Surface effects on thermoelectric properties of metallic and semiconducting nanowires
Metallic and semiconducting nanowires (NWs) are of interest in the field of thermoelectrics, because they act as model system to investigate the influence of surfaces on the thermoelectric transport properties. In single crystalline NWs, the grain boundary scattering is negligible and the surface‐to...
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Veröffentlicht in: | Physica status solidi. A, Applications and materials science Applications and materials science, 2016-03, Vol.213 (3), p.557-570 |
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creator | Kojda, Danny Mitdank, Rüdiger Weidemann, Stefan Mogilatenko, Anna Wang, Zhi Ruhhammer, Johannes Kroener, Michael Töllner, William Woias, Peter Nielsch, Kornelius Fischer, Saskia F. |
description | Metallic and semiconducting nanowires (NWs) are of interest in the field of thermoelectrics, because they act as model system to investigate the influence of surfaces on the thermoelectric transport properties. In single crystalline NWs, the grain boundary scattering is negligible and the surface‐to‐volume‐ratio is high. We present state‐of‐the‐art of the combination of the structural, chemical, and temperature‐dependent full thermoelectric characterization for individual single crystalline NWs, which is essential to conclude on surface effects. Temperature‐dependent measurements allow further conclusions on the scattering mechanisms. Simulations by the finite element method are performed on indented NWs to interpret the measurement results.
Calculated surface temperature of a single‐indented and a multi‐indented NW.
Combined thermoelectrical, structural and chemical characterisation of individual metallic and semiconducting nanowires is presented. In the temperature range between 4.2 K and room temperature the thermoelectrical properties are determined. Transmission electron microscopy yields the structural properties, the chemical composition and the morphology of the nanowires. This comprehensive study unambiguously allows identifying surface effects on the thermoelectric properties and scattering mechanisms for electrons and phonons. |
doi_str_mv | 10.1002/pssa.201532464 |
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Calculated surface temperature of a single‐indented and a multi‐indented NW.
Combined thermoelectrical, structural and chemical characterisation of individual metallic and semiconducting nanowires is presented. In the temperature range between 4.2 K and room temperature the thermoelectrical properties are determined. Transmission electron microscopy yields the structural properties, the chemical composition and the morphology of the nanowires. This comprehensive study unambiguously allows identifying surface effects on the thermoelectric properties and scattering mechanisms for electrons and phonons.</description><identifier>ISSN: 1862-6300</identifier><identifier>EISSN: 1862-6319</identifier><identifier>DOI: 10.1002/pssa.201532464</identifier><language>eng</language><publisher>Weinheim: Blackwell Publishing Ltd</publisher><subject>Computer simulation ; Crystal structure ; Finite element analysis ; finite element method ; Grain boundaries ; Lorenz number ; Materials science ; Nanowires ; Scattering ; surface effects ; Surface temperature ; Thermoelectricity ; Thermoelectrics</subject><ispartof>Physica status solidi. A, Applications and materials science, 2016-03, Vol.213 (3), p.557-570</ispartof><rights>2015 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim</rights><rights>2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c4584-4a02746cd44e6febcc8553bc0522452ee74f3a43e688d1f7178abbe2d09ab5e13</citedby><cites>FETCH-LOGICAL-c4584-4a02746cd44e6febcc8553bc0522452ee74f3a43e688d1f7178abbe2d09ab5e13</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1002%2Fpssa.201532464$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1002%2Fpssa.201532464$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>314,780,784,1417,27924,27925,45574,45575</link.rule.ids></links><search><creatorcontrib>Kojda, Danny</creatorcontrib><creatorcontrib>Mitdank, Rüdiger</creatorcontrib><creatorcontrib>Weidemann, Stefan</creatorcontrib><creatorcontrib>Mogilatenko, Anna</creatorcontrib><creatorcontrib>Wang, Zhi</creatorcontrib><creatorcontrib>Ruhhammer, Johannes</creatorcontrib><creatorcontrib>Kroener, Michael</creatorcontrib><creatorcontrib>Töllner, William</creatorcontrib><creatorcontrib>Woias, Peter</creatorcontrib><creatorcontrib>Nielsch, Kornelius</creatorcontrib><creatorcontrib>Fischer, Saskia F.</creatorcontrib><title>Surface effects on thermoelectric properties of metallic and semiconducting nanowires</title><title>Physica status solidi. A, Applications and materials science</title><addtitle>Phys. Status Solidi A</addtitle><description>Metallic and semiconducting nanowires (NWs) are of interest in the field of thermoelectrics, because they act as model system to investigate the influence of surfaces on the thermoelectric transport properties. In single crystalline NWs, the grain boundary scattering is negligible and the surface‐to‐volume‐ratio is high. We present state‐of‐the‐art of the combination of the structural, chemical, and temperature‐dependent full thermoelectric characterization for individual single crystalline NWs, which is essential to conclude on surface effects. Temperature‐dependent measurements allow further conclusions on the scattering mechanisms. Simulations by the finite element method are performed on indented NWs to interpret the measurement results.
Calculated surface temperature of a single‐indented and a multi‐indented NW.
Combined thermoelectrical, structural and chemical characterisation of individual metallic and semiconducting nanowires is presented. In the temperature range between 4.2 K and room temperature the thermoelectrical properties are determined. Transmission electron microscopy yields the structural properties, the chemical composition and the morphology of the nanowires. This comprehensive study unambiguously allows identifying surface effects on the thermoelectric properties and scattering mechanisms for electrons and phonons.</description><subject>Computer simulation</subject><subject>Crystal structure</subject><subject>Finite element analysis</subject><subject>finite element method</subject><subject>Grain boundaries</subject><subject>Lorenz number</subject><subject>Materials science</subject><subject>Nanowires</subject><subject>Scattering</subject><subject>surface effects</subject><subject>Surface temperature</subject><subject>Thermoelectricity</subject><subject>Thermoelectrics</subject><issn>1862-6300</issn><issn>1862-6319</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2016</creationdate><recordtype>article</recordtype><recordid>eNqFkElPwzAQhS0EElC4co7EhUuK7Yxj94jYJTa1II6W44zBkKXYiaD_nlRFFeLCabb3jWYeIQeMjhml_HgeoxlzykTGIYcNssNUztM8Y5PNdU7pNtmN8Y1SECDZDnma9cEZiwk6h7aLSdsk3SuGusVqqIO3yTy0cwydx2Hokho7U1VD2zRlErH2tm3K3na-eUka07SfPmDcI1vOVBH3f-KIPF2cP55epTf3l9enJzepBaEgBUO5hNyWAJg7LKxVQmSFpYJzEBxRgssMZJgrVTInmVSmKJCXdGIKgSwbkaPV3uHGjx5jp2sfLVaVabDto2ZqeFQBl0vp4R_pW9uHZrhOMym5ogCDcyMyXqlsaGMM6PQ8-NqEhWZUL13WS5f12uUBmKyAT1_h4h-1fpjNTn6z6Yr1scOvNWvCu85lJoV-vrvUU3YLZ9OzK62yb8rvkS0</recordid><startdate>201603</startdate><enddate>201603</enddate><creator>Kojda, Danny</creator><creator>Mitdank, Rüdiger</creator><creator>Weidemann, Stefan</creator><creator>Mogilatenko, Anna</creator><creator>Wang, Zhi</creator><creator>Ruhhammer, Johannes</creator><creator>Kroener, Michael</creator><creator>Töllner, William</creator><creator>Woias, Peter</creator><creator>Nielsch, Kornelius</creator><creator>Fischer, Saskia F.</creator><general>Blackwell Publishing Ltd</general><general>Wiley Subscription Services, Inc</general><scope>BSCLL</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SP</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope></search><sort><creationdate>201603</creationdate><title>Surface effects on thermoelectric properties of metallic and semiconducting nanowires</title><author>Kojda, Danny ; Mitdank, Rüdiger ; Weidemann, Stefan ; Mogilatenko, Anna ; Wang, Zhi ; Ruhhammer, Johannes ; Kroener, Michael ; Töllner, William ; Woias, Peter ; Nielsch, Kornelius ; Fischer, Saskia F.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c4584-4a02746cd44e6febcc8553bc0522452ee74f3a43e688d1f7178abbe2d09ab5e13</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2016</creationdate><topic>Computer simulation</topic><topic>Crystal structure</topic><topic>Finite element analysis</topic><topic>finite element method</topic><topic>Grain boundaries</topic><topic>Lorenz number</topic><topic>Materials science</topic><topic>Nanowires</topic><topic>Scattering</topic><topic>surface effects</topic><topic>Surface temperature</topic><topic>Thermoelectricity</topic><topic>Thermoelectrics</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Kojda, Danny</creatorcontrib><creatorcontrib>Mitdank, Rüdiger</creatorcontrib><creatorcontrib>Weidemann, Stefan</creatorcontrib><creatorcontrib>Mogilatenko, Anna</creatorcontrib><creatorcontrib>Wang, Zhi</creatorcontrib><creatorcontrib>Ruhhammer, Johannes</creatorcontrib><creatorcontrib>Kroener, Michael</creatorcontrib><creatorcontrib>Töllner, William</creatorcontrib><creatorcontrib>Woias, Peter</creatorcontrib><creatorcontrib>Nielsch, Kornelius</creatorcontrib><creatorcontrib>Fischer, Saskia F.</creatorcontrib><collection>Istex</collection><collection>CrossRef</collection><collection>Electronics & Communications Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Physica status solidi. A, Applications and materials science</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Kojda, Danny</au><au>Mitdank, Rüdiger</au><au>Weidemann, Stefan</au><au>Mogilatenko, Anna</au><au>Wang, Zhi</au><au>Ruhhammer, Johannes</au><au>Kroener, Michael</au><au>Töllner, William</au><au>Woias, Peter</au><au>Nielsch, Kornelius</au><au>Fischer, Saskia F.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Surface effects on thermoelectric properties of metallic and semiconducting nanowires</atitle><jtitle>Physica status solidi. A, Applications and materials science</jtitle><addtitle>Phys. Status Solidi A</addtitle><date>2016-03</date><risdate>2016</risdate><volume>213</volume><issue>3</issue><spage>557</spage><epage>570</epage><pages>557-570</pages><issn>1862-6300</issn><eissn>1862-6319</eissn><abstract>Metallic and semiconducting nanowires (NWs) are of interest in the field of thermoelectrics, because they act as model system to investigate the influence of surfaces on the thermoelectric transport properties. In single crystalline NWs, the grain boundary scattering is negligible and the surface‐to‐volume‐ratio is high. We present state‐of‐the‐art of the combination of the structural, chemical, and temperature‐dependent full thermoelectric characterization for individual single crystalline NWs, which is essential to conclude on surface effects. Temperature‐dependent measurements allow further conclusions on the scattering mechanisms. Simulations by the finite element method are performed on indented NWs to interpret the measurement results.
Calculated surface temperature of a single‐indented and a multi‐indented NW.
Combined thermoelectrical, structural and chemical characterisation of individual metallic and semiconducting nanowires is presented. In the temperature range between 4.2 K and room temperature the thermoelectrical properties are determined. Transmission electron microscopy yields the structural properties, the chemical composition and the morphology of the nanowires. This comprehensive study unambiguously allows identifying surface effects on the thermoelectric properties and scattering mechanisms for electrons and phonons.</abstract><cop>Weinheim</cop><pub>Blackwell Publishing Ltd</pub><doi>10.1002/pssa.201532464</doi><tpages>14</tpages></addata></record> |
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subjects | Computer simulation Crystal structure Finite element analysis finite element method Grain boundaries Lorenz number Materials science Nanowires Scattering surface effects Surface temperature Thermoelectricity Thermoelectrics |
title | Surface effects on thermoelectric properties of metallic and semiconducting nanowires |
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