Enhancement of ultracold molecule formation by local control in the nanosecond regime

We describe quantum simulations of ultracold 87Rb2 molecule formation using photoassociation (PA) with nanosecond-time-scale pulses of frequency chirped light. In particular, we compare the case of a linear chirp to one where the frequency evolution is optimized by local control (LC) of the phase, a...

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Veröffentlicht in:New journal of physics 2015-02, Vol.17 (2), p.25008-12
Hauptverfasser: Carini, J L, Kallush, S, Kosloff, R, Gould, P L
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creator Carini, J L
Kallush, S
Kosloff, R
Gould, P L
description We describe quantum simulations of ultracold 87Rb2 molecule formation using photoassociation (PA) with nanosecond-time-scale pulses of frequency chirped light. In particular, we compare the case of a linear chirp to one where the frequency evolution is optimized by local control (LC) of the phase, and find that LC can provide a significant enhancement. The resulting optimal frequency evolution corresponds to a rapid jump from the PA absorption resonance to a downward transition to a bound level of the lowest triplet state. We also consider the case of two frequencies and investigate interference effects. The assumed chirp parameters should be achievable with nanosecond pulse shaping techniques and are predicted to provide a significant enhancement over recent experiments with linear chirps.
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subjects ATOMIC AND MOLECULAR PHYSICS
Atomic energy levels
Chirp
coherent control
Evolution
Formations
Interference
Nanosecond pulses
Nanostructure
Optimization
photoassociation
Physics
quantum control
Simulation
ultracold molecules
title Enhancement of ultracold molecule formation by local control in the nanosecond regime
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