On the role of hydrophobic Si-based protective coatings in limiting mortar deterioration
In order to avoid both natural and artificial stone decay, mainly due to the interaction with atmospheric pollutants (both gases such as NOₓ and SO₂ and particulate matter), polymeric materials have been widely studied as protective coatings enable to limit the penetration of fluids into the bulk ma...
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| Veröffentlicht in: | Environmental science and pollution research international 2015-11, Vol.22 (22), p.17733-17743 |
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| creator | Cappelletti, G Fermo, P Pino, F Pargoletti, E Pecchioni, E Fratini, F Ruffolo, S. A La Russa, M. F |
| description | In order to avoid both natural and artificial stone decay, mainly due to the interaction with atmospheric pollutants (both gases such as NOₓ and SO₂ and particulate matter), polymeric materials have been widely studied as protective coatings enable to limit the penetration of fluids into the bulk material. In the current work, an air hardening calcic lime mortar (ALM) and a natural hydraulic lime mortar (HLM) were used as substrates, and commercially available Si-based resins (Alpha®SI30 and Silres®BS16) were adopted as protective agents to give hydrophobicity features to the artificial stones. Surface properties of coatings and their performance as hydrophobic agents were studied using different techniques such as contact angle measurements, capillary absorption test, mercury intrusion porosimetry, surface free energy, colorimetric measurements and water vapour permeability tests. Finally, some exposure tests to UV radiation and to real polluted atmospheric environments (a city centre and an urban background site) were carried out during a wintertime period (when the concentrations of the main atmospheric pollutants are higher) in order to study the durability of the coating systems applied. The effectiveness of the two commercial resins in reducing salt formation (sulphate and nitrate), induced by the interaction of the mortars with the atmospheric pollutants, was demonstrated in the case of the HLM mortar. |
| doi_str_mv | 10.1007/s11356-015-4962-0 |
| format | Article |
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Surface properties of coatings and their performance as hydrophobic agents were studied using different techniques such as contact angle measurements, capillary absorption test, mercury intrusion porosimetry, surface free energy, colorimetric measurements and water vapour permeability tests. Finally, some exposure tests to UV radiation and to real polluted atmospheric environments (a city centre and an urban background site) were carried out during a wintertime period (when the concentrations of the main atmospheric pollutants are higher) in order to study the durability of the coating systems applied. The effectiveness of the two commercial resins in reducing salt formation (sulphate and nitrate), induced by the interaction of the mortars with the atmospheric pollutants, was demonstrated in the case of the HLM mortar.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-015-4962-0</identifier><identifier>PMID: 26154039</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>absorption ; air ; Air Pollutants - chemistry ; Air pollution ; Alkalies ; Aquatic ecosystems ; Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; Calcium Compounds - chemistry ; Coatings ; Colorimetry ; Construction Industry ; Construction Materials ; Contact angle ; Cultural heritage ; Decay ; durability ; Earth and Environmental Science ; Ecotoxicology ; energy ; Environment ; Environmental Chemistry ; Environmental conditions ; Environmental Health ; Free energy ; Hydraulics ; Hydrophobic and Hydrophilic Interactions ; Hydrophobicity ; Membrane permeability ; Mercury ; nitrates ; nitrogen oxides ; Oxides - chemistry ; Particulate matter ; Particulate Matter - chemistry ; particulates ; Permeability ; Pollutants ; Polymers ; Protective coatings ; Radiation measurement ; Research Article ; Resins ; silicon ; Stone ; sulfates ; Sulfur dioxide ; Surface Properties ; Thermodynamics ; Ultraviolet radiation ; Waste Water Technology ; Water Management ; Water Pollution Control ; Water vapor ; winter</subject><ispartof>Environmental science and pollution research international, 2015-11, Vol.22 (22), p.17733-17743</ispartof><rights>Springer-Verlag Berlin Heidelberg 2015</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c540t-53c1dc691585c815675909846293568334da998eefadd7b90005ea84372e8ab3</citedby><cites>FETCH-LOGICAL-c540t-53c1dc691585c815675909846293568334da998eefadd7b90005ea84372e8ab3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-015-4962-0$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-015-4962-0$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,778,782,27907,27908,41471,42540,51302</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/26154039$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Cappelletti, G</creatorcontrib><creatorcontrib>Fermo, P</creatorcontrib><creatorcontrib>Pino, F</creatorcontrib><creatorcontrib>Pargoletti, E</creatorcontrib><creatorcontrib>Pecchioni, E</creatorcontrib><creatorcontrib>Fratini, F</creatorcontrib><creatorcontrib>Ruffolo, S. A</creatorcontrib><creatorcontrib>La Russa, M. F</creatorcontrib><title>On the role of hydrophobic Si-based protective coatings in limiting mortar deterioration</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>In order to avoid both natural and artificial stone decay, mainly due to the interaction with atmospheric pollutants (both gases such as NOₓ and SO₂ and particulate matter), polymeric materials have been widely studied as protective coatings enable to limit the penetration of fluids into the bulk material. In the current work, an air hardening calcic lime mortar (ALM) and a natural hydraulic lime mortar (HLM) were used as substrates, and commercially available Si-based resins (Alpha®SI30 and Silres®BS16) were adopted as protective agents to give hydrophobicity features to the artificial stones. Surface properties of coatings and their performance as hydrophobic agents were studied using different techniques such as contact angle measurements, capillary absorption test, mercury intrusion porosimetry, surface free energy, colorimetric measurements and water vapour permeability tests. Finally, some exposure tests to UV radiation and to real polluted atmospheric environments (a city centre and an urban background site) were carried out during a wintertime period (when the concentrations of the main atmospheric pollutants are higher) in order to study the durability of the coating systems applied. The effectiveness of the two commercial resins in reducing salt formation (sulphate and nitrate), induced by the interaction of the mortars with the atmospheric pollutants, was demonstrated in the case of the HLM mortar.</description><subject>absorption</subject><subject>air</subject><subject>Air Pollutants - chemistry</subject><subject>Air pollution</subject><subject>Alkalies</subject><subject>Aquatic ecosystems</subject><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Calcium Compounds - chemistry</subject><subject>Coatings</subject><subject>Colorimetry</subject><subject>Construction Industry</subject><subject>Construction Materials</subject><subject>Contact angle</subject><subject>Cultural heritage</subject><subject>Decay</subject><subject>durability</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>energy</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental conditions</subject><subject>Environmental Health</subject><subject>Free energy</subject><subject>Hydraulics</subject><subject>Hydrophobic and Hydrophilic Interactions</subject><subject>Hydrophobicity</subject><subject>Membrane permeability</subject><subject>Mercury</subject><subject>nitrates</subject><subject>nitrogen oxides</subject><subject>Oxides - chemistry</subject><subject>Particulate matter</subject><subject>Particulate Matter - chemistry</subject><subject>particulates</subject><subject>Permeability</subject><subject>Pollutants</subject><subject>Polymers</subject><subject>Protective coatings</subject><subject>Radiation measurement</subject><subject>Research Article</subject><subject>Resins</subject><subject>silicon</subject><subject>Stone</subject><subject>sulfates</subject><subject>Sulfur dioxide</subject><subject>Surface Properties</subject><subject>Thermodynamics</subject><subject>Ultraviolet radiation</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water Pollution Control</subject><subject>Water vapor</subject><subject>winter</subject><issn>0944-1344</issn><issn>1614-7499</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2015</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNqNkU2LFDEQhoMo7uzoD_CiAS97aa3KVydHWfyChT3sCt5COp2eydLdGZOehf33ZuhVxIN4Kop63reqeAl5hfAOAdr3BZFL1QDKRhjFGnhCNqhQNK0w5inZgBGiQS7EGTkv5Q6AgWHtc3LGFEoB3GzI9-uZLvtAcxoDTQPdP_Q5Hfapi57exKZzJfT0kNMS_BLvA_XJLXHeFRpnOsYpnho6pby4TPuwhBxTrkSaX5BngxtLePlYt-T208fbyy_N1fXnr5cfrhpfL1gayT32XhmUWnqNUrXSgNFCMVNf05yL3hmjQxhc37edAQAZnBa8ZUG7jm_JxWpbb_xxDGWxUyw-jKObQzoWi61Ehkpw8R8ol5wzqFu35O1f6F065rn-USmtpTEtZ5XClfI5lZLDYA85Ti4_WAR7CsiuAdkakD0FZKFqXj86H7sp9L8VvxKpAFuBUkfzLuQ_Vv_D9c0qGlyybpdjsd9uGKACQI5CKP4T7gSicw</recordid><startdate>20151101</startdate><enddate>20151101</enddate><creator>Cappelletti, G</creator><creator>Fermo, P</creator><creator>Pino, F</creator><creator>Pargoletti, E</creator><creator>Pecchioni, E</creator><creator>Fratini, F</creator><creator>Ruffolo, S. 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| subjects | absorption air Air Pollutants - chemistry Air pollution Alkalies Aquatic ecosystems Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Calcium Compounds - chemistry Coatings Colorimetry Construction Industry Construction Materials Contact angle Cultural heritage Decay durability Earth and Environmental Science Ecotoxicology energy Environment Environmental Chemistry Environmental conditions Environmental Health Free energy Hydraulics Hydrophobic and Hydrophilic Interactions Hydrophobicity Membrane permeability Mercury nitrates nitrogen oxides Oxides - chemistry Particulate matter Particulate Matter - chemistry particulates Permeability Pollutants Polymers Protective coatings Radiation measurement Research Article Resins silicon Stone sulfates Sulfur dioxide Surface Properties Thermodynamics Ultraviolet radiation Waste Water Technology Water Management Water Pollution Control Water vapor winter |
| title | On the role of hydrophobic Si-based protective coatings in limiting mortar deterioration |
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