Intrinsic and extrinsic absorption of chemical vapor deposition single-crystal diamond from the middle ultraviolet to the far infrared

Optical absorption is reported in high-quality single-crystal Type IIa diamonds grown by microwave-assisted chemical vapor deposition. Laser calorimetry and spectrophotometry were used at wavelengths from the ultraviolet to the infrared. There is minimal evidence of extrinsic absorption on or near t...

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Veröffentlicht in:Journal of the Optical Society of America. B, Optical physics Optical physics, 2015-03, Vol.32 (3), p.479-484
Hauptverfasser: Webster, Scott, Chen, Ying, Turri, Giorgio, Bennett, Andrew, Wickham, Benjamin, Bass, Michael
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container_end_page 484
container_issue 3
container_start_page 479
container_title Journal of the Optical Society of America. B, Optical physics
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creator Webster, Scott
Chen, Ying
Turri, Giorgio
Bennett, Andrew
Wickham, Benjamin
Bass, Michael
description Optical absorption is reported in high-quality single-crystal Type IIa diamonds grown by microwave-assisted chemical vapor deposition. Laser calorimetry and spectrophotometry were used at wavelengths from the ultraviolet to the infrared. There is minimal evidence of extrinsic absorption on or near the short wavelength side of the middle-ultraviolet (MUV) region (200-300 nm) or in the infrared absorption bands. At the long wavelength side of the MUV and extending into the visible, extrinsic absorption dominates, which is related to the amount of nitrogen and nitrogen-related lattice defects in diamond. In the samples studied nitrogen concentrations were between 10 and 40 ppb. At 10.6 mu m, the measured absorption coefficient of a representative sample is comparable with, or less than, those of the highest quality samples previously reported. Evidence is presented showing that our measurements serve as upper bounds on the absorption coefficients and call into question previous calorimetric reports of intrinsic absorption in the visible, near infrared, and at 10.6 mu m.
doi_str_mv 10.1364/JOSAB.32.000479
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subjects Absorption coefficient
Bands
Calorimetry
Chemical vapor deposition
Diamonds
Infrared
Single crystals
Ultraviolet
Wavelengths
title Intrinsic and extrinsic absorption of chemical vapor deposition single-crystal diamond from the middle ultraviolet to the far infrared
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