A novel catalyst for ammonia synthesis at ambient temperature and pressure: Visible light responsive photocatalyst using localized surface plasmon resonance
A novel catalyst for ammonia synthesis using localized surface plasmon resonance (LSPR) was investigated. Os–Au composite nanoparticles showed a high catalytic activity in ammonia synthesis reaction under visible light irradiation at room temperature and atmospheric pressure. Photo energy was likely...
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Veröffentlicht in: | Catalysis communications 2015-01, Vol.59, p.40-44 |
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container_title | Catalysis communications |
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creator | Zeng, Haisheng Terazono, Shinji Tanuma, Toshihiro |
description | A novel catalyst for ammonia synthesis using localized surface plasmon resonance (LSPR) was investigated. Os–Au composite nanoparticles showed a high catalytic activity in ammonia synthesis reaction under visible light irradiation at room temperature and atmospheric pressure. Photo energy was likely to be transferred to Os via Au particles, and contributed to the enhancement of the catalytic activity, because the ammonia production rate and the LSPR absorbance of Au particles showed similar dependence on the irradiation wavelength.
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•A novel photocatalyst for ammonia synthesis at room temperature was investigated.•Os–Au showed a catalytic activity for ammonia synthesis under visible light irradiation.•Localized surface plasmon resonance was suggested to play the role in photocatalytic activity. |
doi_str_mv | 10.1016/j.catcom.2014.09.034 |
format | Article |
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•A novel photocatalyst for ammonia synthesis at room temperature was investigated.•Os–Au showed a catalytic activity for ammonia synthesis under visible light irradiation.•Localized surface plasmon resonance was suggested to play the role in photocatalytic activity.</description><identifier>ISSN: 1566-7367</identifier><identifier>ISSN: 0004-4210</identifier><identifier>EISSN: 1873-3905</identifier><identifier>DOI: 10.1016/j.catcom.2014.09.034</identifier><language>eng</language><publisher>Elsevier B.V</publisher><subject>Ammonia ; Ammonia synthesis ; Catalysts ; Catalytic activity ; Localized surface plasmon resonance ; Particulate composites ; Photocatalyst ; Plasmons ; Surface chemistry ; Synthesis ; Synthesis (chemistry)</subject><ispartof>Catalysis communications, 2015-01, Vol.59, p.40-44</ispartof><rights>2014 Elsevier B.V.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c366t-b4d691d9b8a30414abbe692a852064286849d8562dae39dc5f681f6b908743703</citedby><cites>FETCH-LOGICAL-c366t-b4d691d9b8a30414abbe692a852064286849d8562dae39dc5f681f6b908743703</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://www.sciencedirect.com/science/article/pii/S1566736714003926$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,776,780,3537,27901,27902,65306</link.rule.ids></links><search><creatorcontrib>Zeng, Haisheng</creatorcontrib><creatorcontrib>Terazono, Shinji</creatorcontrib><creatorcontrib>Tanuma, Toshihiro</creatorcontrib><title>A novel catalyst for ammonia synthesis at ambient temperature and pressure: Visible light responsive photocatalyst using localized surface plasmon resonance</title><title>Catalysis communications</title><description>A novel catalyst for ammonia synthesis using localized surface plasmon resonance (LSPR) was investigated. Os–Au composite nanoparticles showed a high catalytic activity in ammonia synthesis reaction under visible light irradiation at room temperature and atmospheric pressure. Photo energy was likely to be transferred to Os via Au particles, and contributed to the enhancement of the catalytic activity, because the ammonia production rate and the LSPR absorbance of Au particles showed similar dependence on the irradiation wavelength.
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•A novel photocatalyst for ammonia synthesis at room temperature was investigated.•Os–Au showed a catalytic activity for ammonia synthesis under visible light irradiation.•Localized surface plasmon resonance was suggested to play the role in photocatalytic activity.</description><subject>Ammonia</subject><subject>Ammonia synthesis</subject><subject>Catalysts</subject><subject>Catalytic activity</subject><subject>Localized surface plasmon resonance</subject><subject>Particulate composites</subject><subject>Photocatalyst</subject><subject>Plasmons</subject><subject>Surface chemistry</subject><subject>Synthesis</subject><subject>Synthesis (chemistry)</subject><issn>1566-7367</issn><issn>0004-4210</issn><issn>1873-3905</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2015</creationdate><recordtype>article</recordtype><recordid>eNp9kc1u3CAUha2qlZomeYMuWHZjFwzG0EWlKOqfFKmbNluE8XWGEQaXy4w0fZY8bBlN1WVXwNH5ztXlNM1bRjtGmXy_75wtLq1dT5noqO4oFy-aK6ZG3nJNh5f1PkjZjlyOr5s3iHtaMc31VfN8R2I6QiA1wYYTFrKkTOy6pugtwVMsO0CPxJYqTh5iIQXWDbIthwzExplsGRDr4wN59OinACT4p10hVd5SRH8Esu1SSf8mHNDHJxKqEPxvmEmFF-uqK1isc89gijY6uGleLTYg3P49r5ufnz_9uP_aPnz_8u3-7qF1XMrSTmKWms16UpZTwYSdJpC6t2roqRS9kkroWQ2yny1wPbthkYotctJUjYKPlF837y65W06_DoDFrB4dhGAjpAMapqhiVA5irFZxsbqcEDMsZst-tflkGDXnMszeXMow5zIM1aaWUbGPFwzqGkcP2aCrn-lg9hlcMXPy_w_4A1NymPg</recordid><startdate>20150110</startdate><enddate>20150110</enddate><creator>Zeng, Haisheng</creator><creator>Terazono, Shinji</creator><creator>Tanuma, Toshihiro</creator><general>Elsevier B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7QQ</scope><scope>7SR</scope><scope>8FD</scope><scope>JG9</scope></search><sort><creationdate>20150110</creationdate><title>A novel catalyst for ammonia synthesis at ambient temperature and pressure: Visible light responsive photocatalyst using localized surface plasmon resonance</title><author>Zeng, Haisheng ; Terazono, Shinji ; Tanuma, Toshihiro</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c366t-b4d691d9b8a30414abbe692a852064286849d8562dae39dc5f681f6b908743703</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2015</creationdate><topic>Ammonia</topic><topic>Ammonia synthesis</topic><topic>Catalysts</topic><topic>Catalytic activity</topic><topic>Localized surface plasmon resonance</topic><topic>Particulate composites</topic><topic>Photocatalyst</topic><topic>Plasmons</topic><topic>Surface chemistry</topic><topic>Synthesis</topic><topic>Synthesis (chemistry)</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zeng, Haisheng</creatorcontrib><creatorcontrib>Terazono, Shinji</creatorcontrib><creatorcontrib>Tanuma, Toshihiro</creatorcontrib><collection>CrossRef</collection><collection>Ceramic Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><jtitle>Catalysis communications</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zeng, Haisheng</au><au>Terazono, Shinji</au><au>Tanuma, Toshihiro</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>A novel catalyst for ammonia synthesis at ambient temperature and pressure: Visible light responsive photocatalyst using localized surface plasmon resonance</atitle><jtitle>Catalysis communications</jtitle><date>2015-01-10</date><risdate>2015</risdate><volume>59</volume><spage>40</spage><epage>44</epage><pages>40-44</pages><issn>1566-7367</issn><issn>0004-4210</issn><eissn>1873-3905</eissn><abstract>A novel catalyst for ammonia synthesis using localized surface plasmon resonance (LSPR) was investigated. Os–Au composite nanoparticles showed a high catalytic activity in ammonia synthesis reaction under visible light irradiation at room temperature and atmospheric pressure. Photo energy was likely to be transferred to Os via Au particles, and contributed to the enhancement of the catalytic activity, because the ammonia production rate and the LSPR absorbance of Au particles showed similar dependence on the irradiation wavelength.
[Display omitted]
•A novel photocatalyst for ammonia synthesis at room temperature was investigated.•Os–Au showed a catalytic activity for ammonia synthesis under visible light irradiation.•Localized surface plasmon resonance was suggested to play the role in photocatalytic activity.</abstract><pub>Elsevier B.V</pub><doi>10.1016/j.catcom.2014.09.034</doi><tpages>5</tpages></addata></record> |
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source | Open Access Titles of Japan; Elsevier ScienceDirect Journals; EZB-FREE-00999 freely available EZB journals |
subjects | Ammonia Ammonia synthesis Catalysts Catalytic activity Localized surface plasmon resonance Particulate composites Photocatalyst Plasmons Surface chemistry Synthesis Synthesis (chemistry) |
title | A novel catalyst for ammonia synthesis at ambient temperature and pressure: Visible light responsive photocatalyst using localized surface plasmon resonance |
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