Ultraclean Single, Double, and Triple Carbon Nanotube Quantum Dots with Recessed Re Bottom Gates
We demonstrate that ultraclean single, double, and triple quantum dots (QDs) can be formed reliably in a carbon nanotube (CNT) by a straightforward fabrication technique. The QDs are electrostatically defined in the CNT by closely spaced metallic bottom gates deposited in trenches in SiO2 by sputter...
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Veröffentlicht in: | Nano letters 2013-09, Vol.13 (9), p.4522-4526 |
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creator | Jung, Minkyung Schindele, Jens Nau, Stefan Weiss, Markus Baumgartner, Andreas Schönenberger, Christian |
description | We demonstrate that ultraclean single, double, and triple quantum dots (QDs) can be formed reliably in a carbon nanotube (CNT) by a straightforward fabrication technique. The QDs are electrostatically defined in the CNT by closely spaced metallic bottom gates deposited in trenches in SiO2 by sputter deposition of Re. The carbon nanotubes are then grown by chemical vapor deposition (CVD) across the trenches and contacted using conventional resist-based electron beam lithography. Unlike in previous work, the devices exhibit reproducibly the characteristics of ultraclean QDs behavior even after the subsequent electron beam lithography and chemical processing steps. We specifically demonstrate the high quality using CNT devices with two narrow bottom gates and one global back gate. Tunable by the gate voltages, the device can be operated in four different regimes: (i) fully p-type with ballistic transport between the outermost contacts (over a length of 700 nm), (ii) clean n-type single QD behavior where a QD can be induced by either the left or the right bottom gate, (iii) n-type double QD, and (iv) triple bipolar QD where the middle QD has opposite doping (p-type). Our simple fabrication scheme opens up a route to more complex devices based on ultraclean CNTs, since it allows for postgrowth processing. |
doi_str_mv | 10.1021/nl402455n |
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The QDs are electrostatically defined in the CNT by closely spaced metallic bottom gates deposited in trenches in SiO2 by sputter deposition of Re. The carbon nanotubes are then grown by chemical vapor deposition (CVD) across the trenches and contacted using conventional resist-based electron beam lithography. Unlike in previous work, the devices exhibit reproducibly the characteristics of ultraclean QDs behavior even after the subsequent electron beam lithography and chemical processing steps. We specifically demonstrate the high quality using CNT devices with two narrow bottom gates and one global back gate. Tunable by the gate voltages, the device can be operated in four different regimes: (i) fully p-type with ballistic transport between the outermost contacts (over a length of 700 nm), (ii) clean n-type single QD behavior where a QD can be induced by either the left or the right bottom gate, (iii) n-type double QD, and (iv) triple bipolar QD where the middle QD has opposite doping (p-type). Our simple fabrication scheme opens up a route to more complex devices based on ultraclean CNTs, since it allows for postgrowth processing.</description><identifier>ISSN: 1530-6984</identifier><identifier>EISSN: 1530-6992</identifier><identifier>DOI: 10.1021/nl402455n</identifier><identifier>PMID: 23962122</identifier><language>eng</language><publisher>Washington, DC: American Chemical Society</publisher><subject>Applied sciences ; Carbon nanotubes ; Chemical vapor deposition ; Cross-disciplinary physics: materials science; rheology ; Deposition ; Devices ; Electron beam lithography ; Electronics ; Exact sciences and technology ; Gates ; Materials science ; Molecular electronics, nanoelectronics ; Nanocrystalline materials ; Nanoscale materials and structures: fabrication and characterization ; Nanotubes ; Physics ; Quantum dots ; Semiconductor electronics. Microelectronics. Optoelectronics. Solid state devices ; Trenches</subject><ispartof>Nano letters, 2013-09, Vol.13 (9), p.4522-4526</ispartof><rights>Copyright © 2013 American Chemical Society</rights><rights>2014 INIST-CNRS</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a378t-1fa99ff8b0fcf24b4d94d4613b835535dd101c8acc973e95f6ebae0ab617e3a3</citedby><cites>FETCH-LOGICAL-a378t-1fa99ff8b0fcf24b4d94d4613b835535dd101c8acc973e95f6ebae0ab617e3a3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/nl402455n$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/nl402455n$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>314,780,784,2763,27074,27922,27923,56736,56786</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=27762746$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/23962122$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Jung, Minkyung</creatorcontrib><creatorcontrib>Schindele, Jens</creatorcontrib><creatorcontrib>Nau, Stefan</creatorcontrib><creatorcontrib>Weiss, Markus</creatorcontrib><creatorcontrib>Baumgartner, Andreas</creatorcontrib><creatorcontrib>Schönenberger, Christian</creatorcontrib><title>Ultraclean Single, Double, and Triple Carbon Nanotube Quantum Dots with Recessed Re Bottom Gates</title><title>Nano letters</title><addtitle>Nano Lett</addtitle><description>We demonstrate that ultraclean single, double, and triple quantum dots (QDs) can be formed reliably in a carbon nanotube (CNT) by a straightforward fabrication technique. The QDs are electrostatically defined in the CNT by closely spaced metallic bottom gates deposited in trenches in SiO2 by sputter deposition of Re. The carbon nanotubes are then grown by chemical vapor deposition (CVD) across the trenches and contacted using conventional resist-based electron beam lithography. Unlike in previous work, the devices exhibit reproducibly the characteristics of ultraclean QDs behavior even after the subsequent electron beam lithography and chemical processing steps. We specifically demonstrate the high quality using CNT devices with two narrow bottom gates and one global back gate. Tunable by the gate voltages, the device can be operated in four different regimes: (i) fully p-type with ballistic transport between the outermost contacts (over a length of 700 nm), (ii) clean n-type single QD behavior where a QD can be induced by either the left or the right bottom gate, (iii) n-type double QD, and (iv) triple bipolar QD where the middle QD has opposite doping (p-type). Our simple fabrication scheme opens up a route to more complex devices based on ultraclean CNTs, since it allows for postgrowth processing.</description><subject>Applied sciences</subject><subject>Carbon nanotubes</subject><subject>Chemical vapor deposition</subject><subject>Cross-disciplinary physics: materials science; rheology</subject><subject>Deposition</subject><subject>Devices</subject><subject>Electron beam lithography</subject><subject>Electronics</subject><subject>Exact sciences and technology</subject><subject>Gates</subject><subject>Materials science</subject><subject>Molecular electronics, nanoelectronics</subject><subject>Nanocrystalline materials</subject><subject>Nanoscale materials and structures: fabrication and characterization</subject><subject>Nanotubes</subject><subject>Physics</subject><subject>Quantum dots</subject><subject>Semiconductor electronics. Microelectronics. Optoelectronics. Solid state devices</subject><subject>Trenches</subject><issn>1530-6984</issn><issn>1530-6992</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2013</creationdate><recordtype>article</recordtype><recordid>eNqF0E2LFDEQBuAgiruuHvwDkoug4Gg-O52jjroKi6KO57aSrmgv6WRM0oj_3l52nL0Inuo9PFUFLyEPOXvOmeAvUlRMKK3TLXLKtWSbzlpx-5h7dULu1XrJGLNSs7vkREjbCS7EKfn2NbYCPiIk-mVK3yM-o6_z4q4mpJHuyrSPSLdQXE70A6TcFof00wKpLfNKW6W_pvaDfkaPteK4Bvoqt5Zneg4N631yJ0Cs-OAwz8ju7Zvd9t3m4uP5--3Liw1I07cND2BtCL1jwQehnBqtGlXHpeul1lKPI2fc9-C9NRKtDh06QAau4wYlyDPy5PrsvuSfC9Y2zFP1GCMkzEsduNFS9Zyt2_-lSgpmtLF6pU-vqS-51oJh2JdphvJ74Gy4qn44Vr_aR4ezi5txPMq_Xa_g8QFA9RBDgeSneuOM6YRR3Y0DX4fLvJS09vaPh38AhCOWrA</recordid><startdate>20130911</startdate><enddate>20130911</enddate><creator>Jung, Minkyung</creator><creator>Schindele, Jens</creator><creator>Nau, Stefan</creator><creator>Weiss, Markus</creator><creator>Baumgartner, Andreas</creator><creator>Schönenberger, Christian</creator><general>American Chemical Society</general><scope>IQODW</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope></search><sort><creationdate>20130911</creationdate><title>Ultraclean Single, Double, and Triple Carbon Nanotube Quantum Dots with Recessed Re Bottom Gates</title><author>Jung, Minkyung ; Schindele, Jens ; Nau, Stefan ; Weiss, Markus ; Baumgartner, Andreas ; Schönenberger, Christian</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a378t-1fa99ff8b0fcf24b4d94d4613b835535dd101c8acc973e95f6ebae0ab617e3a3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2013</creationdate><topic>Applied sciences</topic><topic>Carbon nanotubes</topic><topic>Chemical vapor deposition</topic><topic>Cross-disciplinary physics: materials science; rheology</topic><topic>Deposition</topic><topic>Devices</topic><topic>Electron beam lithography</topic><topic>Electronics</topic><topic>Exact sciences and technology</topic><topic>Gates</topic><topic>Materials science</topic><topic>Molecular electronics, nanoelectronics</topic><topic>Nanocrystalline materials</topic><topic>Nanoscale materials and structures: fabrication and characterization</topic><topic>Nanotubes</topic><topic>Physics</topic><topic>Quantum dots</topic><topic>Semiconductor electronics. Microelectronics. Optoelectronics. Solid state devices</topic><topic>Trenches</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Jung, Minkyung</creatorcontrib><creatorcontrib>Schindele, Jens</creatorcontrib><creatorcontrib>Nau, Stefan</creatorcontrib><creatorcontrib>Weiss, Markus</creatorcontrib><creatorcontrib>Baumgartner, Andreas</creatorcontrib><creatorcontrib>Schönenberger, Christian</creatorcontrib><collection>Pascal-Francis</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Nano letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Jung, Minkyung</au><au>Schindele, Jens</au><au>Nau, Stefan</au><au>Weiss, Markus</au><au>Baumgartner, Andreas</au><au>Schönenberger, Christian</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Ultraclean Single, Double, and Triple Carbon Nanotube Quantum Dots with Recessed Re Bottom Gates</atitle><jtitle>Nano letters</jtitle><addtitle>Nano Lett</addtitle><date>2013-09-11</date><risdate>2013</risdate><volume>13</volume><issue>9</issue><spage>4522</spage><epage>4526</epage><pages>4522-4526</pages><issn>1530-6984</issn><eissn>1530-6992</eissn><abstract>We demonstrate that ultraclean single, double, and triple quantum dots (QDs) can be formed reliably in a carbon nanotube (CNT) by a straightforward fabrication technique. The QDs are electrostatically defined in the CNT by closely spaced metallic bottom gates deposited in trenches in SiO2 by sputter deposition of Re. The carbon nanotubes are then grown by chemical vapor deposition (CVD) across the trenches and contacted using conventional resist-based electron beam lithography. Unlike in previous work, the devices exhibit reproducibly the characteristics of ultraclean QDs behavior even after the subsequent electron beam lithography and chemical processing steps. We specifically demonstrate the high quality using CNT devices with two narrow bottom gates and one global back gate. Tunable by the gate voltages, the device can be operated in four different regimes: (i) fully p-type with ballistic transport between the outermost contacts (over a length of 700 nm), (ii) clean n-type single QD behavior where a QD can be induced by either the left or the right bottom gate, (iii) n-type double QD, and (iv) triple bipolar QD where the middle QD has opposite doping (p-type). Our simple fabrication scheme opens up a route to more complex devices based on ultraclean CNTs, since it allows for postgrowth processing.</abstract><cop>Washington, DC</cop><pub>American Chemical Society</pub><pmid>23962122</pmid><doi>10.1021/nl402455n</doi><tpages>5</tpages></addata></record> |
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subjects | Applied sciences Carbon nanotubes Chemical vapor deposition Cross-disciplinary physics: materials science rheology Deposition Devices Electron beam lithography Electronics Exact sciences and technology Gates Materials science Molecular electronics, nanoelectronics Nanocrystalline materials Nanoscale materials and structures: fabrication and characterization Nanotubes Physics Quantum dots Semiconductor electronics. Microelectronics. Optoelectronics. Solid state devices Trenches |
title | Ultraclean Single, Double, and Triple Carbon Nanotube Quantum Dots with Recessed Re Bottom Gates |
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