1.66 × 0.82 × 0.54 nm, and this parameter was correlated with determined micropore size distributions of activated carbons.</abstract><cop>Cham</cop><pub>Springer International Publishing</pub><doi>10.1007/s11270-015-2474-7</doi><tpages>15</tpages></addata></record> |
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| ispartof | Water, air, and soil pollution, 2015-07, Vol.226 (7), p.1-15, Article 214 |
| issn | 0049-6979 1573-2932 |
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| subjects | Activated carbon Adsorption Agricultural pollution Agricultural production Agricultural wastes Analysis Atmospheric Protection/Air Quality Control/Air Pollution Biomass Bioremediation Climate Change/Climate Change Impacts Cocoa Coffee Comparative studies Earth and Environmental Science Environment Environmental monitoring Hydrogeology Industrial wastes Mangifera indica Methylene blue Pollutants Pore size Porosity Raw materials Size distribution Soil Science & Conservation Studies Water Quality/Water Pollution |
| title | A Comparative Study on Activated Carbons Derived from a Broad Range of Agro-industrial Wastes in Removal of Large-Molecular-Size Organic Pollutants in Aqueous Phase |
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