Zero-Strain Na2FeSiO4 as Novel Cathode Material for Sodium-Ion Batteries

Zero-Strain Na2FeSiO4 as Novel Cathode Material for Sodium-Ion Batteries

A new cubic polymorph of sodium iron silicate, Na2FeSiO4, is reported for the first time as a cathode material for Na-ion batteries. It adopts an unprecedented cubic rigid tetrahedral open framework structure, i.e., F4̅3m, leading to a polyanion cathode material without apparent cell volume change d...

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Veröffentlicht in:ACS applied materials & interfaces 2016-07, Vol.8 (27), p.17233-17238
Hauptverfasser: Li, Shouding, Guo, Jianghuai, Ye, Zhuo, Zhao, Xin, Wu, Shunqing, Mi, Jin-Xiao, Wang, Cai-Zhuang, Gong, Zhengliang, McDonald, Matthew J, Zhu, Zizhong, Ho, Kai-Ming, Yang, Yong
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container_end_page 17238
container_issue 27
container_start_page 17233
container_title ACS applied materials & interfaces
container_volume 8
creator Li, Shouding
Guo, Jianghuai
Ye, Zhuo
Zhao, Xin
Wu, Shunqing
Mi, Jin-Xiao
Wang, Cai-Zhuang
Gong, Zhengliang
McDonald, Matthew J
Zhu, Zizhong
Ho, Kai-Ming
Yang, Yong
description A new cubic polymorph of sodium iron silicate, Na2FeSiO4, is reported for the first time as a cathode material for Na-ion batteries. It adopts an unprecedented cubic rigid tetrahedral open framework structure, i.e., F4̅3m, leading to a polyanion cathode material without apparent cell volume change during the charge/discharge processes. This cathode shows a reversible capacity of 106 mAh g–1 and a capacity retention of 96% at 5 mA g–1 after 20 cycles.
doi_str_mv 10.1021/acsami.6b03969
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title Zero-Strain Na2FeSiO4 as Novel Cathode Material for Sodium-Ion Batteries
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