Polybrominated diphenyl ethers (PBDEs) and polychlorinated biphenyls (PCBs) in sediments of Liaohe River: levels, spatial and temporal distribution, possible sources, and inventory

Spatial and seasonal variations of polybrominated diphenyl ethers (PBDEs) and polychlorinated biphenyls (PCBs) in the sediment of Liaohe River were investigated in this study. A total of 29 surface sediment samples were collected in May and September in 2013. Results showed that levels of the two cl...

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Veröffentlicht in:Environmental science and pollution research international 2015-03, Vol.22 (6), p.4256-4264
Hauptverfasser: Lv, Jiapei, Zhang, Yuan, Zhao, Xin, Zhou, Changbo, Guo, Changsheng, Luo, Yi, Meng, Wei, Zou, Guofang, Xu, Jian
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container_title Environmental science and pollution research international
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Zhang, Yuan
Zhao, Xin
Zhou, Changbo
Guo, Changsheng
Luo, Yi
Meng, Wei
Zou, Guofang
Xu, Jian
description Spatial and seasonal variations of polybrominated diphenyl ethers (PBDEs) and polychlorinated biphenyls (PCBs) in the sediment of Liaohe River were investigated in this study. A total of 29 surface sediment samples were collected in May and September in 2013. Results showed that levels of the two classes of compounds were higher in September than in May. The total concentration of PBDEs (∑8PBDEs) ranged from 0.30 to 5.09 ng g⁻¹in May and from 0.17 to 13.73 ng g⁻¹in September, respectively, and BDE 209 was the dominant compound. The total concentration of PCBs (∑33PCBs) was in the range of 4.92–76.86 and 11.69–179.61 ng g⁻¹in May and September, respectively, with tri- and tetra-CBs dominated in the total PCBs in the sediments. According to the congener profiles and the principal component analysis, the major sources of PCBs and PBDEs in sediments of Liaohe River were from the usage of commercial products and industrial activities, and the degradation of high brominated BDEs also contributed to the current PBDEs in the sediments. The mass inventories of PBDEs and PCBs in the sediments of Liaohe River were 1.74 and 21.96 t, respectively, indicating that Liaohe River sediments may act as the potential sources of PBDEs and PCBs to the downstream coastal areas.
doi_str_mv 10.1007/s11356-014-3666-1
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A total of 29 surface sediment samples were collected in May and September in 2013. Results showed that levels of the two classes of compounds were higher in September than in May. The total concentration of PBDEs (∑8PBDEs) ranged from 0.30 to 5.09 ng g⁻¹in May and from 0.17 to 13.73 ng g⁻¹in September, respectively, and BDE 209 was the dominant compound. The total concentration of PCBs (∑33PCBs) was in the range of 4.92–76.86 and 11.69–179.61 ng g⁻¹in May and September, respectively, with tri- and tetra-CBs dominated in the total PCBs in the sediments. According to the congener profiles and the principal component analysis, the major sources of PCBs and PBDEs in sediments of Liaohe River were from the usage of commercial products and industrial activities, and the degradation of high brominated BDEs also contributed to the current PBDEs in the sediments. 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A total of 29 surface sediment samples were collected in May and September in 2013. Results showed that levels of the two classes of compounds were higher in September than in May. The total concentration of PBDEs (∑8PBDEs) ranged from 0.30 to 5.09 ng g⁻¹in May and from 0.17 to 13.73 ng g⁻¹in September, respectively, and BDE 209 was the dominant compound. The total concentration of PCBs (∑33PCBs) was in the range of 4.92–76.86 and 11.69–179.61 ng g⁻¹in May and September, respectively, with tri- and tetra-CBs dominated in the total PCBs in the sediments. According to the congener profiles and the principal component analysis, the major sources of PCBs and PBDEs in sediments of Liaohe River were from the usage of commercial products and industrial activities, and the degradation of high brominated BDEs also contributed to the current PBDEs in the sediments. The mass inventories of PBDEs and PCBs in the sediments of Liaohe River were 1.74 and 21.96 t, respectively, indicating that Liaohe River sediments may act as the potential sources of PBDEs and PCBs to the downstream coastal areas.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer-Verlag</pub><pmid>25292305</pmid><doi>10.1007/s11356-014-3666-1</doi><tpages>9</tpages></addata></record>
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ispartof Environmental science and pollution research international, 2015-03, Vol.22 (6), p.4256-4264
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1614-7499
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source MEDLINE; Springer Nature - Complete Springer Journals
subjects Aquatic Pollution
Atmospheric Protection/Air Quality Control/Air Pollution
Biofilms
Calibration
China
Coastal areas
Coastal zone
coasts
Congeners
Earth and Environmental Science
Ecotoxicology
Environment
Environmental Chemistry
Environmental Health
Environmental Monitoring - methods
Environmental science
Ethers
Fluvial sediments
Freshwater environments
Geologic Sediments - analysis
Halogenated Diphenyl Ethers - chemistry
Industrial areas
Inventories
Laboratories
PCB
Pesticide toxicity
Pesticides
Pollutants
Polybrominated diphenyl ethers
Polychlorinated biphenyls
Polychlorinated Biphenyls - chemistry
principal component analysis
Principal components analysis
Quality control
Quality standards
Research Article
Rivers
Rivers - chemistry
seasonal variation
Seasonal variations
Seasons
Sediment samplers
Sediments
Stockpiling
Sulfuric acid
Temporal distribution
Toxicity
Waste Water Technology
Water Management
Water Pollutants, Chemical - analysis
Water Pollution Control
title Polybrominated diphenyl ethers (PBDEs) and polychlorinated biphenyls (PCBs) in sediments of Liaohe River: levels, spatial and temporal distribution, possible sources, and inventory
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