Site-specific vibrational spectral signatures of water molecules in the magic H₃O⁺(H₂O)₂₀ and Cs⁺(H₂O)₂₀ clusters

Significance Understanding the mechanics underlying the diffuse OH stretching spectrum of water is a grand challenge for contemporary physical chemistry. Water clusters play an increasingly important role in this endeavor, as they allow one to freeze and isolate the spectral behavior of relatively l...

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Veröffentlicht in:	Proceedings of the National Academy of Sciences - PNAS 2014-12, Vol.111 (51), p.18132-18137
Hauptverfasser:	Fournier, Joseph A., Wolke, Conrad T., Johnson, Christopher J., Johnson, Mark A., Heine, Nadja, Gewinner, Sandy, Schöllkopf, Wieland, Esser, Tim K., Fagiani, Matias R., Knorke, Harald, Asmis, Knut R.
Format:	Artikel
Sprache:	eng
Schlagworte:	cages cesium Contrapuntal motion Infrared radiation Ions mass spectrometry mechanics Molecular structure Molecules physical chemistry Physical Sciences Spectral bands Spectral signatures Spectroscopy Surface water Vibrational spectra
Online-Zugang:	Volltext
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