k=0 magnetic structure and absence of ferroelectricity in SmFeO3

SmFeO3 has attracted considerable attention very recently due to its reported multiferroic properties above room temperature. We have performed powder and single crystal neutron diffraction as well as complementary polarization dependent soft X-ray absorption spectroscopy measurements on floating-zo...

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Veröffentlicht in:Physical review letters 2014-11, Vol.113 (21), p.217203-217203
Hauptverfasser: Kuo, C-Y, Drees, Y, Fernández-Díaz, M T, Zhao, L, Vasylechko, L, Sheptyakov, D, Bell, A M T, Pi, T W, Lin, H-J, Wu, M-K, Pellegrin, E, Valvidares, S M, Li, Z W, Adler, P, Todorova, A, Küchler, R, Steppke, A, Tjeng, L H, Hu, Z, Komarek, A C
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container_end_page 217203
container_issue 21
container_start_page 217203
container_title Physical review letters
container_volume 113
creator Kuo, C-Y
Drees, Y
Fernández-Díaz, M T
Zhao, L
Vasylechko, L
Sheptyakov, D
Bell, A M T
Pi, T W
Lin, H-J
Wu, M-K
Pellegrin, E
Valvidares, S M
Li, Z W
Adler, P
Todorova, A
Küchler, R
Steppke, A
Tjeng, L H
Hu, Z
Komarek, A C
description SmFeO3 has attracted considerable attention very recently due to its reported multiferroic properties above room temperature. We have performed powder and single crystal neutron diffraction as well as complementary polarization dependent soft X-ray absorption spectroscopy measurements on floating-zone grown SmFeO3 single crystals in order to determine its magnetic structure. We found a k=0 G-type collinear antiferromagnetic structure that is not compatible with inverse Dzyaloshinskii-Moriya interaction driven ferroelectricity. While the structural data reveal a clear sign for magneto-elastic coupling at the Néel-temperature of ∼675  K, the dielectric measurements remain silent as far as ferroelectricity is concerned.
doi_str_mv 10.1103/PhysRevLett.113.217203
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1079-7114
language eng
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source American Physical Society Journals
subjects Absorption spectroscopy
Compatibility
Dielectrics
Ferroelectricity
Inverse
Magnetic structure
Neutron diffraction
Single crystals
title k=0 magnetic structure and absence of ferroelectricity in SmFeO3
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