Programmable Sub-nanometer Sculpting of Graphene with Electron Beams
Electron beams in transmission electron microscopes are very attractive to engineer and pattern graphene toward all-carbon device fabrication. The use of condensed beams typically used for sequential raster imaging is particularly exciting since they potentially provide high degrees of precision. Ho...
Gespeichert in:
Veröffentlicht in: | ACS nano 2012-11, Vol.6 (11), p.10327-10334 |
---|---|
Hauptverfasser: | , , , , , |
Format: | Artikel |
Sprache: | eng |
Schlagworte: | |
Online-Zugang: | Volltext |
Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
container_end_page | 10334 |
---|---|
container_issue | 11 |
container_start_page | 10327 |
container_title | ACS nano |
container_volume | 6 |
creator | Börrnert, Felix Fu, Lei Gorantla, Sandeep Knupfer, Martin Büchner, Bernd Rümmeli, Mark H |
description | Electron beams in transmission electron microscopes are very attractive to engineer and pattern graphene toward all-carbon device fabrication. The use of condensed beams typically used for sequential raster imaging is particularly exciting since they potentially provide high degrees of precision. However, technical difficulties, such as the formation of electron beam induced deposits on sample surfaces, have hindered the development of this technique. We demonstrate how one can successfully use a condensed electron beam, either with or without C s correction, to structure graphene with sub-nanometer precision in a programmable manner. We further demonstrate the potential of the developed technique by combining it with an established route to engineer graphene nanoribbons to single-atom carbon chains. |
doi_str_mv | 10.1021/nn304256a |
format | Article |
fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_1762051545</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>1762051545</sourcerecordid><originalsourceid>FETCH-LOGICAL-a348t-efa932d063212768f1e2ae26e36ab491e5aca8a388520479809483b30f2b29c53</originalsourceid><addsrcrecordid>eNqN0EtLw0AUhuFBFFsvC_-AZCPoIjqXzCVLrbUKBYUquAsn6UmbkszUmQTx3xtp7cqFq3MWD9_iJeSM0WtGObuxVtCESwV7ZMhSoWJq1Pv-7pdsQI5CWFEqtdHqkAy4YIxqzobk_sW7hYemgbzGaNblsQXrGmzRR7Oiq9dtZReRK6OJh_USLUafVbuMxjUWrXc2ukNowgk5KKEOeLq9x-TtYfw6eoynz5On0e00BpGYNsYSUsHnVAnOuFamZMgBuUKhIE9ShhIKMCCMkZwmOjU0TYzIBS15ztNCimNyudlde_fRYWizpgoF1jVYdF3ImFacSiaTf1DeS8214D292tDCuxA8ltnaVw34r4zR7Kdvtuvb2_PtbJc3ON_J36A9uNgAKEK2cp23fZA_hr4BhZh_WA</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>1220572732</pqid></control><display><type>article</type><title>Programmable Sub-nanometer Sculpting of Graphene with Electron Beams</title><source>ACS Publications</source><source>MEDLINE</source><creator>Börrnert, Felix ; Fu, Lei ; Gorantla, Sandeep ; Knupfer, Martin ; Büchner, Bernd ; Rümmeli, Mark H</creator><creatorcontrib>Börrnert, Felix ; Fu, Lei ; Gorantla, Sandeep ; Knupfer, Martin ; Büchner, Bernd ; Rümmeli, Mark H</creatorcontrib><description>Electron beams in transmission electron microscopes are very attractive to engineer and pattern graphene toward all-carbon device fabrication. The use of condensed beams typically used for sequential raster imaging is particularly exciting since they potentially provide high degrees of precision. However, technical difficulties, such as the formation of electron beam induced deposits on sample surfaces, have hindered the development of this technique. We demonstrate how one can successfully use a condensed electron beam, either with or without C s correction, to structure graphene with sub-nanometer precision in a programmable manner. We further demonstrate the potential of the developed technique by combining it with an established route to engineer graphene nanoribbons to single-atom carbon chains.</description><identifier>ISSN: 1936-0851</identifier><identifier>EISSN: 1936-086X</identifier><identifier>DOI: 10.1021/nn304256a</identifier><identifier>PMID: 23110721</identifier><language>eng</language><publisher>United States: American Chemical Society</publisher><subject>Beams (radiation) ; Carbon ; Condensing ; Crystallization - methods ; Deposition ; Devices ; Electron beams ; Electron microscopes ; Electrons ; Graphene ; Graphite - chemistry ; Graphite - radiation effects ; Macromolecular Substances - chemistry ; Macromolecular Substances - radiation effects ; Materials Testing ; Molecular Conformation - radiation effects ; Molecular Imprinting - methods ; Nanostructure ; Nanostructures - chemistry ; Nanostructures - radiation effects ; Nanostructures - ultrastructure ; Particle Size ; Surface Properties - radiation effects</subject><ispartof>ACS nano, 2012-11, Vol.6 (11), p.10327-10334</ispartof><rights>Copyright © 2012 American Chemical Society</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a348t-efa932d063212768f1e2ae26e36ab491e5aca8a388520479809483b30f2b29c53</citedby><cites>FETCH-LOGICAL-a348t-efa932d063212768f1e2ae26e36ab491e5aca8a388520479809483b30f2b29c53</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/nn304256a$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/nn304256a$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>314,776,780,2752,27053,27901,27902,56713,56763</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/23110721$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Börrnert, Felix</creatorcontrib><creatorcontrib>Fu, Lei</creatorcontrib><creatorcontrib>Gorantla, Sandeep</creatorcontrib><creatorcontrib>Knupfer, Martin</creatorcontrib><creatorcontrib>Büchner, Bernd</creatorcontrib><creatorcontrib>Rümmeli, Mark H</creatorcontrib><title>Programmable Sub-nanometer Sculpting of Graphene with Electron Beams</title><title>ACS nano</title><addtitle>ACS Nano</addtitle><description>Electron beams in transmission electron microscopes are very attractive to engineer and pattern graphene toward all-carbon device fabrication. The use of condensed beams typically used for sequential raster imaging is particularly exciting since they potentially provide high degrees of precision. However, technical difficulties, such as the formation of electron beam induced deposits on sample surfaces, have hindered the development of this technique. We demonstrate how one can successfully use a condensed electron beam, either with or without C s correction, to structure graphene with sub-nanometer precision in a programmable manner. We further demonstrate the potential of the developed technique by combining it with an established route to engineer graphene nanoribbons to single-atom carbon chains.</description><subject>Beams (radiation)</subject><subject>Carbon</subject><subject>Condensing</subject><subject>Crystallization - methods</subject><subject>Deposition</subject><subject>Devices</subject><subject>Electron beams</subject><subject>Electron microscopes</subject><subject>Electrons</subject><subject>Graphene</subject><subject>Graphite - chemistry</subject><subject>Graphite - radiation effects</subject><subject>Macromolecular Substances - chemistry</subject><subject>Macromolecular Substances - radiation effects</subject><subject>Materials Testing</subject><subject>Molecular Conformation - radiation effects</subject><subject>Molecular Imprinting - methods</subject><subject>Nanostructure</subject><subject>Nanostructures - chemistry</subject><subject>Nanostructures - radiation effects</subject><subject>Nanostructures - ultrastructure</subject><subject>Particle Size</subject><subject>Surface Properties - radiation effects</subject><issn>1936-0851</issn><issn>1936-086X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2012</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqN0EtLw0AUhuFBFFsvC_-AZCPoIjqXzCVLrbUKBYUquAsn6UmbkszUmQTx3xtp7cqFq3MWD9_iJeSM0WtGObuxVtCESwV7ZMhSoWJq1Pv-7pdsQI5CWFEqtdHqkAy4YIxqzobk_sW7hYemgbzGaNblsQXrGmzRR7Oiq9dtZReRK6OJh_USLUafVbuMxjUWrXc2ukNowgk5KKEOeLq9x-TtYfw6eoynz5On0e00BpGYNsYSUsHnVAnOuFamZMgBuUKhIE9ShhIKMCCMkZwmOjU0TYzIBS15ztNCimNyudlde_fRYWizpgoF1jVYdF3ImFacSiaTf1DeS8214D292tDCuxA8ltnaVw34r4zR7Kdvtuvb2_PtbJc3ON_J36A9uNgAKEK2cp23fZA_hr4BhZh_WA</recordid><startdate>20121127</startdate><enddate>20121127</enddate><creator>Börrnert, Felix</creator><creator>Fu, Lei</creator><creator>Gorantla, Sandeep</creator><creator>Knupfer, Martin</creator><creator>Büchner, Bernd</creator><creator>Rümmeli, Mark H</creator><general>American Chemical Society</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope></search><sort><creationdate>20121127</creationdate><title>Programmable Sub-nanometer Sculpting of Graphene with Electron Beams</title><author>Börrnert, Felix ; Fu, Lei ; Gorantla, Sandeep ; Knupfer, Martin ; Büchner, Bernd ; Rümmeli, Mark H</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a348t-efa932d063212768f1e2ae26e36ab491e5aca8a388520479809483b30f2b29c53</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2012</creationdate><topic>Beams (radiation)</topic><topic>Carbon</topic><topic>Condensing</topic><topic>Crystallization - methods</topic><topic>Deposition</topic><topic>Devices</topic><topic>Electron beams</topic><topic>Electron microscopes</topic><topic>Electrons</topic><topic>Graphene</topic><topic>Graphite - chemistry</topic><topic>Graphite - radiation effects</topic><topic>Macromolecular Substances - chemistry</topic><topic>Macromolecular Substances - radiation effects</topic><topic>Materials Testing</topic><topic>Molecular Conformation - radiation effects</topic><topic>Molecular Imprinting - methods</topic><topic>Nanostructure</topic><topic>Nanostructures - chemistry</topic><topic>Nanostructures - radiation effects</topic><topic>Nanostructures - ultrastructure</topic><topic>Particle Size</topic><topic>Surface Properties - radiation effects</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Börrnert, Felix</creatorcontrib><creatorcontrib>Fu, Lei</creatorcontrib><creatorcontrib>Gorantla, Sandeep</creatorcontrib><creatorcontrib>Knupfer, Martin</creatorcontrib><creatorcontrib>Büchner, Bernd</creatorcontrib><creatorcontrib>Rümmeli, Mark H</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>ACS nano</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Börrnert, Felix</au><au>Fu, Lei</au><au>Gorantla, Sandeep</au><au>Knupfer, Martin</au><au>Büchner, Bernd</au><au>Rümmeli, Mark H</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Programmable Sub-nanometer Sculpting of Graphene with Electron Beams</atitle><jtitle>ACS nano</jtitle><addtitle>ACS Nano</addtitle><date>2012-11-27</date><risdate>2012</risdate><volume>6</volume><issue>11</issue><spage>10327</spage><epage>10334</epage><pages>10327-10334</pages><issn>1936-0851</issn><eissn>1936-086X</eissn><abstract>Electron beams in transmission electron microscopes are very attractive to engineer and pattern graphene toward all-carbon device fabrication. The use of condensed beams typically used for sequential raster imaging is particularly exciting since they potentially provide high degrees of precision. However, technical difficulties, such as the formation of electron beam induced deposits on sample surfaces, have hindered the development of this technique. We demonstrate how one can successfully use a condensed electron beam, either with or without C s correction, to structure graphene with sub-nanometer precision in a programmable manner. We further demonstrate the potential of the developed technique by combining it with an established route to engineer graphene nanoribbons to single-atom carbon chains.</abstract><cop>United States</cop><pub>American Chemical Society</pub><pmid>23110721</pmid><doi>10.1021/nn304256a</doi><tpages>8</tpages></addata></record> |
fulltext | fulltext |
identifier | ISSN: 1936-0851 |
ispartof | ACS nano, 2012-11, Vol.6 (11), p.10327-10334 |
issn | 1936-0851 1936-086X |
language | eng |
recordid | cdi_proquest_miscellaneous_1762051545 |
source | ACS Publications; MEDLINE |
subjects | Beams (radiation) Carbon Condensing Crystallization - methods Deposition Devices Electron beams Electron microscopes Electrons Graphene Graphite - chemistry Graphite - radiation effects Macromolecular Substances - chemistry Macromolecular Substances - radiation effects Materials Testing Molecular Conformation - radiation effects Molecular Imprinting - methods Nanostructure Nanostructures - chemistry Nanostructures - radiation effects Nanostructures - ultrastructure Particle Size Surface Properties - radiation effects |
title | Programmable Sub-nanometer Sculpting of Graphene with Electron Beams |
url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-02-13T21%3A45%3A30IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Programmable%20Sub-nanometer%20Sculpting%20of%20Graphene%20with%20Electron%20Beams&rft.jtitle=ACS%20nano&rft.au=Bo%CC%88rrnert,%20Felix&rft.date=2012-11-27&rft.volume=6&rft.issue=11&rft.spage=10327&rft.epage=10334&rft.pages=10327-10334&rft.issn=1936-0851&rft.eissn=1936-086X&rft_id=info:doi/10.1021/nn304256a&rft_dat=%3Cproquest_cross%3E1762051545%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=1220572732&rft_id=info:pmid/23110721&rfr_iscdi=true |