Iodine-129 Time Series in Danish, Norwegian and Northwest Greenland Coast and the Baltic Sea by Seaweed

The concentrations of129I and127I were determined in archived time series seaweed samples from Klint in the Kattegat, Bornholm in the Baltic Sea, Roskilde Fjord in Zealand of Denmark, Utsira in the western Norwegian coast and NW Greenland by neutron activation analysis. The results indicate that the...

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Veröffentlicht in:Estuarine, coastal and shelf science coastal and shelf science, 2000-11, Vol.51 (5), p.571-584
Hauptverfasser: Hou, X.L., Dahlgaard, H., Nielsen, S.P.
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container_title Estuarine, coastal and shelf science
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creator Hou, X.L.
Dahlgaard, H.
Nielsen, S.P.
description The concentrations of129I and127I were determined in archived time series seaweed samples from Klint in the Kattegat, Bornholm in the Baltic Sea, Roskilde Fjord in Zealand of Denmark, Utsira in the western Norwegian coast and NW Greenland by neutron activation analysis. The results indicate that the129I levels in all locations investigated are one to three orders of magnitude higher than the fall-out background and strongly dominated by the discharges from reprocessing facilities at La Hague and Sellafield. The129I/99Tc ratio is applied to estimate the origin of and transit times of129I. Transit times of129I are estimated to be 1–2 years from La Hague to Klint and Utsira and 9–14 years to NW Greenland. Transfer factors of129I are calculated to be 54yrm−3from La Hague to Klint, 60yrm−3to Utsira and 1·2yrm−3to NW Greenland. Based on the estimated transit times, transfer factors and annual discharge data of radionulides from the reprocessing facilities, the variations of129I concentrations and129I/99Tc and129I/137Cs ratios are modelled. Except129I/137Cs, others are in a good agreement between the modelled and measured values.
doi_str_mv 10.1006/ecss.2000.0698
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The results indicate that the129I levels in all locations investigated are one to three orders of magnitude higher than the fall-out background and strongly dominated by the discharges from reprocessing facilities at La Hague and Sellafield. The129I/99Tc ratio is applied to estimate the origin of and transit times of129I. Transit times of129I are estimated to be 1–2 years from La Hague to Klint and Utsira and 9–14 years to NW Greenland. Transfer factors of129I are calculated to be 54yrm−3from La Hague to Klint, 60yrm−3to Utsira and 1·2yrm−3to NW Greenland. Based on the estimated transit times, transfer factors and annual discharge data of radionulides from the reprocessing facilities, the variations of129I concentrations and129I/99Tc and129I/137Cs ratios are modelled. 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The results indicate that the129I levels in all locations investigated are one to three orders of magnitude higher than the fall-out background and strongly dominated by the discharges from reprocessing facilities at La Hague and Sellafield. The129I/99Tc ratio is applied to estimate the origin of and transit times of129I. Transit times of129I are estimated to be 1–2 years from La Hague to Klint and Utsira and 9–14 years to NW Greenland. Transfer factors of129I are calculated to be 54yrm−3from La Hague to Klint, 60yrm−3to Utsira and 1·2yrm−3to NW Greenland. Based on the estimated transit times, transfer factors and annual discharge data of radionulides from the reprocessing facilities, the variations of129I concentrations and129I/99Tc and129I/137Cs ratios are modelled. 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source ScienceDirect Journals (5 years ago - present)
subjects Animal, plant and microbial ecology
Applied ecology
Baltic Sea
Biological and medical sciences
Denmark coast
Ecotoxicology, biological effects of pollution
Fundamental and applied biological sciences. Psychology
Greenland coast
iodine-129
Marine
Marine and brackish environment
radioactive tracers
seaweed
time series
transport
title Iodine-129 Time Series in Danish, Norwegian and Northwest Greenland Coast and the Baltic Sea by Seaweed
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