Effects of intermediate layer on interfacial resistance for all-solid-state lithium batteries using lithium borohydride
All-solid-state lithium batteries using LiBH4 electrolyte and LiCoO2 cathode were prepared, and the effect of the intermediate layers between LiBH4 and LiCoO2 was demonstrated by electrochemical measurement. Li3PO4, LiNbO3 and Al2O3 thin films with smooth surfaces deposited by PLD were utilized for...
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| Veröffentlicht in: | Solid state ionics 2014-09, Vol.262, p.179-182 |
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| creator | Takahashi, Kuniaki Maekawa, Hideki Takamura, Hitoshi |
| description | All-solid-state lithium batteries using LiBH4 electrolyte and LiCoO2 cathode were prepared, and the effect of the intermediate layers between LiBH4 and LiCoO2 was demonstrated by electrochemical measurement. Li3PO4, LiNbO3 and Al2O3 thin films with smooth surfaces deposited by PLD were utilized for the intermediate layer. With the intermediate layer, the interfacial resistance between LiBH4 and LiCoO2 decreased by as much as 3 orders of magnitude by suppressing the interfacial reaction between LiBH4 and LiCoO2. A 10–25nm-thick Li3PO4 intermediate layer was found to be the most effective to suppress the interfacial resistance.
•All-solid-state batteries using LiBH4 as a solid electrolyte were prepared.•Large interfacial resistance between LiBH4 and LiCoO2 is the main issue.•Li3PO4, LiNbO3 and Al2O3 were adopted as the intermediate layers.•The 10–25nm-thick Li3PO4 layer presents the best characteristics. |
| doi_str_mv | 10.1016/j.ssi.2013.10.028 |
| format | Article |
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•All-solid-state batteries using LiBH4 as a solid electrolyte were prepared.•Large interfacial resistance between LiBH4 and LiCoO2 is the main issue.•Li3PO4, LiNbO3 and Al2O3 were adopted as the intermediate layers.•The 10–25nm-thick Li3PO4 layer presents the best characteristics.</description><identifier>ISSN: 0167-2738</identifier><identifier>EISSN: 1872-7689</identifier><identifier>DOI: 10.1016/j.ssi.2013.10.028</identifier><language>eng</language><publisher>Elsevier B.V</publisher><subject>All-solid-state battery ; Aluminum oxide ; Borohydrides ; Deposition ; Electrolytes ; Interface reactions ; Lithium batteries ; Lithium borohydride ; Lithium phosphate ; Pulsed laser deposition ; Retarding ; Solid electrolyte ; Thin films</subject><ispartof>Solid state ionics, 2014-09, Vol.262, p.179-182</ispartof><rights>2013 Elsevier B.V.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c466t-28f18221aa6f4679606023ce9283195c9289bc0e7a929e05a0de2c13c0bc61233</citedby><cites>FETCH-LOGICAL-c466t-28f18221aa6f4679606023ce9283195c9289bc0e7a929e05a0de2c13c0bc61233</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.ssi.2013.10.028$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,780,784,3550,27924,27925,45995</link.rule.ids></links><search><creatorcontrib>Takahashi, Kuniaki</creatorcontrib><creatorcontrib>Maekawa, Hideki</creatorcontrib><creatorcontrib>Takamura, Hitoshi</creatorcontrib><title>Effects of intermediate layer on interfacial resistance for all-solid-state lithium batteries using lithium borohydride</title><title>Solid state ionics</title><description>All-solid-state lithium batteries using LiBH4 electrolyte and LiCoO2 cathode were prepared, and the effect of the intermediate layers between LiBH4 and LiCoO2 was demonstrated by electrochemical measurement. Li3PO4, LiNbO3 and Al2O3 thin films with smooth surfaces deposited by PLD were utilized for the intermediate layer. With the intermediate layer, the interfacial resistance between LiBH4 and LiCoO2 decreased by as much as 3 orders of magnitude by suppressing the interfacial reaction between LiBH4 and LiCoO2. A 10–25nm-thick Li3PO4 intermediate layer was found to be the most effective to suppress the interfacial resistance.
•All-solid-state batteries using LiBH4 as a solid electrolyte were prepared.•Large interfacial resistance between LiBH4 and LiCoO2 is the main issue.•Li3PO4, LiNbO3 and Al2O3 were adopted as the intermediate layers.•The 10–25nm-thick Li3PO4 layer presents the best characteristics.</description><subject>All-solid-state battery</subject><subject>Aluminum oxide</subject><subject>Borohydrides</subject><subject>Deposition</subject><subject>Electrolytes</subject><subject>Interface reactions</subject><subject>Lithium batteries</subject><subject>Lithium borohydride</subject><subject>Lithium phosphate</subject><subject>Pulsed laser deposition</subject><subject>Retarding</subject><subject>Solid electrolyte</subject><subject>Thin films</subject><issn>0167-2738</issn><issn>1872-7689</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2014</creationdate><recordtype>article</recordtype><recordid>eNp9kE1LAzEQhoMoWD9-gLccvWxNsm02wZOU-gEFL3oOaXZip2w3NbNV-u9NqeDN0zAv7zMwD2M3UoylkPpuPSbCsRKyLvtYKHPCRtI0qmq0sadsVDpNpZranLMLorUQQtdGj9j3PEYIA_EUOfYD5A206Afgnd9D5qk_ptEH9B3PQEiD7wPwmDL3XVdR6rCtSnhgcFjhbsOXfigMAvEdYf_xl6ecVvs2YwtX7Cz6juD6d16y98f52-y5Wrw-vcweFlWYaD1UykRplJLe6zjRjdVCC1UHsMrU0k5DmXYZBDTeKgti6kULKsg6iGXQUtX1Jbs93t3m9LkDGtwGKUDX-R7SjlzRIqfWaDstVXmshpyIMkS3zbjxee-kcAfJbu2KZHeQfIiK5MLcHxkoP3whZEcBofhpMRetrk34D_0D8xWG2A</recordid><startdate>20140901</startdate><enddate>20140901</enddate><creator>Takahashi, Kuniaki</creator><creator>Maekawa, Hideki</creator><creator>Takamura, Hitoshi</creator><general>Elsevier B.V</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7TB</scope><scope>7U5</scope><scope>8FD</scope><scope>FR3</scope><scope>L7M</scope></search><sort><creationdate>20140901</creationdate><title>Effects of intermediate layer on interfacial resistance for all-solid-state lithium batteries using lithium borohydride</title><author>Takahashi, Kuniaki ; Maekawa, Hideki ; Takamura, Hitoshi</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c466t-28f18221aa6f4679606023ce9283195c9289bc0e7a929e05a0de2c13c0bc61233</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2014</creationdate><topic>All-solid-state battery</topic><topic>Aluminum oxide</topic><topic>Borohydrides</topic><topic>Deposition</topic><topic>Electrolytes</topic><topic>Interface reactions</topic><topic>Lithium batteries</topic><topic>Lithium borohydride</topic><topic>Lithium phosphate</topic><topic>Pulsed laser deposition</topic><topic>Retarding</topic><topic>Solid electrolyte</topic><topic>Thin films</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Takahashi, Kuniaki</creatorcontrib><creatorcontrib>Maekawa, Hideki</creatorcontrib><creatorcontrib>Takamura, Hitoshi</creatorcontrib><collection>CrossRef</collection><collection>Mechanical & Transportation Engineering Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Engineering Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Solid state ionics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Takahashi, Kuniaki</au><au>Maekawa, Hideki</au><au>Takamura, Hitoshi</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Effects of intermediate layer on interfacial resistance for all-solid-state lithium batteries using lithium borohydride</atitle><jtitle>Solid state ionics</jtitle><date>2014-09-01</date><risdate>2014</risdate><volume>262</volume><spage>179</spage><epage>182</epage><pages>179-182</pages><issn>0167-2738</issn><eissn>1872-7689</eissn><abstract>All-solid-state lithium batteries using LiBH4 electrolyte and LiCoO2 cathode were prepared, and the effect of the intermediate layers between LiBH4 and LiCoO2 was demonstrated by electrochemical measurement. Li3PO4, LiNbO3 and Al2O3 thin films with smooth surfaces deposited by PLD were utilized for the intermediate layer. With the intermediate layer, the interfacial resistance between LiBH4 and LiCoO2 decreased by as much as 3 orders of magnitude by suppressing the interfacial reaction between LiBH4 and LiCoO2. A 10–25nm-thick Li3PO4 intermediate layer was found to be the most effective to suppress the interfacial resistance.
•All-solid-state batteries using LiBH4 as a solid electrolyte were prepared.•Large interfacial resistance between LiBH4 and LiCoO2 is the main issue.•Li3PO4, LiNbO3 and Al2O3 were adopted as the intermediate layers.•The 10–25nm-thick Li3PO4 layer presents the best characteristics.</abstract><pub>Elsevier B.V</pub><doi>10.1016/j.ssi.2013.10.028</doi><tpages>4</tpages></addata></record> |
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| language | eng |
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| source | Access via ScienceDirect (Elsevier) |
| subjects | All-solid-state battery Aluminum oxide Borohydrides Deposition Electrolytes Interface reactions Lithium batteries Lithium borohydride Lithium phosphate Pulsed laser deposition Retarding Solid electrolyte Thin films |
| title | Effects of intermediate layer on interfacial resistance for all-solid-state lithium batteries using lithium borohydride |
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