Immobilization and Leaching of Pb and Zn in an Acidic Soil Treated with Zerovalent Iron Nanoparticles (nZVI): Physicochemical and Toxicological Analysis of Leachates
A column experiment was conducted to evaluate the effectiveness of nanoscale zerovalent iron (nZVI) for the in situ immobilization of Pb and Zn in an acidic soil. The impact of nZVI on soil was evaluated by monitoring the physicochemical characteristics of the leachates and their ecotoxicological ef...
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| Veröffentlicht in: | Water, air, and soil pollution air, and soil pollution, 2014-06, Vol.225 (6), p.1-13, Article 1990 |
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| container_title | Water, air, and soil pollution |
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| creator | Gil-Díaz, M Ortiz, L. T Costa, G Alonso, J Rodríguez-Membibre, M. L Sánchez-Fortún, S Pérez-Sanz, A Martín, M Lobo, M. C |
| description | A column experiment was conducted to evaluate the effectiveness of nanoscale zerovalent iron (nZVI) for the in situ immobilization of Pb and Zn in an acidic soil. The impact of nZVI on soil was evaluated by monitoring the physicochemical characteristics of the leachates and their ecotoxicological effects on three species, Vibrio fischeri, Artemia franciscana, and Caenorhabditis elegans. Treatment with nZVI resulted in more effective Pb immobilization in comparison to Zn and reduced the leachability by 98 and 72 %, respectively; the immobilization was stable throughout the experiment. Leachates from nZVI-treated soils showed lower toxicity than leachates from untreated ones. The highest toxicity in treated soils was observed in the first leachate, which presented high values of electrical conductivity due to the leachability of soil ions and those provided by the commercial nanoparticle suspension (Na and Fe). V. fischeri and C. elegans were more sensitive to leachates from nZVI-treated soils polluted with Zn than those from soils polluted with Pb; A. franciscana showed the opposite trend. |
| doi_str_mv | 10.1007/s11270-014-1990-1 |
| format | Article |
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The highest toxicity in treated soils was observed in the first leachate, which presented high values of electrical conductivity due to the leachability of soil ions and those provided by the commercial nanoparticle suspension (Na and Fe). V. fischeri and C. elegans were more sensitive to leachates from nZVI-treated soils polluted with Zn than those from soils polluted with Pb; A. franciscana showed the opposite trend.</description><identifier>ISSN: 0049-6979</identifier><identifier>EISSN: 1573-2932</identifier><identifier>DOI: 10.1007/s11270-014-1990-1</identifier><language>eng</language><publisher>Cham: Springer-Verlag</publisher><subject>Acidic soils ; Analysis ; Artemia franciscana ; Atmospheric Protection/Air Quality Control/Air Pollution ; Bioavailability ; Caenorhabditis elegans ; Chemical elements ; Climate Change/Climate Change Impacts ; Earth and Environmental Science ; Ecological effects ; Ecotoxicology ; Electric properties ; Electrical conductivity ; Environment ; Environmental impact ; Environmental monitoring ; Experiments ; Hydrogeology ; Immobilization ; Iron ; Leachates ; Leaching ; Lead ; Lead (metal) ; Metals ; Microorganisms ; Nanoparticles ; Nanostructure ; Nematodes ; Nitrates ; Pollutants ; polluted soils ; sodium ; Soil (material) ; Soil contaminants ; Soil pollution ; Soil Science & Conservation ; Soil treatment ; Studies ; Toxicity ; Vibrio fischeri ; Water Quality/Water Pollution ; Zinc</subject><ispartof>Water, air, and soil pollution, 2014-06, Vol.225 (6), p.1-13, Article 1990</ispartof><rights>Springer International Publishing Switzerland 2014</rights><rights>COPYRIGHT 2014 Springer</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a468t-68001fc1b33dbe3f24712203a3a4bacc6649a66d22aa55b6f133a140c1e466e83</citedby><cites>FETCH-LOGICAL-a468t-68001fc1b33dbe3f24712203a3a4bacc6649a66d22aa55b6f133a140c1e466e83</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11270-014-1990-1$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11270-014-1990-1$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids></links><search><creatorcontrib>Gil-Díaz, M</creatorcontrib><creatorcontrib>Ortiz, L. 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The impact of nZVI on soil was evaluated by monitoring the physicochemical characteristics of the leachates and their ecotoxicological effects on three species, Vibrio fischeri, Artemia franciscana, and Caenorhabditis elegans. Treatment with nZVI resulted in more effective Pb immobilization in comparison to Zn and reduced the leachability by 98 and 72 %, respectively; the immobilization was stable throughout the experiment. Leachates from nZVI-treated soils showed lower toxicity than leachates from untreated ones. The highest toxicity in treated soils was observed in the first leachate, which presented high values of electrical conductivity due to the leachability of soil ions and those provided by the commercial nanoparticle suspension (Na and Fe). V. fischeri and C. elegans were more sensitive to leachates from nZVI-treated soils polluted with Zn than those from soils polluted with Pb; A. franciscana showed the opposite trend.</description><subject>Acidic soils</subject><subject>Analysis</subject><subject>Artemia franciscana</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Bioavailability</subject><subject>Caenorhabditis elegans</subject><subject>Chemical elements</subject><subject>Climate Change/Climate Change Impacts</subject><subject>Earth and Environmental Science</subject><subject>Ecological effects</subject><subject>Ecotoxicology</subject><subject>Electric properties</subject><subject>Electrical conductivity</subject><subject>Environment</subject><subject>Environmental impact</subject><subject>Environmental monitoring</subject><subject>Experiments</subject><subject>Hydrogeology</subject><subject>Immobilization</subject><subject>Iron</subject><subject>Leachates</subject><subject>Leaching</subject><subject>Lead</subject><subject>Lead (metal)</subject><subject>Metals</subject><subject>Microorganisms</subject><subject>Nanoparticles</subject><subject>Nanostructure</subject><subject>Nematodes</subject><subject>Nitrates</subject><subject>Pollutants</subject><subject>polluted soils</subject><subject>sodium</subject><subject>Soil (material)</subject><subject>Soil contaminants</subject><subject>Soil pollution</subject><subject>Soil Science & Conservation</subject><subject>Soil treatment</subject><subject>Studies</subject><subject>Toxicity</subject><subject>Vibrio fischeri</subject><subject>Water Quality/Water Pollution</subject><subject>Zinc</subject><issn>0049-6979</issn><issn>1573-2932</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2014</creationdate><recordtype>article</recordtype><sourceid>BENPR</sourceid><recordid>eNqFks1u1DAUhSMEEkPhAVhhiU1ZpPgvTsxuVFEYaQSVOmUxG-vGcTKuPPZgZ6DlfXhPnAkLxALshaXj71xfH92ieEnwBcG4fpsIoTUuMeElkRKX5FGxIFXNSioZfVwsMOayFLKWT4tnKd3hvGRTL4qfq_0-tNbZHzDa4BH4Dq0N6J31Awo9um5P0tYjO12ipbad1egmWIc20cBoOvTdjju0NTF8A2f8iFYxF_oEPhwgjlY7k9C5335ZvXmHrncPyeqgd2ZvNbhT7U24z5ILw0lZenCZSdPjp0byE-l58aQHl8yL3-dZcXv1fnP5sVx__rC6XK5L4KIZS9FgTHpNWsa61rCe8ppQihkw4C1oLQSXIERHKUBVtaInjAHhWBPDhTANOyvO57qHGL4eTRrV3iZtnANvwjEpImoicpRN9X-0qrisqBA4o6__Qu_CMeZ_ThSrKy6qRmbqYqaGnKKyvg9jBJ13N2UVvOlt1pes5oI2jNBsILNBx5BSNL06RLuH-KAIVtNQqHkoVB4KNQ2FItlDZ0_KrB9M_KOVf5hezaYegoIh2qRub2gGctp4ap79AnAwwjk</recordid><startdate>20140601</startdate><enddate>20140601</enddate><creator>Gil-Díaz, M</creator><creator>Ortiz, L. 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The impact of nZVI on soil was evaluated by monitoring the physicochemical characteristics of the leachates and their ecotoxicological effects on three species, Vibrio fischeri, Artemia franciscana, and Caenorhabditis elegans. Treatment with nZVI resulted in more effective Pb immobilization in comparison to Zn and reduced the leachability by 98 and 72 %, respectively; the immobilization was stable throughout the experiment. Leachates from nZVI-treated soils showed lower toxicity than leachates from untreated ones. The highest toxicity in treated soils was observed in the first leachate, which presented high values of electrical conductivity due to the leachability of soil ions and those provided by the commercial nanoparticle suspension (Na and Fe). 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| identifier | ISSN: 0049-6979 |
| ispartof | Water, air, and soil pollution, 2014-06, Vol.225 (6), p.1-13, Article 1990 |
| issn | 0049-6979 1573-2932 |
| language | eng |
| recordid | cdi_proquest_miscellaneous_1671600485 |
| source | SpringerLink Journals - AutoHoldings |
| subjects | Acidic soils Analysis Artemia franciscana Atmospheric Protection/Air Quality Control/Air Pollution Bioavailability Caenorhabditis elegans Chemical elements Climate Change/Climate Change Impacts Earth and Environmental Science Ecological effects Ecotoxicology Electric properties Electrical conductivity Environment Environmental impact Environmental monitoring Experiments Hydrogeology Immobilization Iron Leachates Leaching Lead Lead (metal) Metals Microorganisms Nanoparticles Nanostructure Nematodes Nitrates Pollutants polluted soils sodium Soil (material) Soil contaminants Soil pollution Soil Science & Conservation Soil treatment Studies Toxicity Vibrio fischeri Water Quality/Water Pollution Zinc |
| title | Immobilization and Leaching of Pb and Zn in an Acidic Soil Treated with Zerovalent Iron Nanoparticles (nZVI): Physicochemical and Toxicological Analysis of Leachates |
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