Effects of Interactions with Cyclic Solvent Molecules on Optical Dephasing of CdSe/ZnS Colloidal Quantum Dots Detected by Femtosecond Four-Wave Mixing Spectroscopy

We have studied the effects of interactions with cyclic solvent molecules on the optical dephasing of CdSe/ZnS colloidal quantum dots (QDs) by femtosecond four-wave mixing spectroscopy. We have found that the interactions with the cyclic solvents without $\pi$-bonds result in unexpectedly long depha...

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Veröffentlicht in:Japanese Journal of Applied Physics 2013-07, Vol.52 (7), p.070202-070202-4
Hauptverfasser: Hirosawa, Yusuke, Kouzai, Hiroyoshi, Yamazaki, Naoya, Miyagawa, Hayato, Tsurumachi, Noriaki, Koshiba, Shun, Nakanishi, Shunsuke, Biju, VasudevanPillai, Ishikawa, Mituru
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container_issue 7
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container_title Japanese Journal of Applied Physics
container_volume 52
creator Hirosawa, Yusuke
Kouzai, Hiroyoshi
Yamazaki, Naoya
Miyagawa, Hayato
Tsurumachi, Noriaki
Koshiba, Shun
Nakanishi, Shunsuke
Biju, VasudevanPillai
Ishikawa, Mituru
description We have studied the effects of interactions with cyclic solvent molecules on the optical dephasing of CdSe/ZnS colloidal quantum dots (QDs) by femtosecond four-wave mixing spectroscopy. We have found that the interactions with the cyclic solvents without $\pi$-bonds result in unexpectedly long dephasing times of QDs even at room temperature, while the interactions with the cyclic solvents including $\pi$-bonds make the optical dephasing of QDs extremely fast with a dephasing time of less than our time resolution.
doi_str_mv 10.7567/JJAP.52.070202
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subjects Cadmium selenides
Colloids
Femtosecond
Four-wave mixing
Quantum dots
Solvents
Spectroscopy
Zinc sulfides
title Effects of Interactions with Cyclic Solvent Molecules on Optical Dephasing of CdSe/ZnS Colloidal Quantum Dots Detected by Femtosecond Four-Wave Mixing Spectroscopy
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