Carbonyl emissions from heavy-duty diesel vehicle exhaust in China and the contribution to ozone formation potential
Fifteen heavy-duty diesel vehicles were tested on chassis dynamometer by using typical heavy duty driving cycle and fuel economy cycle. The air from the exhaust was sampled by 2,4- dinitrophenyhydrazine cartridge and 23 carbonyl compounds were analyzed by high performance liquid chromatography. The...
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| Veröffentlicht in: | Journal of environmental sciences (China) 2014, Vol.26 (1), p.122-128 |
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| creator | Dong, Dong Shao, Min Li, Yue Lu, Sihua Wang, Yanjun Ji, Zhe Tang, Dagang |
| description | Fifteen heavy-duty diesel vehicles were tested on chassis dynamometer by using typical heavy duty driving cycle and fuel economy cycle. The air from the exhaust was sampled by 2,4- dinitrophenyhydrazine cartridge and 23 carbonyl compounds were analyzed by high performance liquid chromatography. The average emission factor of carbonyls was 97.2 mg/km, higher than that of light-duty diesel vehicles and gasoline-powered vehicles. Formaldehyde, acetaldehyde, acetone and propionaidehyde were the species with the highest emission factors. Main influencing factors for carbonyl emissions were vehicle type, average speed and regulated emission standard, and the impact of vehicle loading was not evident in this study. National emission of carbonyls from diesel vehicles exhaust was calculated for China, 2011, based on both vehicle miles traveled and fuel consumption. Carbonyl emission of diesel vehicle was estimated to be 45.8 Gg, and was comparable to gasolinepowered vehicles （58.4 Gg）. The emissions of formaldehyde, acetaldehyde and acetone were 12.6, 6.9, 3.8 Gg, respectively. The ozone formation potential of carbonyls from diesel vehicles exhaust was 537 mg O3/km, higher than 497 mg O3/km of none-methane hydrocarbons emitted from diesel vehicles. |
| doi_str_mv | 10.1016/S1001-0742(13)60387-3 |
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The air from the exhaust was sampled by 2,4- dinitrophenyhydrazine cartridge and 23 carbonyl compounds were analyzed by high performance liquid chromatography. The average emission factor of carbonyls was 97.2 mg/km, higher than that of light-duty diesel vehicles and gasoline-powered vehicles. Formaldehyde, acetaldehyde, acetone and propionaidehyde were the species with the highest emission factors. Main influencing factors for carbonyl emissions were vehicle type, average speed and regulated emission standard, and the impact of vehicle loading was not evident in this study. National emission of carbonyls from diesel vehicles exhaust was calculated for China, 2011, based on both vehicle miles traveled and fuel consumption. Carbonyl emission of diesel vehicle was estimated to be 45.8 Gg, and was comparable to gasolinepowered vehicles （58.4 Gg）. The emissions of formaldehyde, acetaldehyde and acetone were 12.6, 6.9, 3.8 Gg, respectively. The ozone formation potential of carbonyls from diesel vehicles exhaust was 537 mg O3/km, higher than 497 mg O3/km of none-methane hydrocarbons emitted from diesel vehicles.</description><identifier>ISSN: 1001-0742</identifier><identifier>EISSN: 1878-7320</identifier><identifier>DOI: 10.1016/S1001-0742(13)60387-3</identifier><identifier>PMID: 24649697</identifier><language>eng</language><publisher>Netherlands: Elsevier B.V</publisher><subject>Air Pollutants - analysis ; Air Pollutants - chemical synthesis ; Air Pollutants - standards ; Aldehydes - analysis ; carbonyl ; Carbonyls ; chassis dynamometer ; China ; Diesel ; Diesel fuels ; diesel vehicle ; Emission ; Emission analysis ; Exhaust ; Ketones - analysis ; Ozone - chemical synthesis ; ozone formation potential ; Vehicle Emissions - analysis ; Vehicles ; 中国 ; 平均排放因子 ; 柴油车辆 ; 汽车尾气 ; 羰基化合物 ; 臭氧 ; 重型 ; 高效液相色谱法</subject><ispartof>Journal of environmental sciences (China), 2014, Vol.26 (1), p.122-128</ispartof><rights>2014 The Research Centre for Eco-Environmental Sciences, Chinese Academy of Sciences</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c457t-323b9bf81413eacb42cfc091b0ffde3eb765709f09558d06398797500eba8e3d3</citedby><cites>FETCH-LOGICAL-c457t-323b9bf81413eacb42cfc091b0ffde3eb765709f09558d06398797500eba8e3d3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Uhttp://image.cqvip.com/vip1000/qk/85265X/85265X.jpg</thumbnail><linktohtml>$$Uhttps://www.sciencedirect.com/science/article/pii/S1001074213603873$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,776,780,3537,4010,27900,27901,27902,65306</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/24649697$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Dong, Dong</creatorcontrib><creatorcontrib>Shao, Min</creatorcontrib><creatorcontrib>Li, Yue</creatorcontrib><creatorcontrib>Lu, Sihua</creatorcontrib><creatorcontrib>Wang, Yanjun</creatorcontrib><creatorcontrib>Ji, Zhe</creatorcontrib><creatorcontrib>Tang, Dagang</creatorcontrib><title>Carbonyl emissions from heavy-duty diesel vehicle exhaust in China and the contribution to ozone formation potential</title><title>Journal of environmental sciences (China)</title><addtitle>Journal of Environmental Sciences</addtitle><description>Fifteen heavy-duty diesel vehicles were tested on chassis dynamometer by using typical heavy duty driving cycle and fuel economy cycle. The air from the exhaust was sampled by 2,4- dinitrophenyhydrazine cartridge and 23 carbonyl compounds were analyzed by high performance liquid chromatography. The average emission factor of carbonyls was 97.2 mg/km, higher than that of light-duty diesel vehicles and gasoline-powered vehicles. Formaldehyde, acetaldehyde, acetone and propionaidehyde were the species with the highest emission factors. Main influencing factors for carbonyl emissions were vehicle type, average speed and regulated emission standard, and the impact of vehicle loading was not evident in this study. National emission of carbonyls from diesel vehicles exhaust was calculated for China, 2011, based on both vehicle miles traveled and fuel consumption. Carbonyl emission of diesel vehicle was estimated to be 45.8 Gg, and was comparable to gasolinepowered vehicles （58.4 Gg）. The emissions of formaldehyde, acetaldehyde and acetone were 12.6, 6.9, 3.8 Gg, respectively. The ozone formation potential of carbonyls from diesel vehicles exhaust was 537 mg O3/km, higher than 497 mg O3/km of none-methane hydrocarbons emitted from diesel vehicles.</description><subject>Air Pollutants - analysis</subject><subject>Air Pollutants - chemical synthesis</subject><subject>Air Pollutants - standards</subject><subject>Aldehydes - analysis</subject><subject>carbonyl</subject><subject>Carbonyls</subject><subject>chassis dynamometer</subject><subject>China</subject><subject>Diesel</subject><subject>Diesel fuels</subject><subject>diesel vehicle</subject><subject>Emission</subject><subject>Emission analysis</subject><subject>Exhaust</subject><subject>Ketones - analysis</subject><subject>Ozone - chemical synthesis</subject><subject>ozone formation potential</subject><subject>Vehicle Emissions - analysis</subject><subject>Vehicles</subject><subject>中国</subject><subject>平均排放因子</subject><subject>柴油车辆</subject><subject>汽车尾气</subject><subject>羰基化合物</subject><subject>臭氧</subject><subject>重型</subject><subject>高效液相色谱法</subject><issn>1001-0742</issn><issn>1878-7320</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2014</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqNkU1v1DAQhiMEoqXwE0DmVg6BcfwVn1C14kuqxAE4W44zaYwSe2s7K5ZfT7q77bWcPLKemdeep6peU3hPgcoPPygArUHx5pKydxJYq2r2pDqnrWprxRp4utb3yFn1IuffAMAFiOfVWcMl11Kr86psbOpi2E8EZ5-zjyGTIcWZjGh3-7pfyp70HjNOZIejdxMS_DPaJRfiA9mMPlhiQ0_KiMTFUJLvlrJOISWS-DcGJENMsz1cbWPBULydXlbPBjtlfHU6L6pfnz_93Hytr79_-ba5uq4dF6rUrGGd7oaWcsrQuo43bnCgaQfD0CPDTkmhQA-ghWh7kEy3SisBgJ1tkfXsoro8zt2meLtgLmb9o8NpsgHjkg1VChhIofXjqKBScU3p_6CgOW2opisqjqhLMeeEg9kmP9u0NxTMnUZz0GjuHBnKzEGjYWvfm1PE0s3YP3Tde1uBj0cA1_XtPCaTncfgsPcJXTF99I9GvD09bYzh5taHm4cU3sqmUQ1j_wCpIrh-</recordid><startdate>2014</startdate><enddate>2014</enddate><creator>Dong, Dong</creator><creator>Shao, Min</creator><creator>Li, Yue</creator><creator>Lu, Sihua</creator><creator>Wang, Yanjun</creator><creator>Ji, Zhe</creator><creator>Tang, Dagang</creator><general>Elsevier B.V</general><scope>2RA</scope><scope>92L</scope><scope>CQIGP</scope><scope>W92</scope><scope>~WA</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>7ST</scope><scope>7TG</scope><scope>7TV</scope><scope>C1K</scope><scope>KL.</scope><scope>SOI</scope><scope>7SU</scope><scope>7TB</scope><scope>8FD</scope><scope>FR3</scope><scope>KR7</scope></search><sort><creationdate>2014</creationdate><title>Carbonyl emissions from heavy-duty diesel vehicle exhaust in China and the contribution to ozone formation potential</title><author>Dong, Dong ; 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The air from the exhaust was sampled by 2,4- dinitrophenyhydrazine cartridge and 23 carbonyl compounds were analyzed by high performance liquid chromatography. The average emission factor of carbonyls was 97.2 mg/km, higher than that of light-duty diesel vehicles and gasoline-powered vehicles. Formaldehyde, acetaldehyde, acetone and propionaidehyde were the species with the highest emission factors. Main influencing factors for carbonyl emissions were vehicle type, average speed and regulated emission standard, and the impact of vehicle loading was not evident in this study. National emission of carbonyls from diesel vehicles exhaust was calculated for China, 2011, based on both vehicle miles traveled and fuel consumption. Carbonyl emission of diesel vehicle was estimated to be 45.8 Gg, and was comparable to gasolinepowered vehicles （58.4 Gg）. The emissions of formaldehyde, acetaldehyde and acetone were 12.6, 6.9, 3.8 Gg, respectively. The ozone formation potential of carbonyls from diesel vehicles exhaust was 537 mg O3/km, higher than 497 mg O3/km of none-methane hydrocarbons emitted from diesel vehicles.</abstract><cop>Netherlands</cop><pub>Elsevier B.V</pub><pmid>24649697</pmid><doi>10.1016/S1001-0742(13)60387-3</doi><tpages>7</tpages></addata></record> |
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| ispartof | Journal of environmental sciences (China), 2014, Vol.26 (1), p.122-128 |
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| language | eng |
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| source | MEDLINE; Elsevier ScienceDirect Journals; Alma/SFX Local Collection |
| subjects | Air Pollutants - analysis Air Pollutants - chemical synthesis Air Pollutants - standards Aldehydes - analysis carbonyl Carbonyls chassis dynamometer China Diesel Diesel fuels diesel vehicle Emission Emission analysis Exhaust Ketones - analysis Ozone - chemical synthesis ozone formation potential Vehicle Emissions - analysis Vehicles 中国 平均排放因子 柴油车辆 汽车尾气 羰基化合物 臭氧 重型 高效液相色谱法 |
| title | Carbonyl emissions from heavy-duty diesel vehicle exhaust in China and the contribution to ozone formation potential |
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