Sources and ecological risk assessment of PAHs in surface sediments from Bohai Sea and northern part of the Yellow Sea, China

•Coal combustion, vehicle emission and coke oven are key PAH sources in BS and NPYS.•Combined biological toxicity of PAHs is lower than that of the individual PAHs.•TEQcarcs suggest potentially low carcinogenicity of PAHs exposure in BS and NPYS. Sources and ecological risk of sixteen priority PAHs...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Marine pollution bulletin 2015-07, Vol.96 (1-2), p.485-490
Hauptverfasser: Li, Jiafu, Dong, Han, Zhang, Dahai, Han, Bin, Zhu, Chenjian, Liu, Shaopeng, Liu, Xiangmin, Ma, Qianyao, Li, Xianguo
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page 490
container_issue 1-2
container_start_page 485
container_title Marine pollution bulletin
container_volume 96
creator Li, Jiafu
Dong, Han
Zhang, Dahai
Han, Bin
Zhu, Chenjian
Liu, Shaopeng
Liu, Xiangmin
Ma, Qianyao
Li, Xianguo
description •Coal combustion, vehicle emission and coke oven are key PAH sources in BS and NPYS.•Combined biological toxicity of PAHs is lower than that of the individual PAHs.•TEQcarcs suggest potentially low carcinogenicity of PAHs exposure in BS and NPYS. Sources and ecological risk of sixteen priority PAHs in surface sediments from Bohai Sea (BS) and northern part of the Yellow Sea (NPYS) were investigated. The total concentrations of PAHs varied in ranges 149.24–1211.81 and 148.28–907.47ng/g for BS and NPYS, respectively. Principal component analysis-multiple linear regression (PCA–MLR) suggested that coal combustion, vehicular emission and coke oven could be the primary PAH contributors, accounting for 56.6%, 29.2% and 14.2% of PAH concentrations, respectively. Analysis with sediment quality guidelines (SQGs) indicated that acenaphthylene, fluorene, phenanthrene, fluoranthene, pyrene and dibenzo(a,h)anthracene may occasionally cause adverse biological effects in some stations. Organic carbon (OC)-normalized analysis and mean effects range-median quotient (M-ERM-Q) suggested that the combined ecological risk of PAHs was generally low. The toxic equivalent concentrations of carcinogenic PAHs were 12.87–64.6ng/g-BaPeq and 5.95–68.80ng/g-BaPeq in BS and NPYS, respectively, suggesting low carcinogenic risk for both BS and NPYS.
doi_str_mv 10.1016/j.marpolbul.2015.05.002
format Article
fullrecord <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_1701484472</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><els_id>S0025326X15002593</els_id><sourcerecordid>1701484472</sourcerecordid><originalsourceid>FETCH-LOGICAL-a497t-93397c50f25aedc80e2c0e071e1dfb2303e6f9b7e32110b765131025b4deefe43</originalsourceid><addsrcrecordid>eNqFkMFu1DAQhi0EotvCK4CPHMgytpN4c1xWhSJVAqkgwclynDHrJYkXTwLiwLvX6ZZekUYazfj_ZzwfYy8FrAWI-s1hPdh0jH0792sJolpDDpCP2EpsdFMoVavHbJU7VaFk_fWMnRMdAEBLLZ6yM1k1NUhdrtjfmzgnh8Tt2HF0sY_fg7M9T4F-cEuERAOOE4-ef9peEQ8jpzl565ATdmF5I-5THPjbuLeB36C9GzXGNO0xjfxo0507V_wb9n38vWhe890-jPYZe-JtT_j8Pl-wL-8uP--uiuuP7z_stteFLRs9FY1SjXYVeFlZ7NwGUDpA0AJF51upQGHtm1ajkkJAq-tKKJFvb8sO0WOpLtir09xjij9npMkMgVz-jR0xzmSEBlFuylLLLNUnqUuRKKE3xxQy7D9GgFnYm4N5YG8W9gZywOJ8cb9kbgfsHnz_YGfB9iTAfOqvgMmQCzi6zDGhm0wXw3-X3AIGCZpz</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>1701484472</pqid></control><display><type>article</type><title>Sources and ecological risk assessment of PAHs in surface sediments from Bohai Sea and northern part of the Yellow Sea, China</title><source>MEDLINE</source><source>Elsevier ScienceDirect Journals Complete</source><creator>Li, Jiafu ; Dong, Han ; Zhang, Dahai ; Han, Bin ; Zhu, Chenjian ; Liu, Shaopeng ; Liu, Xiangmin ; Ma, Qianyao ; Li, Xianguo</creator><creatorcontrib>Li, Jiafu ; Dong, Han ; Zhang, Dahai ; Han, Bin ; Zhu, Chenjian ; Liu, Shaopeng ; Liu, Xiangmin ; Ma, Qianyao ; Li, Xianguo</creatorcontrib><description>•Coal combustion, vehicle emission and coke oven are key PAH sources in BS and NPYS.•Combined biological toxicity of PAHs is lower than that of the individual PAHs.•TEQcarcs suggest potentially low carcinogenicity of PAHs exposure in BS and NPYS. Sources and ecological risk of sixteen priority PAHs in surface sediments from Bohai Sea (BS) and northern part of the Yellow Sea (NPYS) were investigated. The total concentrations of PAHs varied in ranges 149.24–1211.81 and 148.28–907.47ng/g for BS and NPYS, respectively. Principal component analysis-multiple linear regression (PCA–MLR) suggested that coal combustion, vehicular emission and coke oven could be the primary PAH contributors, accounting for 56.6%, 29.2% and 14.2% of PAH concentrations, respectively. Analysis with sediment quality guidelines (SQGs) indicated that acenaphthylene, fluorene, phenanthrene, fluoranthene, pyrene and dibenzo(a,h)anthracene may occasionally cause adverse biological effects in some stations. Organic carbon (OC)-normalized analysis and mean effects range-median quotient (M-ERM-Q) suggested that the combined ecological risk of PAHs was generally low. The toxic equivalent concentrations of carcinogenic PAHs were 12.87–64.6ng/g-BaPeq and 5.95–68.80ng/g-BaPeq in BS and NPYS, respectively, suggesting low carcinogenic risk for both BS and NPYS.</description><identifier>ISSN: 0025-326X</identifier><identifier>EISSN: 1879-3363</identifier><identifier>DOI: 10.1016/j.marpolbul.2015.05.002</identifier><identifier>PMID: 25960274</identifier><language>eng</language><publisher>England: Elsevier Ltd</publisher><subject>China ; Coal ; Ecology ; Environmental Monitoring ; Fluorenes - analysis ; Gas Chromatography-Mass Spectrometry ; Geologic Sediments - chemistry ; Linear Models ; Marine ; Phenanthrenes - analysis ; Polycyclic aromatic hydrocarbons (PAHs) ; Polycyclic Aromatic Hydrocarbons - analysis ; Polycyclic Aromatic Hydrocarbons - toxicity ; Pyrenes - analysis ; Risk Assessment ; Sediment ; Source ; Toxic equivalent quantity (TEQ) ; Vehicle Emissions ; Water Pollutants, Chemical - analysis</subject><ispartof>Marine pollution bulletin, 2015-07, Vol.96 (1-2), p.485-490</ispartof><rights>2015 Elsevier Ltd</rights><rights>Copyright © 2015 Elsevier Ltd. All rights reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a497t-93397c50f25aedc80e2c0e071e1dfb2303e6f9b7e32110b765131025b4deefe43</citedby><cites>FETCH-LOGICAL-a497t-93397c50f25aedc80e2c0e071e1dfb2303e6f9b7e32110b765131025b4deefe43</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.marpolbul.2015.05.002$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,780,784,3550,27924,27925,45995</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/25960274$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Li, Jiafu</creatorcontrib><creatorcontrib>Dong, Han</creatorcontrib><creatorcontrib>Zhang, Dahai</creatorcontrib><creatorcontrib>Han, Bin</creatorcontrib><creatorcontrib>Zhu, Chenjian</creatorcontrib><creatorcontrib>Liu, Shaopeng</creatorcontrib><creatorcontrib>Liu, Xiangmin</creatorcontrib><creatorcontrib>Ma, Qianyao</creatorcontrib><creatorcontrib>Li, Xianguo</creatorcontrib><title>Sources and ecological risk assessment of PAHs in surface sediments from Bohai Sea and northern part of the Yellow Sea, China</title><title>Marine pollution bulletin</title><addtitle>Mar Pollut Bull</addtitle><description>•Coal combustion, vehicle emission and coke oven are key PAH sources in BS and NPYS.•Combined biological toxicity of PAHs is lower than that of the individual PAHs.•TEQcarcs suggest potentially low carcinogenicity of PAHs exposure in BS and NPYS. Sources and ecological risk of sixteen priority PAHs in surface sediments from Bohai Sea (BS) and northern part of the Yellow Sea (NPYS) were investigated. The total concentrations of PAHs varied in ranges 149.24–1211.81 and 148.28–907.47ng/g for BS and NPYS, respectively. Principal component analysis-multiple linear regression (PCA–MLR) suggested that coal combustion, vehicular emission and coke oven could be the primary PAH contributors, accounting for 56.6%, 29.2% and 14.2% of PAH concentrations, respectively. Analysis with sediment quality guidelines (SQGs) indicated that acenaphthylene, fluorene, phenanthrene, fluoranthene, pyrene and dibenzo(a,h)anthracene may occasionally cause adverse biological effects in some stations. Organic carbon (OC)-normalized analysis and mean effects range-median quotient (M-ERM-Q) suggested that the combined ecological risk of PAHs was generally low. The toxic equivalent concentrations of carcinogenic PAHs were 12.87–64.6ng/g-BaPeq and 5.95–68.80ng/g-BaPeq in BS and NPYS, respectively, suggesting low carcinogenic risk for both BS and NPYS.</description><subject>China</subject><subject>Coal</subject><subject>Ecology</subject><subject>Environmental Monitoring</subject><subject>Fluorenes - analysis</subject><subject>Gas Chromatography-Mass Spectrometry</subject><subject>Geologic Sediments - chemistry</subject><subject>Linear Models</subject><subject>Marine</subject><subject>Phenanthrenes - analysis</subject><subject>Polycyclic aromatic hydrocarbons (PAHs)</subject><subject>Polycyclic Aromatic Hydrocarbons - analysis</subject><subject>Polycyclic Aromatic Hydrocarbons - toxicity</subject><subject>Pyrenes - analysis</subject><subject>Risk Assessment</subject><subject>Sediment</subject><subject>Source</subject><subject>Toxic equivalent quantity (TEQ)</subject><subject>Vehicle Emissions</subject><subject>Water Pollutants, Chemical - analysis</subject><issn>0025-326X</issn><issn>1879-3363</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2015</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqFkMFu1DAQhi0EotvCK4CPHMgytpN4c1xWhSJVAqkgwclynDHrJYkXTwLiwLvX6ZZekUYazfj_ZzwfYy8FrAWI-s1hPdh0jH0792sJolpDDpCP2EpsdFMoVavHbJU7VaFk_fWMnRMdAEBLLZ6yM1k1NUhdrtjfmzgnh8Tt2HF0sY_fg7M9T4F-cEuERAOOE4-ef9peEQ8jpzl565ATdmF5I-5THPjbuLeB36C9GzXGNO0xjfxo0507V_wb9n38vWhe890-jPYZe-JtT_j8Pl-wL-8uP--uiuuP7z_stteFLRs9FY1SjXYVeFlZ7NwGUDpA0AJF51upQGHtm1ajkkJAq-tKKJFvb8sO0WOpLtir09xjij9npMkMgVz-jR0xzmSEBlFuylLLLNUnqUuRKKE3xxQy7D9GgFnYm4N5YG8W9gZywOJ8cb9kbgfsHnz_YGfB9iTAfOqvgMmQCzi6zDGhm0wXw3-X3AIGCZpz</recordid><startdate>20150715</startdate><enddate>20150715</enddate><creator>Li, Jiafu</creator><creator>Dong, Han</creator><creator>Zhang, Dahai</creator><creator>Han, Bin</creator><creator>Zhu, Chenjian</creator><creator>Liu, Shaopeng</creator><creator>Liu, Xiangmin</creator><creator>Ma, Qianyao</creator><creator>Li, Xianguo</creator><general>Elsevier Ltd</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7ST</scope><scope>7TN</scope><scope>7TV</scope><scope>7U1</scope><scope>7U2</scope><scope>7U7</scope><scope>7UA</scope><scope>C1K</scope><scope>F1W</scope><scope>H97</scope><scope>L.G</scope><scope>SOI</scope></search><sort><creationdate>20150715</creationdate><title>Sources and ecological risk assessment of PAHs in surface sediments from Bohai Sea and northern part of the Yellow Sea, China</title><author>Li, Jiafu ; Dong, Han ; Zhang, Dahai ; Han, Bin ; Zhu, Chenjian ; Liu, Shaopeng ; Liu, Xiangmin ; Ma, Qianyao ; Li, Xianguo</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a497t-93397c50f25aedc80e2c0e071e1dfb2303e6f9b7e32110b765131025b4deefe43</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2015</creationdate><topic>China</topic><topic>Coal</topic><topic>Ecology</topic><topic>Environmental Monitoring</topic><topic>Fluorenes - analysis</topic><topic>Gas Chromatography-Mass Spectrometry</topic><topic>Geologic Sediments - chemistry</topic><topic>Linear Models</topic><topic>Marine</topic><topic>Phenanthrenes - analysis</topic><topic>Polycyclic aromatic hydrocarbons (PAHs)</topic><topic>Polycyclic Aromatic Hydrocarbons - analysis</topic><topic>Polycyclic Aromatic Hydrocarbons - toxicity</topic><topic>Pyrenes - analysis</topic><topic>Risk Assessment</topic><topic>Sediment</topic><topic>Source</topic><topic>Toxic equivalent quantity (TEQ)</topic><topic>Vehicle Emissions</topic><topic>Water Pollutants, Chemical - analysis</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Li, Jiafu</creatorcontrib><creatorcontrib>Dong, Han</creatorcontrib><creatorcontrib>Zhang, Dahai</creatorcontrib><creatorcontrib>Han, Bin</creatorcontrib><creatorcontrib>Zhu, Chenjian</creatorcontrib><creatorcontrib>Liu, Shaopeng</creatorcontrib><creatorcontrib>Liu, Xiangmin</creatorcontrib><creatorcontrib>Ma, Qianyao</creatorcontrib><creatorcontrib>Li, Xianguo</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>Environment Abstracts</collection><collection>Oceanic Abstracts</collection><collection>Pollution Abstracts</collection><collection>Risk Abstracts</collection><collection>Safety Science and Risk</collection><collection>Toxicology Abstracts</collection><collection>Water Resources Abstracts</collection><collection>Environmental Sciences and Pollution Management</collection><collection>ASFA: Aquatic Sciences and Fisheries Abstracts</collection><collection>Aquatic Science &amp; Fisheries Abstracts (ASFA) 3: Aquatic Pollution &amp; Environmental Quality</collection><collection>Aquatic Science &amp; Fisheries Abstracts (ASFA) Professional</collection><collection>Environment Abstracts</collection><jtitle>Marine pollution bulletin</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Li, Jiafu</au><au>Dong, Han</au><au>Zhang, Dahai</au><au>Han, Bin</au><au>Zhu, Chenjian</au><au>Liu, Shaopeng</au><au>Liu, Xiangmin</au><au>Ma, Qianyao</au><au>Li, Xianguo</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Sources and ecological risk assessment of PAHs in surface sediments from Bohai Sea and northern part of the Yellow Sea, China</atitle><jtitle>Marine pollution bulletin</jtitle><addtitle>Mar Pollut Bull</addtitle><date>2015-07-15</date><risdate>2015</risdate><volume>96</volume><issue>1-2</issue><spage>485</spage><epage>490</epage><pages>485-490</pages><issn>0025-326X</issn><eissn>1879-3363</eissn><abstract>•Coal combustion, vehicle emission and coke oven are key PAH sources in BS and NPYS.•Combined biological toxicity of PAHs is lower than that of the individual PAHs.•TEQcarcs suggest potentially low carcinogenicity of PAHs exposure in BS and NPYS. Sources and ecological risk of sixteen priority PAHs in surface sediments from Bohai Sea (BS) and northern part of the Yellow Sea (NPYS) were investigated. The total concentrations of PAHs varied in ranges 149.24–1211.81 and 148.28–907.47ng/g for BS and NPYS, respectively. Principal component analysis-multiple linear regression (PCA–MLR) suggested that coal combustion, vehicular emission and coke oven could be the primary PAH contributors, accounting for 56.6%, 29.2% and 14.2% of PAH concentrations, respectively. Analysis with sediment quality guidelines (SQGs) indicated that acenaphthylene, fluorene, phenanthrene, fluoranthene, pyrene and dibenzo(a,h)anthracene may occasionally cause adverse biological effects in some stations. Organic carbon (OC)-normalized analysis and mean effects range-median quotient (M-ERM-Q) suggested that the combined ecological risk of PAHs was generally low. The toxic equivalent concentrations of carcinogenic PAHs were 12.87–64.6ng/g-BaPeq and 5.95–68.80ng/g-BaPeq in BS and NPYS, respectively, suggesting low carcinogenic risk for both BS and NPYS.</abstract><cop>England</cop><pub>Elsevier Ltd</pub><pmid>25960274</pmid><doi>10.1016/j.marpolbul.2015.05.002</doi><tpages>6</tpages></addata></record>
fulltext fulltext
identifier ISSN: 0025-326X
ispartof Marine pollution bulletin, 2015-07, Vol.96 (1-2), p.485-490
issn 0025-326X
1879-3363
language eng
recordid cdi_proquest_miscellaneous_1701484472
source MEDLINE; Elsevier ScienceDirect Journals Complete
subjects China
Coal
Ecology
Environmental Monitoring
Fluorenes - analysis
Gas Chromatography-Mass Spectrometry
Geologic Sediments - chemistry
Linear Models
Marine
Phenanthrenes - analysis
Polycyclic aromatic hydrocarbons (PAHs)
Polycyclic Aromatic Hydrocarbons - analysis
Polycyclic Aromatic Hydrocarbons - toxicity
Pyrenes - analysis
Risk Assessment
Sediment
Source
Toxic equivalent quantity (TEQ)
Vehicle Emissions
Water Pollutants, Chemical - analysis
title Sources and ecological risk assessment of PAHs in surface sediments from Bohai Sea and northern part of the Yellow Sea, China
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2024-12-27T08%3A12%3A36IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Sources%20and%20ecological%20risk%20assessment%20of%20PAHs%20in%20surface%20sediments%20from%20Bohai%20Sea%20and%20northern%20part%20of%20the%20Yellow%20Sea,%20China&rft.jtitle=Marine%20pollution%20bulletin&rft.au=Li,%20Jiafu&rft.date=2015-07-15&rft.volume=96&rft.issue=1-2&rft.spage=485&rft.epage=490&rft.pages=485-490&rft.issn=0025-326X&rft.eissn=1879-3363&rft_id=info:doi/10.1016/j.marpolbul.2015.05.002&rft_dat=%3Cproquest_cross%3E1701484472%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=1701484472&rft_id=info:pmid/25960274&rft_els_id=S0025326X15002593&rfr_iscdi=true