Effect of sample pretreatment on the fractionation of arsenic in anoxic soils
Using by sequential extraction procedures to obtain the chemical forms of arsenic in soils can provide useful information for the assessment of arsenic mobility and bioavailability in soils. However, sample pretreatments before the extraction probably have some effects on the fractionation of arseni...
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description | Using by sequential extraction procedures to obtain the chemical forms of arsenic in soils can provide useful information for the assessment of arsenic mobility and bioavailability in soils. However, sample pretreatments before the extraction probably have some effects on the fractionation of arsenic in soils. Impact of sample pretreatments (freeze-drying, oven-drying, air-drying, and the fresh soil) on the fractionation of arsenic in anoxic soils was investigated in this study. The results show that there are some differences for arsenic fractions in soils between by drying pretreatments and by the fresh soil, indicating that the redistribution among arsenic fractions in anoxic soils occurs after drying pretreatments. The redistribution of arsenic fractions in anoxic soils is ascribed to the oxidation of organic matter and sulfides, the crystallization of iron (hydr)oxides, the ageing process, and the diffusion of arsenic into micropores. The freeze-drying is the best drying method to minimize the effect on the fractionation of arsenic in anoxic soils, while air-drying is the worst one. Drying pretreatments are not recommended for the fractionation of arsenic in anoxic soils with high concentration of iron. |
doi_str_mv | 10.1007/s11356-014-3958-5 |
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However, sample pretreatments before the extraction probably have some effects on the fractionation of arsenic in soils. Impact of sample pretreatments (freeze-drying, oven-drying, air-drying, and the fresh soil) on the fractionation of arsenic in anoxic soils was investigated in this study. The results show that there are some differences for arsenic fractions in soils between by drying pretreatments and by the fresh soil, indicating that the redistribution among arsenic fractions in anoxic soils occurs after drying pretreatments. The redistribution of arsenic fractions in anoxic soils is ascribed to the oxidation of organic matter and sulfides, the crystallization of iron (hydr)oxides, the ageing process, and the diffusion of arsenic into micropores. The freeze-drying is the best drying method to minimize the effect on the fractionation of arsenic in anoxic soils, while air-drying is the worst one. Drying pretreatments are not recommended for the fractionation of arsenic in anoxic soils with high concentration of iron.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-014-3958-5</identifier><identifier>PMID: 25537285</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Aquatic Pollution ; Arsenic ; Arsenic - analysis ; Arsenic - chemistry ; Arsenic removal ; Atmospheric Protection/Air Quality Control/Air Pollution ; Bioavailability ; Chemical Fractionation ; Crystallization ; Desiccation - methods ; Earth and Environmental Science ; Ecotoxicology ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental impact ; Environmental science ; Extraction processes ; Fractionation ; Freeze drying ; Iron - chemistry ; Methods ; Organic matter ; Oxides - chemistry ; Research Article ; Sediments ; Soil contamination ; Soil Pollutants - analysis ; Soil Pollutants - chemistry ; Soils ; Studies ; Waste Water Technology ; Water Management ; Water Pollution Control</subject><ispartof>Environmental science and pollution research international, 2015-06, Vol.22 (11), p.8367-8374</ispartof><rights>Springer-Verlag Berlin Heidelberg 2014</rights><rights>Springer-Verlag Berlin Heidelberg 2015</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c549t-e0db63361d52da6e5179eaad4f9d8237a66816e095cc64fda7c1f8333180bb823</citedby><cites>FETCH-LOGICAL-c549t-e0db63361d52da6e5179eaad4f9d8237a66816e095cc64fda7c1f8333180bb823</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-014-3958-5$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-014-3958-5$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/25537285$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Huang, Guanxing</creatorcontrib><creatorcontrib>Chen, Zongyu</creatorcontrib><creatorcontrib>Sun, Jichao</creatorcontrib><creatorcontrib>Liu, Fan</creatorcontrib><creatorcontrib>Wang, Jia</creatorcontrib><creatorcontrib>Zhang, Ying</creatorcontrib><title>Effect of sample pretreatment on the fractionation of arsenic in anoxic soils</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>Using by sequential extraction procedures to obtain the chemical forms of arsenic in soils can provide useful information for the assessment of arsenic mobility and bioavailability in soils. However, sample pretreatments before the extraction probably have some effects on the fractionation of arsenic in soils. Impact of sample pretreatments (freeze-drying, oven-drying, air-drying, and the fresh soil) on the fractionation of arsenic in anoxic soils was investigated in this study. The results show that there are some differences for arsenic fractions in soils between by drying pretreatments and by the fresh soil, indicating that the redistribution among arsenic fractions in anoxic soils occurs after drying pretreatments. The redistribution of arsenic fractions in anoxic soils is ascribed to the oxidation of organic matter and sulfides, the crystallization of iron (hydr)oxides, the ageing process, and the diffusion of arsenic into micropores. The freeze-drying is the best drying method to minimize the effect on the fractionation of arsenic in anoxic soils, while air-drying is the worst one. Drying pretreatments are not recommended for the fractionation of arsenic in anoxic soils with high concentration of iron.</description><subject>Aquatic Pollution</subject><subject>Arsenic</subject><subject>Arsenic - analysis</subject><subject>Arsenic - chemistry</subject><subject>Arsenic removal</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Bioavailability</subject><subject>Chemical Fractionation</subject><subject>Crystallization</subject><subject>Desiccation - methods</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental impact</subject><subject>Environmental science</subject><subject>Extraction processes</subject><subject>Fractionation</subject><subject>Freeze drying</subject><subject>Iron - chemistry</subject><subject>Methods</subject><subject>Organic matter</subject><subject>Oxides - chemistry</subject><subject>Research Article</subject><subject>Sediments</subject><subject>Soil contamination</subject><subject>Soil Pollutants - analysis</subject><subject>Soil Pollutants - chemistry</subject><subject>Soils</subject><subject>Studies</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water Pollution Control</subject><issn>0944-1344</issn><issn>1614-7499</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2015</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNp1kMtKxDAUhoMozjj6AG6k4MZNNWluzVKG8QIjbnQd0vREO7RpTTqgb2_KqIjgJic5-c6f8CF0SvAlwVheRUIoFzkmLKeKlznfQ3Mi0kkypfbRHCvGckIZm6GjGDcYF1gV8hDNCs6pLEo-Rw8r58COWe-yaLqhhWwIMAYwYwc-tX02vkLmgrFj03szLRNrQgTf2KzxmfH9e9rFvmnjMTpwpo1w8lUX6Plm9bS8y9ePt_fL63VuOVNjDriuBKWC1LyojQBOpAJjauZUXRZUGiFKIgArbq1grjbSEldSSkmJqyoRC3Sxyx1C_7aFOOquiRba1njot1ETUVIsS6ZkQs__oJt-G3z63UQVXHKakheI7Cgb-hgDOD2EpjPhQxOsJ9d651on13pyrXmaOftK3lYd1D8T33ITUOyAmK78C4RfT_-b-gn2moi-</recordid><startdate>20150601</startdate><enddate>20150601</enddate><creator>Huang, Guanxing</creator><creator>Chen, Zongyu</creator><creator>Sun, Jichao</creator><creator>Liu, Fan</creator><creator>Wang, Jia</creator><creator>Zhang, Ying</creator><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7QL</scope><scope>7SN</scope><scope>7T7</scope><scope>7TV</scope><scope>7U7</scope><scope>7WY</scope><scope>7WZ</scope><scope>7X7</scope><scope>7XB</scope><scope>87Z</scope><scope>88E</scope><scope>88I</scope><scope>8AO</scope><scope>8C1</scope><scope>8FD</scope><scope>8FI</scope><scope>8FJ</scope><scope>8FK</scope><scope>8FL</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>ATCPS</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BEZIV</scope><scope>BHPHI</scope><scope>C1K</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>FR3</scope><scope>FRNLG</scope><scope>FYUFA</scope><scope>F~G</scope><scope>GHDGH</scope><scope>GNUQQ</scope><scope>HCIFZ</scope><scope>K60</scope><scope>K6~</scope><scope>K9.</scope><scope>L.-</scope><scope>M0C</scope><scope>M0S</scope><scope>M1P</scope><scope>M2P</scope><scope>M7N</scope><scope>P64</scope><scope>PATMY</scope><scope>PQBIZ</scope><scope>PQBZA</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PYCSY</scope><scope>Q9U</scope><scope>7X8</scope></search><sort><creationdate>20150601</creationdate><title>Effect of sample pretreatment on the fractionation of arsenic in anoxic soils</title><author>Huang, Guanxing ; Chen, Zongyu ; Sun, Jichao ; Liu, Fan ; Wang, Jia ; Zhang, Ying</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c549t-e0db63361d52da6e5179eaad4f9d8237a66816e095cc64fda7c1f8333180bb823</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2015</creationdate><topic>Aquatic Pollution</topic><topic>Arsenic</topic><topic>Arsenic - 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Academic</collection><jtitle>Environmental science and pollution research international</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Huang, Guanxing</au><au>Chen, Zongyu</au><au>Sun, Jichao</au><au>Liu, Fan</au><au>Wang, Jia</au><au>Zhang, Ying</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Effect of sample pretreatment on the fractionation of arsenic in anoxic soils</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2015-06-01</date><risdate>2015</risdate><volume>22</volume><issue>11</issue><spage>8367</spage><epage>8374</epage><pages>8367-8374</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>Using by sequential extraction procedures to obtain the chemical forms of arsenic in soils can provide useful information for the assessment of arsenic mobility and bioavailability in soils. However, sample pretreatments before the extraction probably have some effects on the fractionation of arsenic in soils. Impact of sample pretreatments (freeze-drying, oven-drying, air-drying, and the fresh soil) on the fractionation of arsenic in anoxic soils was investigated in this study. The results show that there are some differences for arsenic fractions in soils between by drying pretreatments and by the fresh soil, indicating that the redistribution among arsenic fractions in anoxic soils occurs after drying pretreatments. The redistribution of arsenic fractions in anoxic soils is ascribed to the oxidation of organic matter and sulfides, the crystallization of iron (hydr)oxides, the ageing process, and the diffusion of arsenic into micropores. The freeze-drying is the best drying method to minimize the effect on the fractionation of arsenic in anoxic soils, while air-drying is the worst one. Drying pretreatments are not recommended for the fractionation of arsenic in anoxic soils with high concentration of iron.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>25537285</pmid><doi>10.1007/s11356-014-3958-5</doi><tpages>8</tpages></addata></record> |
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subjects | Aquatic Pollution Arsenic Arsenic - analysis Arsenic - chemistry Arsenic removal Atmospheric Protection/Air Quality Control/Air Pollution Bioavailability Chemical Fractionation Crystallization Desiccation - methods Earth and Environmental Science Ecotoxicology Environment Environmental Chemistry Environmental Health Environmental impact Environmental science Extraction processes Fractionation Freeze drying Iron - chemistry Methods Organic matter Oxides - chemistry Research Article Sediments Soil contamination Soil Pollutants - analysis Soil Pollutants - chemistry Soils Studies Waste Water Technology Water Management Water Pollution Control |
title | Effect of sample pretreatment on the fractionation of arsenic in anoxic soils |
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