Dimensionality Dependent Water Splitting Mechanisms on Free Manganese Oxide Clusters

The interaction of ligand-free manganese oxide nanoclusters with water is investigated, aiming at uncovering phenomena which could aid the design of artificial water-splitting molecular catalysts. Gas phase measurements in an ion trap in conjunction with first-principles calculations provide new mec...

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Veröffentlicht in:	Nano letters 2013-11, Vol.13 (11), p.5549-5555
Hauptverfasser:	Lang, Sandra M, Fleischer, Irene, Bernhardt, Thorsten M, Barnett, Robert N, Landman, Uzi
Format:	Artikel
Sprache:	eng
Schlagworte:	Catalysis Catalytic methods Charging Clusters Condensed matter: electronic structure, electrical, magnetic, and optical properties Cross-disciplinary physics: materials science rheology Electron states Exact sciences and technology Gases - chemistry Manganese Compounds - chemistry Manganese oxides Materials science Mathematical analysis Methods of electronic structure calculations Methods of nanofabrication Nanostructure Oxides - chemistry Oxygen - chemistry Phase Transition Physics Spectrum Analysis Transformations Vibration Vibrational spectra Water - chemistry Water splitting
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