Light alkane oxidation using catalysts prepared by chemical vapour impregnation: tuning alcohol selectivity through catalyst pre-treatment

Fe/ZSM-5(30) catalysts have been prepared by chemical vapour impregnation (CVI) using iron(iii) acetylacetonate as the precursor. These materials have been used for the oxidation of methane and ethane using aqueous hydrogen peroxide as oxidant. Heating in air leads to materials that exhibit high cat...

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Veröffentlicht in:	Chemical science (Cambridge) 2014-07, Vol.5 (9), p.3603-3616
Hauptverfasser:	de, Michael M, Armstrong, Robert D, McVicker, Rebecca, Wells, Peter P, Dimitratos, Nikolaos, He, Qian, Lu, Li, Jenkins, Robert L, Hammond, Ceri, Lopez-Sanchez, Jose Antonio, Kiely, Christopher J, Hutchings, Graham J
Format:	Artikel
Sprache:	eng
Schlagworte:	Catalysis Catalysts Ethane Heat treatment Iron Methane Oxidation Selectivity
Online-Zugang:	Volltext
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