Reactive atmospheric pressure plasma for highly efficient removal of structure-directing agents from zeolite thin films
We present a novel approach to remove the structure-directing agent (SDA) from as-synthesized zeolites using an atmospheric pressure plasma jet (APPJ). This reduces the time required to less than 60 seconds as compared to the existing thermal calcination, whose durations range from hours to days. Th...
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| Veröffentlicht in: | Chemical communications (Cambridge, England) England), 2015-09, Vol.51 (73), p.13910-13913 |
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| container_end_page | 13913 |
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| container_issue | 73 |
| container_start_page | 13910 |
| container_title | Chemical communications (Cambridge, England) |
| container_volume | 51 |
| creator | Chien, H-T Chen, M-C Huang, P-S Lai, J-Y Hsu, C-C Kang, D-Y |
| description | We present a novel approach to remove the structure-directing agent (SDA) from as-synthesized zeolites using an atmospheric pressure plasma jet (APPJ). This reduces the time required to less than 60 seconds as compared to the existing thermal calcination, whose durations range from hours to days. The highly reactive plasma also results in a pronounced Q(3)-to-Q(4) transformation in the pure-silica zeolite MFI. |
| doi_str_mv | 10.1039/c5cc04067a |
| format | Article |
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This reduces the time required to less than 60 seconds as compared to the existing thermal calcination, whose durations range from hours to days. The highly reactive plasma also results in a pronounced Q(3)-to-Q(4) transformation in the pure-silica zeolite MFI.</description><subject>Atmospheric pressure</subject><subject>Barometric pressure</subject><subject>Calcination</subject><subject>MFI</subject><subject>Thin films</subject><subject>Transformations</subject><subject>Zeolites</subject><issn>1359-7345</issn><issn>1364-548X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2015</creationdate><recordtype>article</recordtype><recordid>eNqNkU1L7TAQQIMo6lM3_gDJUoRq0jRpspSivgeCIAruSu50cm-kvalJquivtz4_1s5mZnHmbA4hh5ydcibMGUgAVjFV2w2yy4WqClnph82PW5qiFpXcIX9SemTzcKm3yU6pSmFqaXbJyy1ayP4Zqc1DSOMKowc6RkxpikjH3qbBUhciXfnlqn-l6JwHj-tMIw7h2fY0OJpynCDPD0XnI86-9ZLa5Qwl6mIY6BuG3mekeeXX1Pl-SPtky9k-4cHX3iP3lxd3zd_i-ubqX3N-XYAoWS60AMGNMkIB1x2ztbKi4pWyC96xzgA47JALRKk1SmOUAmcNt1wD6IXWYo8cf3rHGJ4mTLkdfALse7vGMKWW11VVc12W7Bco01wxw82MnnyiEENKEV07Rj_Y-Npy1n40aRvZNP-bnM_w0Zd3WgzY_aDfEcQ7d4GJbQ</recordid><startdate>20150921</startdate><enddate>20150921</enddate><creator>Chien, H-T</creator><creator>Chen, M-C</creator><creator>Huang, P-S</creator><creator>Lai, J-Y</creator><creator>Hsu, C-C</creator><creator>Kang, D-Y</creator><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope></search><sort><creationdate>20150921</creationdate><title>Reactive atmospheric pressure plasma for highly efficient removal of structure-directing agents from zeolite thin films</title><author>Chien, H-T ; Chen, M-C ; Huang, P-S ; Lai, J-Y ; Hsu, C-C ; Kang, D-Y</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c320t-83c3196936c18d0a76a34146ab1d0d9ccfede13ee588e59966cfa91a18cc8b883</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2015</creationdate><topic>Atmospheric pressure</topic><topic>Barometric pressure</topic><topic>Calcination</topic><topic>MFI</topic><topic>Thin films</topic><topic>Transformations</topic><topic>Zeolites</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Chien, H-T</creatorcontrib><creatorcontrib>Chen, M-C</creatorcontrib><creatorcontrib>Huang, P-S</creatorcontrib><creatorcontrib>Lai, J-Y</creatorcontrib><creatorcontrib>Hsu, C-C</creatorcontrib><creatorcontrib>Kang, D-Y</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Chemical communications (Cambridge, England)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Chien, H-T</au><au>Chen, M-C</au><au>Huang, P-S</au><au>Lai, J-Y</au><au>Hsu, C-C</au><au>Kang, D-Y</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Reactive atmospheric pressure plasma for highly efficient removal of structure-directing agents from zeolite thin films</atitle><jtitle>Chemical communications (Cambridge, England)</jtitle><addtitle>Chem Commun (Camb)</addtitle><date>2015-09-21</date><risdate>2015</risdate><volume>51</volume><issue>73</issue><spage>13910</spage><epage>13913</epage><pages>13910-13913</pages><issn>1359-7345</issn><eissn>1364-548X</eissn><abstract>We present a novel approach to remove the structure-directing agent (SDA) from as-synthesized zeolites using an atmospheric pressure plasma jet (APPJ). 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| fulltext | fulltext |
| identifier | ISSN: 1359-7345 |
| ispartof | Chemical communications (Cambridge, England), 2015-09, Vol.51 (73), p.13910-13913 |
| issn | 1359-7345 1364-548X |
| language | eng |
| recordid | cdi_proquest_miscellaneous_1744718220 |
| source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
| subjects | Atmospheric pressure Barometric pressure Calcination MFI Thin films Transformations Zeolites |
| title | Reactive atmospheric pressure plasma for highly efficient removal of structure-directing agents from zeolite thin films |
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