High Performance All-Polymer Solar Cell via Polymer Side-Chain Engineering
An average PCE of 4.2% for all‐polymer solar cells from 20 devices with an average J SC of 8.8 mA cm−2 are obtained with a donor‐acceptor pair despite a low LUMO‐LUMO energy offset of less than 0.1 eV. Incorporation of polystyrene side chains into the donor polymer is found to assist in reducing the...
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| Veröffentlicht in: | Advanced materials (Weinheim) 2014-06, Vol.26 (22), p.3767-3772 |
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| creator | Zhou, Yan Kurosawa, Tadanori Ma, Wei Guo, Yikun Fang, Lei Vandewal, Koen Diao, Ying Wang, Chenggong Yan, Qifan Reinspach, Julia Mei, Jianguo Appleton, Anthony Lucas Koleilat, Ghada I. Gao, Yongli Mannsfeld, Stefan C. B. Salleo, Alberto Ade, Harald Zhao, Dahui Bao, Zhenan |
| description | An average PCE of 4.2% for all‐polymer solar cells from 20 devices with an average J
SC of 8.8 mA cm−2 are obtained with a donor‐acceptor pair despite a low LUMO‐LUMO energy offset of less than 0.1 eV. Incorporation of polystyrene side chains into the donor polymer is found to assist in reducing the phase separation domain length scale, and results in more than 20% enhancement of PCE. We observe a direct correlation between the short circuit current (J
SC) and the length scale of BHJ phase separation, which is obtained by resonance soft X‐ray scattering. |
| doi_str_mv | 10.1002/adma.201306242 |
| format | Article |
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SC of 8.8 mA cm−2 are obtained with a donor‐acceptor pair despite a low LUMO‐LUMO energy offset of less than 0.1 eV. Incorporation of polystyrene side chains into the donor polymer is found to assist in reducing the phase separation domain length scale, and results in more than 20% enhancement of PCE. We observe a direct correlation between the short circuit current (J
SC) and the length scale of BHJ phase separation, which is obtained by resonance soft X‐ray scattering.</description><identifier>ISSN: 0935-9648</identifier><identifier>EISSN: 1521-4095</identifier><identifier>DOI: 10.1002/adma.201306242</identifier><identifier>PMID: 24664632</identifier><language>eng</language><publisher>Germany: Blackwell Publishing Ltd</publisher><subject>all-polymer solar cell ; Correlation ; Devices ; low energy loss ; Phase separation ; Photovoltaic cells ; Polystyrene resins ; resonant soft X-ray scattering (RSoXS) ; Scattering ; Short circuit currents ; side-chain engineering ; Solar cells</subject><ispartof>Advanced materials (Weinheim), 2014-06, Vol.26 (22), p.3767-3772</ispartof><rights>2014 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c4822-6d0b6ee751b5c422e6da34a94d3325389eedf2991b32357292b5b6e3267ff2dd3</citedby><cites>FETCH-LOGICAL-c4822-6d0b6ee751b5c422e6da34a94d3325389eedf2991b32357292b5b6e3267ff2dd3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1002%2Fadma.201306242$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1002%2Fadma.201306242$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>314,776,780,1411,27901,27902,45550,45551</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/24664632$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Zhou, Yan</creatorcontrib><creatorcontrib>Kurosawa, Tadanori</creatorcontrib><creatorcontrib>Ma, Wei</creatorcontrib><creatorcontrib>Guo, Yikun</creatorcontrib><creatorcontrib>Fang, Lei</creatorcontrib><creatorcontrib>Vandewal, Koen</creatorcontrib><creatorcontrib>Diao, Ying</creatorcontrib><creatorcontrib>Wang, Chenggong</creatorcontrib><creatorcontrib>Yan, Qifan</creatorcontrib><creatorcontrib>Reinspach, Julia</creatorcontrib><creatorcontrib>Mei, Jianguo</creatorcontrib><creatorcontrib>Appleton, Anthony Lucas</creatorcontrib><creatorcontrib>Koleilat, Ghada I.</creatorcontrib><creatorcontrib>Gao, Yongli</creatorcontrib><creatorcontrib>Mannsfeld, Stefan C. B.</creatorcontrib><creatorcontrib>Salleo, Alberto</creatorcontrib><creatorcontrib>Ade, Harald</creatorcontrib><creatorcontrib>Zhao, Dahui</creatorcontrib><creatorcontrib>Bao, Zhenan</creatorcontrib><title>High Performance All-Polymer Solar Cell via Polymer Side-Chain Engineering</title><title>Advanced materials (Weinheim)</title><addtitle>Adv. Mater</addtitle><description>An average PCE of 4.2% for all‐polymer solar cells from 20 devices with an average J
SC of 8.8 mA cm−2 are obtained with a donor‐acceptor pair despite a low LUMO‐LUMO energy offset of less than 0.1 eV. Incorporation of polystyrene side chains into the donor polymer is found to assist in reducing the phase separation domain length scale, and results in more than 20% enhancement of PCE. We observe a direct correlation between the short circuit current (J
SC) and the length scale of BHJ phase separation, which is obtained by resonance soft X‐ray scattering.</description><subject>all-polymer solar cell</subject><subject>Correlation</subject><subject>Devices</subject><subject>low energy loss</subject><subject>Phase separation</subject><subject>Photovoltaic cells</subject><subject>Polystyrene resins</subject><subject>resonant soft X-ray scattering (RSoXS)</subject><subject>Scattering</subject><subject>Short circuit currents</subject><subject>side-chain engineering</subject><subject>Solar cells</subject><issn>0935-9648</issn><issn>1521-4095</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2014</creationdate><recordtype>article</recordtype><recordid>eNqFkDlPAzEQhS0EgnC0lGhLmg32-Ni4jBJOcYlDlJZ3PRsMewSbAPn3bBSI6KhGGn3v6ekjZJ_RPqMUjqyrbR8o41SBgDXSYxJYKqiW66RHNZepVmKwRbZjfKGUakXVJtkCoZRQHHrk4sxPnpNbDGUbatsUmAyrKr1tq3mNIblvKxuSEVZV8uFtsnp7h-no2fomOW4mvkEMvpnsko3SVhH3fu4OeTw5fhidpZc3p-ej4WVaiAFAqhzNFWImWS4LAYDKWS6sFo5zkHygEV0JWrOcA5cZaMhlF-CgsrIE5_gOOVz2TkP7NsP4bmofi26jbbCdRcNUxhRIEPJ_VPKFqoHKOrS_RIvQxhiwNNPgaxvmhlGzUG0Wqs1KdRc4-Ome5TW6Ff7rtgP0Evj0Fc7_qTPD8dXwb3m6zPr4jl-rrA2vptuaSfN0fWrux9edlbuxeeDfENqXmA</recordid><startdate>20140611</startdate><enddate>20140611</enddate><creator>Zhou, Yan</creator><creator>Kurosawa, Tadanori</creator><creator>Ma, Wei</creator><creator>Guo, Yikun</creator><creator>Fang, Lei</creator><creator>Vandewal, Koen</creator><creator>Diao, Ying</creator><creator>Wang, Chenggong</creator><creator>Yan, Qifan</creator><creator>Reinspach, Julia</creator><creator>Mei, Jianguo</creator><creator>Appleton, Anthony Lucas</creator><creator>Koleilat, Ghada I.</creator><creator>Gao, Yongli</creator><creator>Mannsfeld, Stefan C. B.</creator><creator>Salleo, Alberto</creator><creator>Ade, Harald</creator><creator>Zhao, Dahui</creator><creator>Bao, Zhenan</creator><general>Blackwell Publishing Ltd</general><scope>BSCLL</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>7SP</scope><scope>7SR</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope></search><sort><creationdate>20140611</creationdate><title>High Performance All-Polymer Solar Cell via Polymer Side-Chain Engineering</title><author>Zhou, Yan ; Kurosawa, Tadanori ; Ma, Wei ; Guo, Yikun ; Fang, Lei ; Vandewal, Koen ; Diao, Ying ; Wang, Chenggong ; Yan, Qifan ; Reinspach, Julia ; Mei, Jianguo ; Appleton, Anthony Lucas ; Koleilat, Ghada I. ; Gao, Yongli ; Mannsfeld, Stefan C. 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| source | Wiley Online Library Journals Frontfile Complete |
| subjects | all-polymer solar cell Correlation Devices low energy loss Phase separation Photovoltaic cells Polystyrene resins resonant soft X-ray scattering (RSoXS) Scattering Short circuit currents side-chain engineering Solar cells |
| title | High Performance All-Polymer Solar Cell via Polymer Side-Chain Engineering |
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