Localized plasmons in graphene-coated nanospheres

We present an analytical derivation of the electromagnetic response of a spherical object coated by a conductive film, here exemplified by a graphene coating. Applying the framework of Mie-Lorenz theory augmented to account for a conductive boundary condition, we derive the multipole scattering coef...

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Veröffentlicht in:Physical review. B, Condensed matter and materials physics Condensed matter and materials physics, 2015-03, Vol.91 (12), Article 125414
Hauptverfasser: Christensen, Thomas, Jauho, Antti-Pekka, Wubs, Martijn, Mortensen, N. Asger
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container_title Physical review. B, Condensed matter and materials physics
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creator Christensen, Thomas
Jauho, Antti-Pekka
Wubs, Martijn
Mortensen, N. Asger
description We present an analytical derivation of the electromagnetic response of a spherical object coated by a conductive film, here exemplified by a graphene coating. Applying the framework of Mie-Lorenz theory augmented to account for a conductive boundary condition, we derive the multipole scattering coefficients, modified essentially through the inclusion of an additive correction in numerator and denominator. By reductionist means, starting from the retarded response, we offer simple results in the quasistatic regime by analyzing the multipolar polarizability and associated dispersion equation for the localized plasmons. We consider graphene coatings of both dielectric and conducting spheres, where the graphene coating in the former case introduces the plasmons and in the latter case modifies in interesting ways the existing ones. Finally, we discuss our analytical results in the context of extinction cross section and local density of states. Recent demonstrations of fabricated spherical graphene nanostructures make our study directly relevant to experiments.
doi_str_mv 10.1103/PhysRevB.91.125414
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subjects Coating
Condensed matter
Dispersions
Graphene
Inclusions
Mathematical analysis
Nanostructure
Plasmons
title Localized plasmons in graphene-coated nanospheres
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