Tracing lead pollution sources in abandoned mine areas using stable Pb isotope ratios
This study focused on Pb isotope ratios of sediments in areas around an abandoned mine to determine if the ratios can be used as a source tracer. For pretreatment, sediment samples were dissolved with mixed acids, and a multi-collector inductively coupled plasma mass spectrometer (MC-ICP-MS, Nu plas...
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| Veröffentlicht in: | Environmental monitoring and assessment 2014-02, Vol.186 (2), p.781-789 |
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| creator | Yoo, Eun-Jin Lee, Jung-A Park, Jae-Seon Lee, Khanghyun Lee, Won-Seok Han, Jin-Seok Choi, Jong-Woo |
| description | This study focused on Pb isotope ratios of sediments in areas around an abandoned mine to determine if the ratios can be used as a source tracer. For pretreatment, sediment samples were dissolved with mixed acids, and a multi-collector inductively coupled plasma mass spectrometer (MC-ICP-MS, Nu plasma II) was used to investigate the Pb isotopic composition of the samples. The measured isotope ratios were then corrected for instrumental mass fractionation by measuring the ²⁰³Tl/²⁰⁵Tl ratio. Repeated measurements with the NIST SRM 981 reference material showed that the precision of all ratios was below 104 ppm (±2σ) for 50 ng/g. The isotope ratios (²⁰⁷Pb/²⁰⁶Pb) found were 0.85073 ± 0.0004~0.85373 ± 0.0003 for the main stream, while they were 0.83736 ± 0.0010 for the tributary and 0.84393 ± 0.0002 for the confluence. A binary mixing equation for isotope ratios showed that the contributions of mine lead to neighboring areas were up to 60 %. Therefore, Pb isotope ratios can be a good source tracer for areas around abandoned mines. |
| doi_str_mv | 10.1007/s10661-013-3416-8 |
| format | Article |
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For pretreatment, sediment samples were dissolved with mixed acids, and a multi-collector inductively coupled plasma mass spectrometer (MC-ICP-MS, Nu plasma II) was used to investigate the Pb isotopic composition of the samples. The measured isotope ratios were then corrected for instrumental mass fractionation by measuring the ²⁰³Tl/²⁰⁵Tl ratio. Repeated measurements with the NIST SRM 981 reference material showed that the precision of all ratios was below 104 ppm (±2σ) for 50 ng/g. The isotope ratios (²⁰⁷Pb/²⁰⁶Pb) found were 0.85073 ± 0.0004~0.85373 ± 0.0003 for the main stream, while they were 0.83736 ± 0.0010 for the tributary and 0.84393 ± 0.0002 for the confluence. A binary mixing equation for isotope ratios showed that the contributions of mine lead to neighboring areas were up to 60 %. Therefore, Pb isotope ratios can be a good source tracer for areas around abandoned mines.</description><identifier>ISSN: 0167-6369</identifier><identifier>EISSN: 1573-2959</identifier><identifier>DOI: 10.1007/s10661-013-3416-8</identifier><identifier>PMID: 24197555</identifier><language>eng</language><publisher>Dordrecht: Springer-Verlag</publisher><subject>Abandoned mines ; Acids ; Analysis ; Assessments ; Atmospheric Protection/Air Quality Control/Air Pollution ; Collectors ; Contaminated sediments ; Dissolution ; Earth and Environmental Science ; Ecology ; Ecotoxicology ; Environment ; Environmental Management ; Environmental monitoring ; Environmental Monitoring - methods ; Environmental Pollution - statistics & numerical data ; Environmental research ; Fractionation ; Heavy metals ; Isotope ratios ; Isotopes ; Isotopes - analysis ; Lead ; Lead (metal) ; Lead - analysis ; Mathematical analysis ; Mining ; Monitoring/Environmental Analysis ; National parks ; Pollution ; Pollution sources ; Ratios ; Republic of Korea ; Sediment samplers ; Sediments ; Soil Pollutants - analysis ; spectrometers ; Studies ; Tracers</subject><ispartof>Environmental monitoring and assessment, 2014-02, Vol.186 (2), p.781-789</ispartof><rights>Springer Science+Business Media Dordrecht 2013</rights><rights>Springer Science+Business Media Dordrecht 2014</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c528t-18a5fd77b99e79a480d904864508145f3ed73ba50bce83a3755d35c66326e8013</citedby><cites>FETCH-LOGICAL-c528t-18a5fd77b99e79a480d904864508145f3ed73ba50bce83a3755d35c66326e8013</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10661-013-3416-8$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10661-013-3416-8$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/24197555$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Yoo, Eun-Jin</creatorcontrib><creatorcontrib>Lee, Jung-A</creatorcontrib><creatorcontrib>Park, Jae-Seon</creatorcontrib><creatorcontrib>Lee, Khanghyun</creatorcontrib><creatorcontrib>Lee, Won-Seok</creatorcontrib><creatorcontrib>Han, Jin-Seok</creatorcontrib><creatorcontrib>Choi, Jong-Woo</creatorcontrib><title>Tracing lead pollution sources in abandoned mine areas using stable Pb isotope ratios</title><title>Environmental monitoring and assessment</title><addtitle>Environ Monit Assess</addtitle><addtitle>Environ Monit Assess</addtitle><description>This study focused on Pb isotope ratios of sediments in areas around an abandoned mine to determine if the ratios can be used as a source tracer. For pretreatment, sediment samples were dissolved with mixed acids, and a multi-collector inductively coupled plasma mass spectrometer (MC-ICP-MS, Nu plasma II) was used to investigate the Pb isotopic composition of the samples. The measured isotope ratios were then corrected for instrumental mass fractionation by measuring the ²⁰³Tl/²⁰⁵Tl ratio. Repeated measurements with the NIST SRM 981 reference material showed that the precision of all ratios was below 104 ppm (±2σ) for 50 ng/g. The isotope ratios (²⁰⁷Pb/²⁰⁶Pb) found were 0.85073 ± 0.0004~0.85373 ± 0.0003 for the main stream, while they were 0.83736 ± 0.0010 for the tributary and 0.84393 ± 0.0002 for the confluence. A binary mixing equation for isotope ratios showed that the contributions of mine lead to neighboring areas were up to 60 %. Therefore, Pb isotope ratios can be a good source tracer for areas around abandoned mines.</description><subject>Abandoned mines</subject><subject>Acids</subject><subject>Analysis</subject><subject>Assessments</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Collectors</subject><subject>Contaminated sediments</subject><subject>Dissolution</subject><subject>Earth and Environmental Science</subject><subject>Ecology</subject><subject>Ecotoxicology</subject><subject>Environment</subject><subject>Environmental Management</subject><subject>Environmental monitoring</subject><subject>Environmental Monitoring - methods</subject><subject>Environmental Pollution - statistics & numerical data</subject><subject>Environmental research</subject><subject>Fractionation</subject><subject>Heavy metals</subject><subject>Isotope ratios</subject><subject>Isotopes</subject><subject>Isotopes - analysis</subject><subject>Lead</subject><subject>Lead (metal)</subject><subject>Lead - analysis</subject><subject>Mathematical analysis</subject><subject>Mining</subject><subject>Monitoring/Environmental Analysis</subject><subject>National parks</subject><subject>Pollution</subject><subject>Pollution sources</subject><subject>Ratios</subject><subject>Republic of Korea</subject><subject>Sediment samplers</subject><subject>Sediments</subject><subject>Soil Pollutants - analysis</subject><subject>spectrometers</subject><subject>Studies</subject><subject>Tracers</subject><issn>0167-6369</issn><issn>1573-2959</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2014</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><sourceid>BENPR</sourceid><recordid>eNqFkU9v1DAQxS0EotvCB-AClrhwCYzj_0dUAUWqBBLds-Ukk1WqrL14kgPfHq9SEOIAJx_m957nzWPshYC3AsC-IwHGiAaEbKQSpnGP2E5oK5vWa_-Y7UAY2xhp_AW7JLoHAG-Vf8ouWiW81Vrv2P6uxH5KBz5jHPgpz_O6TDlxymvpkfiUeOxiGnLCgR-nhDwWjMRXOotoid2M_GvHJ8pLPiEvscrpGXsyxpnw-cN7xfYfP9xd3zS3Xz59vn5_2_S6dUsjXNTjYG3nPVoflYPBg3JGaXBC6VHiYGUXNXQ9OhllXXmQujdGtgZdjX3F3my-p5K_r0hLOE7U4zzHhHmlUPMLpYRz8v-o8sY54ZWp6Ou_0Pt6jVSDVMqaVusWoFJio_qSiQqO4VSmYyw_goBwrids9YS6ZzjXE1zVvHxwXrsjDr8Vv_qoQLsBVEfpgOWPr__h-moTjTGHeCgThf23FoSqhet6Ry1_Aj7voXU</recordid><startdate>20140201</startdate><enddate>20140201</enddate><creator>Yoo, Eun-Jin</creator><creator>Lee, Jung-A</creator><creator>Park, Jae-Seon</creator><creator>Lee, Khanghyun</creator><creator>Lee, Won-Seok</creator><creator>Han, Jin-Seok</creator><creator>Choi, Jong-Woo</creator><general>Springer-Verlag</general><general>Springer Netherlands</general><general>Springer Nature B.V</general><scope>FBQ</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7QH</scope><scope>7QL</scope><scope>7SN</scope><scope>7ST</scope><scope>7T7</scope><scope>7TG</scope><scope>7TN</scope><scope>7U7</scope><scope>7UA</scope><scope>7WY</scope><scope>7WZ</scope><scope>7X7</scope><scope>7XB</scope><scope>87Z</scope><scope>88E</scope><scope>88I</scope><scope>8AO</scope><scope>8C1</scope><scope>8FD</scope><scope>8FI</scope><scope>8FJ</scope><scope>8FK</scope><scope>8FL</scope><scope>ABUWG</scope><scope>AEUYN</scope><scope>AFKRA</scope><scope>ATCPS</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BEZIV</scope><scope>BHPHI</scope><scope>C1K</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>F1W</scope><scope>FR3</scope><scope>FRNLG</scope><scope>FYUFA</scope><scope>F~G</scope><scope>GHDGH</scope><scope>GNUQQ</scope><scope>H97</scope><scope>HCIFZ</scope><scope>K60</scope><scope>K6~</scope><scope>K9.</scope><scope>KL.</scope><scope>L.-</scope><scope>L.G</scope><scope>M0C</scope><scope>M0S</scope><scope>M1P</scope><scope>M2P</scope><scope>M7N</scope><scope>P64</scope><scope>PATMY</scope><scope>PQBIZ</scope><scope>PQBZA</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PYCSY</scope><scope>Q9U</scope><scope>SOI</scope><scope>7TV</scope><scope>7SU</scope><scope>KR7</scope></search><sort><creationdate>20140201</creationdate><title>Tracing lead pollution sources in abandoned mine areas using stable Pb isotope ratios</title><author>Yoo, Eun-Jin ; Lee, Jung-A ; Park, Jae-Seon ; Lee, Khanghyun ; Lee, Won-Seok ; Han, Jin-Seok ; Choi, Jong-Woo</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c528t-18a5fd77b99e79a480d904864508145f3ed73ba50bce83a3755d35c66326e8013</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2014</creationdate><topic>Abandoned mines</topic><topic>Acids</topic><topic>Analysis</topic><topic>Assessments</topic><topic>Atmospheric Protection/Air Quality Control/Air Pollution</topic><topic>Collectors</topic><topic>Contaminated sediments</topic><topic>Dissolution</topic><topic>Earth and Environmental Science</topic><topic>Ecology</topic><topic>Ecotoxicology</topic><topic>Environment</topic><topic>Environmental Management</topic><topic>Environmental monitoring</topic><topic>Environmental Monitoring - methods</topic><topic>Environmental Pollution - statistics & numerical data</topic><topic>Environmental research</topic><topic>Fractionation</topic><topic>Heavy metals</topic><topic>Isotope ratios</topic><topic>Isotopes</topic><topic>Isotopes - analysis</topic><topic>Lead</topic><topic>Lead (metal)</topic><topic>Lead - analysis</topic><topic>Mathematical analysis</topic><topic>Mining</topic><topic>Monitoring/Environmental Analysis</topic><topic>National parks</topic><topic>Pollution</topic><topic>Pollution sources</topic><topic>Ratios</topic><topic>Republic of Korea</topic><topic>Sediment samplers</topic><topic>Sediments</topic><topic>Soil Pollutants - analysis</topic><topic>spectrometers</topic><topic>Studies</topic><topic>Tracers</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Yoo, Eun-Jin</creatorcontrib><creatorcontrib>Lee, Jung-A</creatorcontrib><creatorcontrib>Park, Jae-Seon</creatorcontrib><creatorcontrib>Lee, Khanghyun</creatorcontrib><creatorcontrib>Lee, Won-Seok</creatorcontrib><creatorcontrib>Han, Jin-Seok</creatorcontrib><creatorcontrib>Choi, Jong-Woo</creatorcontrib><collection>AGRIS</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>Aqualine</collection><collection>Bacteriology Abstracts (Microbiology B)</collection><collection>Ecology Abstracts</collection><collection>Environment Abstracts</collection><collection>Industrial and Applied Microbiology Abstracts (Microbiology A)</collection><collection>Meteorological & Geoastrophysical Abstracts</collection><collection>Oceanic Abstracts</collection><collection>Toxicology Abstracts</collection><collection>Water Resources Abstracts</collection><collection>ABI/INFORM Collection</collection><collection>ABI/INFORM Global (PDF only)</collection><collection>Health & Medical Collection</collection><collection>ProQuest Central (purchase pre-March 2016)</collection><collection>ABI/INFORM Global (Alumni Edition)</collection><collection>Medical Database (Alumni Edition)</collection><collection>Science Database (Alumni Edition)</collection><collection>ProQuest Pharma Collection</collection><collection>Public Health Database</collection><collection>Technology Research Database</collection><collection>Hospital Premium Collection</collection><collection>Hospital Premium Collection (Alumni Edition)</collection><collection>ProQuest Central (Alumni) (purchase pre-March 2016)</collection><collection>ABI/INFORM Collection (Alumni Edition)</collection><collection>ProQuest Central (Alumni Edition)</collection><collection>ProQuest One Sustainability</collection><collection>ProQuest Central UK/Ireland</collection><collection>Agricultural & Environmental Science Collection</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>Business Premium Collection</collection><collection>Natural Science Collection</collection><collection>Environmental Sciences and Pollution Management</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central Korea</collection><collection>ASFA: Aquatic Sciences and Fisheries Abstracts</collection><collection>Engineering Research Database</collection><collection>Business Premium Collection (Alumni)</collection><collection>Health Research Premium Collection</collection><collection>ABI/INFORM Global (Corporate)</collection><collection>Health Research Premium Collection (Alumni)</collection><collection>ProQuest Central Student</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) 3: Aquatic Pollution & Environmental Quality</collection><collection>SciTech Premium Collection</collection><collection>ProQuest Business Collection (Alumni Edition)</collection><collection>ProQuest Business Collection</collection><collection>ProQuest Health & Medical Complete (Alumni)</collection><collection>Meteorological & Geoastrophysical Abstracts - 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For pretreatment, sediment samples were dissolved with mixed acids, and a multi-collector inductively coupled plasma mass spectrometer (MC-ICP-MS, Nu plasma II) was used to investigate the Pb isotopic composition of the samples. The measured isotope ratios were then corrected for instrumental mass fractionation by measuring the ²⁰³Tl/²⁰⁵Tl ratio. Repeated measurements with the NIST SRM 981 reference material showed that the precision of all ratios was below 104 ppm (±2σ) for 50 ng/g. The isotope ratios (²⁰⁷Pb/²⁰⁶Pb) found were 0.85073 ± 0.0004~0.85373 ± 0.0003 for the main stream, while they were 0.83736 ± 0.0010 for the tributary and 0.84393 ± 0.0002 for the confluence. A binary mixing equation for isotope ratios showed that the contributions of mine lead to neighboring areas were up to 60 %. Therefore, Pb isotope ratios can be a good source tracer for areas around abandoned mines.</abstract><cop>Dordrecht</cop><pub>Springer-Verlag</pub><pmid>24197555</pmid><doi>10.1007/s10661-013-3416-8</doi><tpages>9</tpages></addata></record> |
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| subjects | Abandoned mines Acids Analysis Assessments Atmospheric Protection/Air Quality Control/Air Pollution Collectors Contaminated sediments Dissolution Earth and Environmental Science Ecology Ecotoxicology Environment Environmental Management Environmental monitoring Environmental Monitoring - methods Environmental Pollution - statistics & numerical data Environmental research Fractionation Heavy metals Isotope ratios Isotopes Isotopes - analysis Lead Lead (metal) Lead - analysis Mathematical analysis Mining Monitoring/Environmental Analysis National parks Pollution Pollution sources Ratios Republic of Korea Sediment samplers Sediments Soil Pollutants - analysis spectrometers Studies Tracers |
| title | Tracing lead pollution sources in abandoned mine areas using stable Pb isotope ratios |
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