Development of mean-field electrical double layer theory
In order to understand the electric interfacial behavior, mean field based electric double layer （EDL） theory has been continuously developed over the past 150 years. In this article, we briefly review the development of the EDL model, from the dimensionless Gouy-Chapman model to the symmetric Biker...
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| Veröffentlicht in: | Chinese physics B 2016-01, Vol.25 (1), p.282-288 |
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| creator | 黄一珂 刘晓红 李姝 言天英 |
| description | In order to understand the electric interfacial behavior, mean field based electric double layer （EDL） theory has been continuously developed over the past 150 years. In this article, we briefly review the development of the EDL model, from the dimensionless Gouy-Chapman model to the symmetric Bikerman-Freise model, and finally toward size-asymmetric mean field theory models. We provide the general derivations within the framework of Helmholtz free energy of the lattice- gas model, and it can be seen that the above-mentioned models are consistent in the sense that the interconversi0n among them can be achieved by reducing the basic assumptions. |
| doi_str_mv | 10.1088/1674-1056/25/1/016801 |
| format | Article |
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| ispartof | Chinese physics B, 2016-01, Vol.25 (1), p.282-288 |
| issn | 1674-1056 2058-3834 1741-4199 |
| language | eng |
| recordid | cdi_proquest_miscellaneous_1800473537 |
| source | IOP Publishing Journals |
| subjects | Derivation Double layer Double layer (electric) EDI Electric double layer Field theory Free energy Symmetry 亥姆霍兹自由能 双电层理论 平均场理论 格子气模型 电场 界面行为 非对称 |
| title | Development of mean-field electrical double layer theory |
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