Efficient degradation of rhodamine B using modified graphite felt gas diffusion electrode by electro-Fenton process
The electro-Fenton (EF) process treatment of 0.1-M (rhodamine B) RhB solution was studied with different graphite cathode materials, and graphite felt (GF) was selected as a promising material in further investigation. Then, the degradation performances of gas diffusion electrode (GDE) and graphite...
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| creator | Tian, Jiangnan Olajuyin, Ayobami Matthew Mu, Tingzhen Yang, Maohua Xing, Jianmin |
| description | The electro-Fenton (EF) process treatment of 0.1-M (rhodamine B) RhB solution was studied with different graphite cathode materials, and graphite felt (GF) was selected as a promising material in further investigation. Then, the degradation performances of gas diffusion electrode (GDE) and graphite felt (GF) were compared, and GDE was confirmed to be more efficient in RhB removal. The operational parameters such as Fe
2+
dosage and current density were optimized, and comparison among different modified methods—polytetrafluoroethylene-carbon black (PTFE-CB), polytetrafluoroethylene-carbon nanotube (PTFE-CNT), electrodeposition-CB, and electrodeposition-CNT—showed 98.49 % RhB removal by PTFE-CB-modified cathode in 0.05 M Na
2
SO
4
at a current density of 50 A/m
2
and an air flow rate of 1 L/min after 20 min. Meanwhile, after cathode modified by PTFE-CB, the mineralization efficiency and mineralization current efficiency performed absolutely better than the pristine one. Cyclic voltammograms, SEM images, contact angles, and BET surface area were carried out to demonstrate stronger current responses and higher hydrophilicity of GF after modified. The value of biochemical oxygen demand/chemical oxygen demand (BOD
5
/COD) increased from 0.049 to 0.331 after 90-min treatment, suggesting the solution was biodegradable, and the modified cathode was confirmed to be stable after ten circle runs. Finally, a proposed degradation pathway of RhB was put forward. |
| doi_str_mv | 10.1007/s11356-016-6360-7 |
| format | Article |
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2+
dosage and current density were optimized, and comparison among different modified methods—polytetrafluoroethylene-carbon black (PTFE-CB), polytetrafluoroethylene-carbon nanotube (PTFE-CNT), electrodeposition-CB, and electrodeposition-CNT—showed 98.49 % RhB removal by PTFE-CB-modified cathode in 0.05 M Na
2
SO
4
at a current density of 50 A/m
2
and an air flow rate of 1 L/min after 20 min. Meanwhile, after cathode modified by PTFE-CB, the mineralization efficiency and mineralization current efficiency performed absolutely better than the pristine one. Cyclic voltammograms, SEM images, contact angles, and BET surface area were carried out to demonstrate stronger current responses and higher hydrophilicity of GF after modified. The value of biochemical oxygen demand/chemical oxygen demand (BOD
5
/COD) increased from 0.049 to 0.331 after 90-min treatment, suggesting the solution was biodegradable, and the modified cathode was confirmed to be stable after ten circle runs. Finally, a proposed degradation pathway of RhB was put forward.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-016-6360-7</identifier><identifier>PMID: 26931661</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Air flow ; Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; Biochemical oxygen demand ; Biodegradation ; Biological Oxygen Demand Analysis ; Black carbon ; Carbon ; Carbon black ; Chemical oxygen demand ; Coloring Agents - chemistry ; Degradation ; Dyes ; Earth and Environmental Science ; Ecotoxicology ; Efficiency ; Electrochemical Techniques ; Electrodes ; Electrolytes ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Flow rates ; Graphite ; Graphite - chemistry ; Iron - chemistry ; Mineralization ; Nanotubes, Carbon - chemistry ; Oxidation ; Polytetrafluoroethylene ; Polytetrafluoroethylene - chemistry ; Power supply ; Research Article ; Rhodamine ; Rhodamines - chemistry ; Sodium sulfate ; Studies ; Textiles ; Waste Disposal, Fluid - methods ; Waste Water Technology ; Water Management ; Water Pollutants, Chemical - chemistry ; Water Pollution Control</subject><ispartof>Environmental science and pollution research international, 2016-06, Vol.23 (12), p.11574-11583</ispartof><rights>Springer-Verlag Berlin Heidelberg 2016</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c446t-f312fcc450cfbbf4b6ff582cc2c9449dffd701d65843b16ceb2e0323c8a61053</citedby><cites>FETCH-LOGICAL-c446t-f312fcc450cfbbf4b6ff582cc2c9449dffd701d65843b16ceb2e0323c8a61053</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-016-6360-7$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-016-6360-7$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>315,781,785,27929,27930,41493,42562,51324</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/26931661$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Tian, Jiangnan</creatorcontrib><creatorcontrib>Olajuyin, Ayobami Matthew</creatorcontrib><creatorcontrib>Mu, Tingzhen</creatorcontrib><creatorcontrib>Yang, Maohua</creatorcontrib><creatorcontrib>Xing, Jianmin</creatorcontrib><title>Efficient degradation of rhodamine B using modified graphite felt gas diffusion electrode by electro-Fenton process</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>The electro-Fenton (EF) process treatment of 0.1-M (rhodamine B) RhB solution was studied with different graphite cathode materials, and graphite felt (GF) was selected as a promising material in further investigation. Then, the degradation performances of gas diffusion electrode (GDE) and graphite felt (GF) were compared, and GDE was confirmed to be more efficient in RhB removal. The operational parameters such as Fe
2+
dosage and current density were optimized, and comparison among different modified methods—polytetrafluoroethylene-carbon black (PTFE-CB), polytetrafluoroethylene-carbon nanotube (PTFE-CNT), electrodeposition-CB, and electrodeposition-CNT—showed 98.49 % RhB removal by PTFE-CB-modified cathode in 0.05 M Na
2
SO
4
at a current density of 50 A/m
2
and an air flow rate of 1 L/min after 20 min. Meanwhile, after cathode modified by PTFE-CB, the mineralization efficiency and mineralization current efficiency performed absolutely better than the pristine one. Cyclic voltammograms, SEM images, contact angles, and BET surface area were carried out to demonstrate stronger current responses and higher hydrophilicity of GF after modified. The value of biochemical oxygen demand/chemical oxygen demand (BOD
5
/COD) increased from 0.049 to 0.331 after 90-min treatment, suggesting the solution was biodegradable, and the modified cathode was confirmed to be stable after ten circle runs. Finally, a proposed degradation pathway of RhB was put forward.</description><subject>Air flow</subject><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Biochemical oxygen demand</subject><subject>Biodegradation</subject><subject>Biological Oxygen Demand Analysis</subject><subject>Black carbon</subject><subject>Carbon</subject><subject>Carbon black</subject><subject>Chemical oxygen demand</subject><subject>Coloring Agents - chemistry</subject><subject>Degradation</subject><subject>Dyes</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Efficiency</subject><subject>Electrochemical Techniques</subject><subject>Electrodes</subject><subject>Electrolytes</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Flow rates</subject><subject>Graphite</subject><subject>Graphite - chemistry</subject><subject>Iron - chemistry</subject><subject>Mineralization</subject><subject>Nanotubes, Carbon - chemistry</subject><subject>Oxidation</subject><subject>Polytetrafluoroethylene</subject><subject>Polytetrafluoroethylene - chemistry</subject><subject>Power supply</subject><subject>Research Article</subject><subject>Rhodamine</subject><subject>Rhodamines - chemistry</subject><subject>Sodium sulfate</subject><subject>Studies</subject><subject>Textiles</subject><subject>Waste Disposal, Fluid - methods</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water Pollutants, Chemical - chemistry</subject><subject>Water Pollution Control</subject><issn>0944-1344</issn><issn>1614-7499</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2016</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNqNkUFrFTEUhYMo9ln9AW4k4MZN9N4kk5lZamltoeCm-zCT3LymzEyeycyi_960rxURBFeXy_nOuVwOY-8RPiNA-6UgqsYIQCOMMiDaF2yHBrVodd-_ZDvotRaotD5hb0q5A5DQy_Y1O5GmV2gM7lg5DyG6SMvKPe3z4Ic1poWnwPNt8sMcF-Lf-Fbisudz8jFE8rxyh9u4Eg80rXw_FF6FUKHqpIncmpMnPt4_L-Ki5lftkJOjUt6yV2GYCr17mqfs5uL85uxSXP_4fnX29Vo4rc0qgkIZnNMNuDCOQY8mhKaTzklX_-p9CL4F9KbptBrROBolgZLKdYNBaNQp-3SMrWd_blRWO8fiaJqGhdJWLHbQGQOg_wNte9VXuoeKfvwLvUtbXuofj4FaNSh1pfBIuZxKyRTsIcd5yPcWwT50Z4_d2dqdfejOttXz4Sl5G2fyvx3PZVVAHoFSpWVP-Y_T_0z9BaBxpO4</recordid><startdate>20160601</startdate><enddate>20160601</enddate><creator>Tian, Jiangnan</creator><creator>Olajuyin, Ayobami Matthew</creator><creator>Mu, Tingzhen</creator><creator>Yang, Maohua</creator><creator>Xing, Jianmin</creator><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7QL</scope><scope>7SN</scope><scope>7T7</scope><scope>7TV</scope><scope>7U7</scope><scope>7WY</scope><scope>7WZ</scope><scope>7X7</scope><scope>7XB</scope><scope>87Z</scope><scope>88E</scope><scope>88I</scope><scope>8AO</scope><scope>8C1</scope><scope>8FD</scope><scope>8FI</scope><scope>8FJ</scope><scope>8FK</scope><scope>8FL</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>ATCPS</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BEZIV</scope><scope>BHPHI</scope><scope>C1K</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>FR3</scope><scope>FRNLG</scope><scope>FYUFA</scope><scope>F~G</scope><scope>GHDGH</scope><scope>GNUQQ</scope><scope>HCIFZ</scope><scope>K60</scope><scope>K6~</scope><scope>K9.</scope><scope>L.-</scope><scope>M0C</scope><scope>M0S</scope><scope>M1P</scope><scope>M2P</scope><scope>M7N</scope><scope>P64</scope><scope>PATMY</scope><scope>PQBIZ</scope><scope>PQBZA</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PYCSY</scope><scope>Q9U</scope><scope>7X8</scope><scope>7ST</scope><scope>SOI</scope></search><sort><creationdate>20160601</creationdate><title>Efficient degradation of rhodamine B using modified graphite felt gas diffusion electrode by electro-Fenton process</title><author>Tian, Jiangnan ; Olajuyin, Ayobami Matthew ; Mu, Tingzhen ; Yang, Maohua ; Xing, Jianmin</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c446t-f312fcc450cfbbf4b6ff582cc2c9449dffd701d65843b16ceb2e0323c8a61053</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2016</creationdate><topic>Air flow</topic><topic>Aquatic Pollution</topic><topic>Atmospheric Protection/Air Quality Control/Air Pollution</topic><topic>Biochemical oxygen demand</topic><topic>Biodegradation</topic><topic>Biological Oxygen Demand Analysis</topic><topic>Black carbon</topic><topic>Carbon</topic><topic>Carbon black</topic><topic>Chemical oxygen demand</topic><topic>Coloring Agents - 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Academic</collection><collection>Environment Abstracts</collection><collection>Environment Abstracts</collection><jtitle>Environmental science and pollution research international</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Tian, Jiangnan</au><au>Olajuyin, Ayobami Matthew</au><au>Mu, Tingzhen</au><au>Yang, Maohua</au><au>Xing, Jianmin</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Efficient degradation of rhodamine B using modified graphite felt gas diffusion electrode by electro-Fenton process</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2016-06-01</date><risdate>2016</risdate><volume>23</volume><issue>12</issue><spage>11574</spage><epage>11583</epage><pages>11574-11583</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>The electro-Fenton (EF) process treatment of 0.1-M (rhodamine B) RhB solution was studied with different graphite cathode materials, and graphite felt (GF) was selected as a promising material in further investigation. Then, the degradation performances of gas diffusion electrode (GDE) and graphite felt (GF) were compared, and GDE was confirmed to be more efficient in RhB removal. The operational parameters such as Fe
2+
dosage and current density were optimized, and comparison among different modified methods—polytetrafluoroethylene-carbon black (PTFE-CB), polytetrafluoroethylene-carbon nanotube (PTFE-CNT), electrodeposition-CB, and electrodeposition-CNT—showed 98.49 % RhB removal by PTFE-CB-modified cathode in 0.05 M Na
2
SO
4
at a current density of 50 A/m
2
and an air flow rate of 1 L/min after 20 min. Meanwhile, after cathode modified by PTFE-CB, the mineralization efficiency and mineralization current efficiency performed absolutely better than the pristine one. Cyclic voltammograms, SEM images, contact angles, and BET surface area were carried out to demonstrate stronger current responses and higher hydrophilicity of GF after modified. The value of biochemical oxygen demand/chemical oxygen demand (BOD
5
/COD) increased from 0.049 to 0.331 after 90-min treatment, suggesting the solution was biodegradable, and the modified cathode was confirmed to be stable after ten circle runs. Finally, a proposed degradation pathway of RhB was put forward.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>26931661</pmid><doi>10.1007/s11356-016-6360-7</doi><tpages>10</tpages></addata></record> |
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| subjects | Air flow Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Biochemical oxygen demand Biodegradation Biological Oxygen Demand Analysis Black carbon Carbon Carbon black Chemical oxygen demand Coloring Agents - chemistry Degradation Dyes Earth and Environmental Science Ecotoxicology Efficiency Electrochemical Techniques Electrodes Electrolytes Environment Environmental Chemistry Environmental Health Environmental science Flow rates Graphite Graphite - chemistry Iron - chemistry Mineralization Nanotubes, Carbon - chemistry Oxidation Polytetrafluoroethylene Polytetrafluoroethylene - chemistry Power supply Research Article Rhodamine Rhodamines - chemistry Sodium sulfate Studies Textiles Waste Disposal, Fluid - methods Waste Water Technology Water Management Water Pollutants, Chemical - chemistry Water Pollution Control |
| title | Efficient degradation of rhodamine B using modified graphite felt gas diffusion electrode by electro-Fenton process |
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