Polychlorinated biphenyl contamination of paints containing polycyclic- and Naphthol AS-type pigments
This study reports the concentrations and congener partners of polychlorinated biphenyls (PCBs) in commercially available paints. Polycyclic-type pigments containing dioxazine violet (pigment violet (PV) 23, PV37) and diketopyrrolopyrrole (PR254, PR255) were found to contain PCB-56, PCB-77, PCB-40,...
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| Veröffentlicht in: | Environmental science and pollution research international 2015-10, Vol.22 (19), p.14478-14488 |
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| creator | Anezaki, Katsunori Kannan, Narayanan Nakano, Takeshi |
| description | This study reports the concentrations and congener partners of polychlorinated biphenyls (PCBs) in commercially available paints. Polycyclic-type pigments containing dioxazine violet (pigment violet (PV) 23, PV37) and diketopyrrolopyrrole (PR254, PR255) were found to contain PCB-56, PCB-77, PCB-40, PCB-5, and PCB-12, and PCB-6, PCB-13, and PCB-15, respectively, as major congeners. Dioxazine violet is contaminated with by-products during synthesis from
o
-dichlorobenzene, which is used as a solvent during synthesis, and diketopyrrolopyrrole is contaminated with by-products during synthesis from
p
-chlorobenzonitrile. The concentration of PCBs in paint containing PV23 or PV37 was 0.050–29 mg/kg, and toxic equivalency (TEQ) values ranged 1.1–160 pg-TEQ/g. The concentration of PCBs in paint containing PR254 or PR255 was 0.0019–2.4 mg/kg. Naphthol AS is an azo-type pigment, and PCB-52 was detected in paint containing pigment red (PR) 9 with 2,5-dichloroaniline as its source. PCB-146, PCB-149, and PCB-153 were identified from paint containing PR112 produced from 2,4,5-trichloroaniline, as major congeners. These congeners have chlorine positions similar to aniline, indicating that these congeners are by-products obtained during the synthesis of pigments. The concentrations of PCBs in paints containing PR9 and PR112 were 0.0042–0.43 and 0.0044–3.8 mg/kg, respectively. The corresponding TEQ for PR112 was 0.0039–8.6 pg-TEQ/g. |
| doi_str_mv | 10.1007/s11356-014-2985-6 |
| format | Article |
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o
-dichlorobenzene, which is used as a solvent during synthesis, and diketopyrrolopyrrole is contaminated with by-products during synthesis from
p
-chlorobenzonitrile. The concentration of PCBs in paint containing PV23 or PV37 was 0.050–29 mg/kg, and toxic equivalency (TEQ) values ranged 1.1–160 pg-TEQ/g. The concentration of PCBs in paint containing PR254 or PR255 was 0.0019–2.4 mg/kg. Naphthol AS is an azo-type pigment, and PCB-52 was detected in paint containing pigment red (PR) 9 with 2,5-dichloroaniline as its source. PCB-146, PCB-149, and PCB-153 were identified from paint containing PR112 produced from 2,4,5-trichloroaniline, as major congeners. These congeners have chlorine positions similar to aniline, indicating that these congeners are by-products obtained during the synthesis of pigments. The concentrations of PCBs in paints containing PR9 and PR112 were 0.0042–0.43 and 0.0044–3.8 mg/kg, respectively. The corresponding TEQ for PR112 was 0.0039–8.6 pg-TEQ/g.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-014-2985-6</identifier><identifier>PMID: 24809497</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>12th IHPA Forum and selected studies on POPs ; Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; By products ; Byproducts ; Chlorine ; Coloring Agents - analysis ; Coloring Agents - chemistry ; Conventions ; Dichlorobenzene ; Dioxins ; Earth and Environmental Science ; Ecotoxicology ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental Pollutants - analysis ; Environmental Pollutants - chemistry ; Environmental science ; Gas Chromatography-Mass Spectrometry ; Laboratories ; Limit of Detection ; Molecular Structure ; Molecular weight ; Naphthols - analysis ; Naphthols - chemistry ; Paint - analysis ; Paint - standards ; Paints ; PCB ; Pigments ; Polychlorinated biphenyls ; Polychlorinated Biphenyls - analysis ; Polychlorinated Biphenyls - chemistry ; Polycyclic Aromatic Hydrocarbons - analysis ; Polycyclic Aromatic Hydrocarbons - chemistry ; Solvents ; Studies ; Toxicity ; Waste Water Technology ; Water Management ; Water Pollution Control</subject><ispartof>Environmental science and pollution research international, 2015-10, Vol.22 (19), p.14478-14488</ispartof><rights>Springer-Verlag Berlin Heidelberg 2014</rights><rights>Springer-Verlag Berlin Heidelberg 2015</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c648t-1018d194e8671c24f8339c1e5b83d672d561f9db19a1e1d02ead2f08da7844923</citedby><cites>FETCH-LOGICAL-c648t-1018d194e8671c24f8339c1e5b83d672d561f9db19a1e1d02ead2f08da7844923</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-014-2985-6$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-014-2985-6$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/24809497$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Anezaki, Katsunori</creatorcontrib><creatorcontrib>Kannan, Narayanan</creatorcontrib><creatorcontrib>Nakano, Takeshi</creatorcontrib><title>Polychlorinated biphenyl contamination of paints containing polycyclic- and Naphthol AS-type pigments</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>This study reports the concentrations and congener partners of polychlorinated biphenyls (PCBs) in commercially available paints. Polycyclic-type pigments containing dioxazine violet (pigment violet (PV) 23, PV37) and diketopyrrolopyrrole (PR254, PR255) were found to contain PCB-56, PCB-77, PCB-40, PCB-5, and PCB-12, and PCB-6, PCB-13, and PCB-15, respectively, as major congeners. Dioxazine violet is contaminated with by-products during synthesis from
o
-dichlorobenzene, which is used as a solvent during synthesis, and diketopyrrolopyrrole is contaminated with by-products during synthesis from
p
-chlorobenzonitrile. The concentration of PCBs in paint containing PV23 or PV37 was 0.050–29 mg/kg, and toxic equivalency (TEQ) values ranged 1.1–160 pg-TEQ/g. The concentration of PCBs in paint containing PR254 or PR255 was 0.0019–2.4 mg/kg. Naphthol AS is an azo-type pigment, and PCB-52 was detected in paint containing pigment red (PR) 9 with 2,5-dichloroaniline as its source. PCB-146, PCB-149, and PCB-153 were identified from paint containing PR112 produced from 2,4,5-trichloroaniline, as major congeners. These congeners have chlorine positions similar to aniline, indicating that these congeners are by-products obtained during the synthesis of pigments. The concentrations of PCBs in paints containing PR9 and PR112 were 0.0042–0.43 and 0.0044–3.8 mg/kg, respectively. The corresponding TEQ for PR112 was 0.0039–8.6 pg-TEQ/g.</description><subject>12th IHPA Forum and selected studies on POPs</subject><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>By products</subject><subject>Byproducts</subject><subject>Chlorine</subject><subject>Coloring Agents - analysis</subject><subject>Coloring Agents - chemistry</subject><subject>Conventions</subject><subject>Dichlorobenzene</subject><subject>Dioxins</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental Pollutants - analysis</subject><subject>Environmental Pollutants - chemistry</subject><subject>Environmental science</subject><subject>Gas Chromatography-Mass Spectrometry</subject><subject>Laboratories</subject><subject>Limit of Detection</subject><subject>Molecular Structure</subject><subject>Molecular weight</subject><subject>Naphthols - analysis</subject><subject>Naphthols - chemistry</subject><subject>Paint - analysis</subject><subject>Paint - standards</subject><subject>Paints</subject><subject>PCB</subject><subject>Pigments</subject><subject>Polychlorinated biphenyls</subject><subject>Polychlorinated Biphenyls - analysis</subject><subject>Polychlorinated Biphenyls - chemistry</subject><subject>Polycyclic Aromatic Hydrocarbons - analysis</subject><subject>Polycyclic Aromatic Hydrocarbons - chemistry</subject><subject>Solvents</subject><subject>Studies</subject><subject>Toxicity</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water Pollution Control</subject><issn>0944-1344</issn><issn>1614-7499</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2015</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><sourceid>BENPR</sourceid><recordid>eNp1kU9v1DAQxS0EotvCB-CCLHHhYvA4jv8cq6pQpIpWKpwtr-3sukrsEGcP-fZ1lIIQEqfRzPzeG8sPoXdAPwGl8nMBaFpBKHDCtGqJeIF2IGonudYv0Y5qzgk0nJ-h81IeKWVUM_kanTGu6k7LHQr3uV_csc9TTHYOHu_jeAxp6bHLabbDOo054dzh0cY0l20eU0wHPK7axfXREWyTx9_teJyPuceXD2RexoDHeBhCFb1Brzrbl_D2uV6gn1-uf1zdkNu7r9-uLm-JE1zNBCgoD5oHJSQ4xjvVNNpBaPeq8UIy3wrotN-DthDAUxasZx1V3krFuWbNBfq4-Y5T_nUKZTZDLC70vU0hn4oByaRQDddQ0Q__oI_5NKX6ukqBbptWaVEp2Cg35VKm0JlxioOdFgPUrBmYLQNTMzBrBmbVvH92Pu2H4P8ofn96BdgGlLpKhzD9dfq_rk9rEZH6</recordid><startdate>20151001</startdate><enddate>20151001</enddate><creator>Anezaki, Katsunori</creator><creator>Kannan, Narayanan</creator><creator>Nakano, Takeshi</creator><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7QL</scope><scope>7SN</scope><scope>7T7</scope><scope>7TV</scope><scope>7U7</scope><scope>7WY</scope><scope>7WZ</scope><scope>7X7</scope><scope>7XB</scope><scope>87Z</scope><scope>88E</scope><scope>88I</scope><scope>8AO</scope><scope>8C1</scope><scope>8FD</scope><scope>8FI</scope><scope>8FJ</scope><scope>8FK</scope><scope>8FL</scope><scope>ABUWG</scope><scope>AEUYN</scope><scope>AFKRA</scope><scope>ATCPS</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BEZIV</scope><scope>BHPHI</scope><scope>C1K</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>FR3</scope><scope>FRNLG</scope><scope>FYUFA</scope><scope>F~G</scope><scope>GHDGH</scope><scope>GNUQQ</scope><scope>HCIFZ</scope><scope>K60</scope><scope>K6~</scope><scope>K9.</scope><scope>L.-</scope><scope>M0C</scope><scope>M0S</scope><scope>M1P</scope><scope>M2P</scope><scope>M7N</scope><scope>P64</scope><scope>PATMY</scope><scope>PQBIZ</scope><scope>PQBZA</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PYCSY</scope><scope>Q9U</scope><scope>7ST</scope><scope>SOI</scope></search><sort><creationdate>20151001</creationdate><title>Polychlorinated biphenyl contamination of paints containing polycyclic- and Naphthol AS-type pigments</title><author>Anezaki, Katsunori ; Kannan, Narayanan ; Nakano, Takeshi</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c648t-1018d194e8671c24f8339c1e5b83d672d561f9db19a1e1d02ead2f08da7844923</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2015</creationdate><topic>12th IHPA Forum and selected studies on POPs</topic><topic>Aquatic Pollution</topic><topic>Atmospheric Protection/Air Quality Control/Air Pollution</topic><topic>By products</topic><topic>Byproducts</topic><topic>Chlorine</topic><topic>Coloring Agents - 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analysis</topic><topic>Polycyclic Aromatic Hydrocarbons - chemistry</topic><topic>Solvents</topic><topic>Studies</topic><topic>Toxicity</topic><topic>Waste Water Technology</topic><topic>Water Management</topic><topic>Water Pollution Control</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Anezaki, Katsunori</creatorcontrib><creatorcontrib>Kannan, Narayanan</creatorcontrib><creatorcontrib>Nakano, Takeshi</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>Bacteriology Abstracts (Microbiology B)</collection><collection>Ecology Abstracts</collection><collection>Industrial and Applied Microbiology Abstracts (Microbiology A)</collection><collection>Pollution Abstracts</collection><collection>Toxicology Abstracts</collection><collection>ABI/INFORM Collection</collection><collection>ABI/INFORM Global (PDF only)</collection><collection>Health & Medical Collection</collection><collection>ProQuest Central (purchase pre-March 2016)</collection><collection>ABI/INFORM Global (Alumni Edition)</collection><collection>Medical Database (Alumni Edition)</collection><collection>Science Database (Alumni Edition)</collection><collection>ProQuest Pharma Collection</collection><collection>Public Health Database</collection><collection>Technology Research Database</collection><collection>Hospital Premium Collection</collection><collection>Hospital Premium Collection (Alumni Edition)</collection><collection>ProQuest Central (Alumni) (purchase pre-March 2016)</collection><collection>ABI/INFORM Collection (Alumni Edition)</collection><collection>ProQuest Central (Alumni Edition)</collection><collection>ProQuest One Sustainability</collection><collection>ProQuest Central UK/Ireland</collection><collection>Agricultural & Environmental Science Collection</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>Business Premium Collection</collection><collection>Natural Science Collection</collection><collection>Environmental Sciences and Pollution Management</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central Korea</collection><collection>Engineering Research Database</collection><collection>Business Premium Collection (Alumni)</collection><collection>Health Research Premium Collection</collection><collection>ABI/INFORM Global (Corporate)</collection><collection>Health Research Premium Collection (Alumni)</collection><collection>ProQuest Central Student</collection><collection>SciTech Premium Collection</collection><collection>ProQuest Business Collection (Alumni Edition)</collection><collection>ProQuest Business Collection</collection><collection>ProQuest Health & Medical Complete (Alumni)</collection><collection>ABI/INFORM Professional Advanced</collection><collection>ABI/INFORM Global</collection><collection>Health & Medical Collection (Alumni Edition)</collection><collection>Medical Database</collection><collection>Science Database</collection><collection>Algology Mycology and Protozoology Abstracts (Microbiology C)</collection><collection>Biotechnology and BioEngineering Abstracts</collection><collection>Environmental Science Database</collection><collection>ProQuest One Business</collection><collection>ProQuest One Business (Alumni)</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>Environmental Science Collection</collection><collection>ProQuest Central Basic</collection><collection>Environment Abstracts</collection><collection>Environment Abstracts</collection><jtitle>Environmental science and pollution research international</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Anezaki, Katsunori</au><au>Kannan, Narayanan</au><au>Nakano, Takeshi</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Polychlorinated biphenyl contamination of paints containing polycyclic- and Naphthol AS-type pigments</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2015-10-01</date><risdate>2015</risdate><volume>22</volume><issue>19</issue><spage>14478</spage><epage>14488</epage><pages>14478-14488</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>This study reports the concentrations and congener partners of polychlorinated biphenyls (PCBs) in commercially available paints. Polycyclic-type pigments containing dioxazine violet (pigment violet (PV) 23, PV37) and diketopyrrolopyrrole (PR254, PR255) were found to contain PCB-56, PCB-77, PCB-40, PCB-5, and PCB-12, and PCB-6, PCB-13, and PCB-15, respectively, as major congeners. Dioxazine violet is contaminated with by-products during synthesis from
o
-dichlorobenzene, which is used as a solvent during synthesis, and diketopyrrolopyrrole is contaminated with by-products during synthesis from
p
-chlorobenzonitrile. The concentration of PCBs in paint containing PV23 or PV37 was 0.050–29 mg/kg, and toxic equivalency (TEQ) values ranged 1.1–160 pg-TEQ/g. The concentration of PCBs in paint containing PR254 or PR255 was 0.0019–2.4 mg/kg. Naphthol AS is an azo-type pigment, and PCB-52 was detected in paint containing pigment red (PR) 9 with 2,5-dichloroaniline as its source. PCB-146, PCB-149, and PCB-153 were identified from paint containing PR112 produced from 2,4,5-trichloroaniline, as major congeners. These congeners have chlorine positions similar to aniline, indicating that these congeners are by-products obtained during the synthesis of pigments. The concentrations of PCBs in paints containing PR9 and PR112 were 0.0042–0.43 and 0.0044–3.8 mg/kg, respectively. The corresponding TEQ for PR112 was 0.0039–8.6 pg-TEQ/g.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>24809497</pmid><doi>10.1007/s11356-014-2985-6</doi><tpages>11</tpages></addata></record> |
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| ispartof | Environmental science and pollution research international, 2015-10, Vol.22 (19), p.14478-14488 |
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| subjects | 12th IHPA Forum and selected studies on POPs Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution By products Byproducts Chlorine Coloring Agents - analysis Coloring Agents - chemistry Conventions Dichlorobenzene Dioxins Earth and Environmental Science Ecotoxicology Environment Environmental Chemistry Environmental Health Environmental Pollutants - analysis Environmental Pollutants - chemistry Environmental science Gas Chromatography-Mass Spectrometry Laboratories Limit of Detection Molecular Structure Molecular weight Naphthols - analysis Naphthols - chemistry Paint - analysis Paint - standards Paints PCB Pigments Polychlorinated biphenyls Polychlorinated Biphenyls - analysis Polychlorinated Biphenyls - chemistry Polycyclic Aromatic Hydrocarbons - analysis Polycyclic Aromatic Hydrocarbons - chemistry Solvents Studies Toxicity Waste Water Technology Water Management Water Pollution Control |
| title | Polychlorinated biphenyl contamination of paints containing polycyclic- and Naphthol AS-type pigments |
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