Identifying sources of Pb pollution in urban soils by means of MC-ICP-MS and TOF-SIMS
Lead pollution was evaluated in 17 urban soils from parks and gardens in the city of Vigo (NW Spain). The Pb isotope ratios (²⁰⁷Pb/²⁰⁶Pb,²⁰⁸Pb/²⁰⁴Pb,²⁰⁶Pb/²⁰⁴Pb and²⁰⁸Pb/²⁰⁶Pb) were determined after being measured by MC-ICP-MS. The association of the isotopes (²⁰⁴Pb,²⁰⁶Pb,²⁰⁷Pb and²⁰⁸Pb) with the di...
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| creator | Rodríguez-Seijo, Andrés Arenas-Lago, Daniel Andrade, María Luisa Vega, Flora A |
| description | Lead pollution was evaluated in 17 urban soils from parks and gardens in the city of Vigo (NW Spain). The Pb isotope ratios (²⁰⁷Pb/²⁰⁶Pb,²⁰⁸Pb/²⁰⁴Pb,²⁰⁶Pb/²⁰⁴Pb and²⁰⁸Pb/²⁰⁶Pb) were determined after being measured by MC-ICP-MS. The association of the isotopes (²⁰⁴Pb,²⁰⁶Pb,²⁰⁷Pb and²⁰⁸Pb) with the different components of the soil was studied using TOF-SIMS. The isotopic ranges obtained for the samples were between 1.116 and 1.203 (²⁰⁶Pb/²⁰⁷Pb), 2.044–2.143 (²⁰⁸Pb/²⁰⁶Pb), 37.206–38.608 (²⁰⁸Pb/²⁰⁴Pb), 15.5482–15.6569 (²⁰⁷Pb/²⁰⁴Pb) and 17.357–18.826 (²⁰⁶Pb/²⁰⁴Pb). The application of the three-end-member model indicates that the Pb derived from petrol is the main source of Pb in the soils (43.51 % on average), followed by natural or geogenic Pb (39.12 %) and industrial emissions (17.37 %). The emissions derived from coal combustion do not appear to influence the content of Pb in the soil. TOF-SIMS images show that the Pb mainly interacts with organic matter. This technique contributes to the understanding of the association of anthropogenic Pb with the components of the soil, as well as the particle size of these associations, thus allowing the possible sources of Pb to be identified. |
| doi_str_mv | 10.1007/s11356-014-4027-9 |
| format | Article |
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The Pb isotope ratios (²⁰⁷Pb/²⁰⁶Pb,²⁰⁸Pb/²⁰⁴Pb,²⁰⁶Pb/²⁰⁴Pb and²⁰⁸Pb/²⁰⁶Pb) were determined after being measured by MC-ICP-MS. The association of the isotopes (²⁰⁴Pb,²⁰⁶Pb,²⁰⁷Pb and²⁰⁸Pb) with the different components of the soil was studied using TOF-SIMS. The isotopic ranges obtained for the samples were between 1.116 and 1.203 (²⁰⁶Pb/²⁰⁷Pb), 2.044–2.143 (²⁰⁸Pb/²⁰⁶Pb), 37.206–38.608 (²⁰⁸Pb/²⁰⁴Pb), 15.5482–15.6569 (²⁰⁷Pb/²⁰⁴Pb) and 17.357–18.826 (²⁰⁶Pb/²⁰⁴Pb). The application of the three-end-member model indicates that the Pb derived from petrol is the main source of Pb in the soils (43.51 % on average), followed by natural or geogenic Pb (39.12 %) and industrial emissions (17.37 %). The emissions derived from coal combustion do not appear to influence the content of Pb in the soil. TOF-SIMS images show that the Pb mainly interacts with organic matter. This technique contributes to the understanding of the association of anthropogenic Pb with the components of the soil, as well as the particle size of these associations, thus allowing the possible sources of Pb to be identified.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-014-4027-9</identifier><identifier>PMID: 25583263</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer-Verlag</publisher><subject>Anthropogenic factors ; Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; Coal ; combustion ; Earth and Environmental Science ; Ecosystems ; Ecotoxicology ; Emissions ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental Monitoring - methods ; gardens ; Gasoline ; Industrial emissions ; Isotopes ; Isotopes - analysis ; Lead ; Lead - chemistry ; Mass spectrometry ; Mass Spectrometry - methods ; Organic matter ; Organic soils ; parks ; particle size ; Pollutants ; Pollution ; Ratios ; Research Article ; Scientific imaging ; Sediments ; Sewage sludge ; Soil - chemistry ; Soil Pollutants - chemistry ; Soil sciences ; Soils ; Spain ; Urban areas ; urban soils ; Waste Water Technology ; Water Management ; Water Pollution Control</subject><ispartof>Environmental science and pollution research international, 2015-05, Vol.22 (10), p.7859-7872</ispartof><rights>Springer-Verlag Berlin Heidelberg 2015</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c573t-1d72a3952b1698302615b1d25c47b834dfff8b715f268c71d97c52a63b0992173</citedby><cites>FETCH-LOGICAL-c573t-1d72a3952b1698302615b1d25c47b834dfff8b715f268c71d97c52a63b0992173</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-014-4027-9$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-014-4027-9$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/25583263$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Rodríguez-Seijo, Andrés</creatorcontrib><creatorcontrib>Arenas-Lago, Daniel</creatorcontrib><creatorcontrib>Andrade, María Luisa</creatorcontrib><creatorcontrib>Vega, Flora A</creatorcontrib><title>Identifying sources of Pb pollution in urban soils by means of MC-ICP-MS and TOF-SIMS</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>Lead pollution was evaluated in 17 urban soils from parks and gardens in the city of Vigo (NW Spain). The Pb isotope ratios (²⁰⁷Pb/²⁰⁶Pb,²⁰⁸Pb/²⁰⁴Pb,²⁰⁶Pb/²⁰⁴Pb and²⁰⁸Pb/²⁰⁶Pb) were determined after being measured by MC-ICP-MS. The association of the isotopes (²⁰⁴Pb,²⁰⁶Pb,²⁰⁷Pb and²⁰⁸Pb) with the different components of the soil was studied using TOF-SIMS. The isotopic ranges obtained for the samples were between 1.116 and 1.203 (²⁰⁶Pb/²⁰⁷Pb), 2.044–2.143 (²⁰⁸Pb/²⁰⁶Pb), 37.206–38.608 (²⁰⁸Pb/²⁰⁴Pb), 15.5482–15.6569 (²⁰⁷Pb/²⁰⁴Pb) and 17.357–18.826 (²⁰⁶Pb/²⁰⁴Pb). The application of the three-end-member model indicates that the Pb derived from petrol is the main source of Pb in the soils (43.51 % on average), followed by natural or geogenic Pb (39.12 %) and industrial emissions (17.37 %). The emissions derived from coal combustion do not appear to influence the content of Pb in the soil. TOF-SIMS images show that the Pb mainly interacts with organic matter. This technique contributes to the understanding of the association of anthropogenic Pb with the components of the soil, as well as the particle size of these associations, thus allowing the possible sources of Pb to be identified.</description><subject>Anthropogenic factors</subject><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Coal</subject><subject>combustion</subject><subject>Earth and Environmental Science</subject><subject>Ecosystems</subject><subject>Ecotoxicology</subject><subject>Emissions</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental Monitoring - methods</subject><subject>gardens</subject><subject>Gasoline</subject><subject>Industrial emissions</subject><subject>Isotopes</subject><subject>Isotopes - analysis</subject><subject>Lead</subject><subject>Lead - chemistry</subject><subject>Mass spectrometry</subject><subject>Mass Spectrometry - methods</subject><subject>Organic matter</subject><subject>Organic soils</subject><subject>parks</subject><subject>particle size</subject><subject>Pollutants</subject><subject>Pollution</subject><subject>Ratios</subject><subject>Research Article</subject><subject>Scientific imaging</subject><subject>Sediments</subject><subject>Sewage sludge</subject><subject>Soil - chemistry</subject><subject>Soil Pollutants - chemistry</subject><subject>Soil sciences</subject><subject>Soils</subject><subject>Spain</subject><subject>Urban areas</subject><subject>urban soils</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water Pollution Control</subject><issn>0944-1344</issn><issn>1614-7499</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2015</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNp9kc1uEzEURi0EoqHtA7ABS92wMfj6d7xEEYVIjVopzdqyZ-xoqokn2JlF3h6nUxBiwcqyfL7P18cIvQf6GSjVXwoAl4pQEERQpol5hRag6k4LY16jBTVCEOBCXKB3pTxRyqhh-i26YFI2nCm-QNtVF9Kxj6c-7XAZp9yGgseIHzw-jMMwHfsx4T7hKXuXKtAPBfsT3geXnrn1kqyWD2S9wS51-PH-lmxW680VehPdUML1y3qJtrffHpc_yN3999Xy6x1ppeZHAp1mjhvJPCjTcMoUSA8dk63QvuGiizE2XoOMTDWths7oVjKnuKfGMND8En2aew95_DmFcrT7vrRhGFwK41QsqAaYYlTyit78gz7V16Y6nQXdNNIIrVmlYKbaPJaSQ7SH3O9dPlmg9uzczs5tdW7Pzq2pmQ8vzZPfh-5P4rfkCrAZKPUo7UL-6-r_tH6cQ9GN1u1yX-x2wyjI8y_KCvFfN-SQ5Q</recordid><startdate>20150501</startdate><enddate>20150501</enddate><creator>Rodríguez-Seijo, Andrés</creator><creator>Arenas-Lago, Daniel</creator><creator>Andrade, María Luisa</creator><creator>Vega, Flora A</creator><general>Springer-Verlag</general><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>FBQ</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7QL</scope><scope>7SN</scope><scope>7T7</scope><scope>7TV</scope><scope>7U7</scope><scope>7WY</scope><scope>7WZ</scope><scope>7X7</scope><scope>7XB</scope><scope>87Z</scope><scope>88E</scope><scope>88I</scope><scope>8AO</scope><scope>8C1</scope><scope>8FD</scope><scope>8FI</scope><scope>8FJ</scope><scope>8FK</scope><scope>8FL</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>ATCPS</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BEZIV</scope><scope>BHPHI</scope><scope>C1K</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>FR3</scope><scope>FRNLG</scope><scope>FYUFA</scope><scope>F~G</scope><scope>GHDGH</scope><scope>GNUQQ</scope><scope>HCIFZ</scope><scope>K60</scope><scope>K6~</scope><scope>K9.</scope><scope>L.-</scope><scope>M0C</scope><scope>M0S</scope><scope>M1P</scope><scope>M2P</scope><scope>M7N</scope><scope>P64</scope><scope>PATMY</scope><scope>PQBIZ</scope><scope>PQBZA</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PYCSY</scope><scope>Q9U</scope><scope>7X8</scope></search><sort><creationdate>20150501</creationdate><title>Identifying sources of Pb pollution in urban soils by means of MC-ICP-MS and TOF-SIMS</title><author>Rodríguez-Seijo, Andrés ; Arenas-Lago, Daniel ; Andrade, María Luisa ; Vega, Flora A</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c573t-1d72a3952b1698302615b1d25c47b834dfff8b715f268c71d97c52a63b0992173</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2015</creationdate><topic>Anthropogenic factors</topic><topic>Aquatic Pollution</topic><topic>Atmospheric Protection/Air Quality Control/Air Pollution</topic><topic>Coal</topic><topic>combustion</topic><topic>Earth and Environmental Science</topic><topic>Ecosystems</topic><topic>Ecotoxicology</topic><topic>Emissions</topic><topic>Environment</topic><topic>Environmental Chemistry</topic><topic>Environmental Health</topic><topic>Environmental Monitoring - 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Academic</collection><jtitle>Environmental science and pollution research international</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Rodríguez-Seijo, Andrés</au><au>Arenas-Lago, Daniel</au><au>Andrade, María Luisa</au><au>Vega, Flora A</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Identifying sources of Pb pollution in urban soils by means of MC-ICP-MS and TOF-SIMS</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2015-05-01</date><risdate>2015</risdate><volume>22</volume><issue>10</issue><spage>7859</spage><epage>7872</epage><pages>7859-7872</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>Lead pollution was evaluated in 17 urban soils from parks and gardens in the city of Vigo (NW Spain). The Pb isotope ratios (²⁰⁷Pb/²⁰⁶Pb,²⁰⁸Pb/²⁰⁴Pb,²⁰⁶Pb/²⁰⁴Pb and²⁰⁸Pb/²⁰⁶Pb) were determined after being measured by MC-ICP-MS. The association of the isotopes (²⁰⁴Pb,²⁰⁶Pb,²⁰⁷Pb and²⁰⁸Pb) with the different components of the soil was studied using TOF-SIMS. The isotopic ranges obtained for the samples were between 1.116 and 1.203 (²⁰⁶Pb/²⁰⁷Pb), 2.044–2.143 (²⁰⁸Pb/²⁰⁶Pb), 37.206–38.608 (²⁰⁸Pb/²⁰⁴Pb), 15.5482–15.6569 (²⁰⁷Pb/²⁰⁴Pb) and 17.357–18.826 (²⁰⁶Pb/²⁰⁴Pb). The application of the three-end-member model indicates that the Pb derived from petrol is the main source of Pb in the soils (43.51 % on average), followed by natural or geogenic Pb (39.12 %) and industrial emissions (17.37 %). The emissions derived from coal combustion do not appear to influence the content of Pb in the soil. TOF-SIMS images show that the Pb mainly interacts with organic matter. This technique contributes to the understanding of the association of anthropogenic Pb with the components of the soil, as well as the particle size of these associations, thus allowing the possible sources of Pb to be identified.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer-Verlag</pub><pmid>25583263</pmid><doi>10.1007/s11356-014-4027-9</doi><tpages>14</tpages></addata></record> |
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| subjects | Anthropogenic factors Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Coal combustion Earth and Environmental Science Ecosystems Ecotoxicology Emissions Environment Environmental Chemistry Environmental Health Environmental Monitoring - methods gardens Gasoline Industrial emissions Isotopes Isotopes - analysis Lead Lead - chemistry Mass spectrometry Mass Spectrometry - methods Organic matter Organic soils parks particle size Pollutants Pollution Ratios Research Article Scientific imaging Sediments Sewage sludge Soil - chemistry Soil Pollutants - chemistry Soil sciences Soils Spain Urban areas urban soils Waste Water Technology Water Management Water Pollution Control |
| title | Identifying sources of Pb pollution in urban soils by means of MC-ICP-MS and TOF-SIMS |
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