Ultrafast structural dynamics of perovskite superlattices

Femtosecond x-ray diffraction provides direct insight into the ultrafast reversible lattice dynamics of materials with a perovskite structure. Superlattice (SL) structures consisting of a sequence of nanometer-thick layer pairs allow for optically inducing a tailored stress profile that drives the l...

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Veröffentlicht in:Applied physics. A, Materials science & processing Materials science & processing, 2009-07, Vol.96 (1), p.83-90, Article 83
Hauptverfasser: Woerner, M., v. Korff Schmising, C., Bargheer, M., Zhavoronkov, N., Vrejoiu, I., Hesse, D., Alexe, M., Elsaesser, T.
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container_issue 1
container_start_page 83
container_title Applied physics. A, Materials science & processing
container_volume 96
creator Woerner, M.
v. Korff Schmising, C.
Bargheer, M.
Zhavoronkov, N.
Vrejoiu, I.
Hesse, D.
Alexe, M.
Elsaesser, T.
description Femtosecond x-ray diffraction provides direct insight into the ultrafast reversible lattice dynamics of materials with a perovskite structure. Superlattice (SL) structures consisting of a sequence of nanometer-thick layer pairs allow for optically inducing a tailored stress profile that drives the lattice motions and for limiting the influence of strain propagation on the observed dynamics. We demonstrate this concept in a series of diffraction experiments with femtosecond time resolution, giving detailed information on the ultrafast lattice dynamics of ferroelectric and ferromagnetic superlattices. Anharmonically coupled lattice motions in a SrRuO 3 /PbZr 0.2 Ti 0.8 O 3 (SRO/PZT) SL lead to a switch-off of the electric polarizations on a time scale of the order of 1 ps. Ultrafast magnetostriction of photoexcited SRO layers is demonstrated in a SRO/SrTiO 3 (STO) SL.
doi_str_mv 10.1007/s00339-009-5174-6
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subjects Characterization and Evaluation of Materials
Condensed Matter Physics
Diffraction
Dynamics
Femtosecond
Ferromagnetism
Lattices
Machines
Manufacturing
Nanotechnology
Optical and Electronic Materials
Perovskite structure
Physics
Physics and Astronomy
Processes
Short range order
Superlattices
Surfaces and Interfaces
Thin Films
title Ultrafast structural dynamics of perovskite superlattices
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