The use of biodiesel blends on a non-road generator and its impacts on ozone formation potentials based on carbonyl emissions
In this study, emissions of carbonyl compounds from the use B50 and B100 were measured with a non-road diesel generator. A total of 25 carbonyl compounds were identified in the exhaust, including 10 with laboratory-synthesized standards. Formaldehyde, acetaldehyde, and acrolein were found as the mos...
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| Veröffentlicht in: | Environmental pollution (1987) 2013-07, Vol.178, p.159-165 |
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| creator | Chai, Ming Lu, Mingming Liang, Fuyan Tzillah, Aisha Dendramis, Nancy Watson, Libya |
| description | In this study, emissions of carbonyl compounds from the use B50 and B100 were measured with a non-road diesel generator. A total of 25 carbonyl compounds were identified in the exhaust, including 10 with laboratory-synthesized standards. Formaldehyde, acetaldehyde, and acrolein were found as the most abundant carbonyl compounds emitted for both diesel and biodiesel. The sulphur content of diesel fuels and the source of biodiesel fuels were not found to have a significant impact on the emission of carbonyl compounds. The overall maximum incremental reactivity (MIR) was the highest at 0 kW and slightly increased from 25 to 75 kW. The MIR of B100 was the highest, followed by diesel and B50, which is consistent with the emission rates of total carbonyl compounds. This suggests that the use of biodiesel blends may be more beneficial to the environment than using pure biodiesel.
•Carbonyl compound emission from biodiesel blends combustion on a non-road generator.•25 compounds were identified, including 10 by laboratory-synthesized standards.•Sources of biodiesel have insignificant impacts on carbonyl compounds emission.•Sulphur contents have insignificant impacts on carbonyl compounds emission.•MIR of emitted carbonyls decreases in the following order: B100, diesel, B50.
The study found that B50 resulted in lower total carbonyl emission rates and ozone formation potential resultant from these compounds, whereas both increased with B100. |
| doi_str_mv | 10.1016/j.envpol.2013.03.021 |
| format | Article |
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•Carbonyl compound emission from biodiesel blends combustion on a non-road generator.•25 compounds were identified, including 10 by laboratory-synthesized standards.•Sources of biodiesel have insignificant impacts on carbonyl compounds emission.•Sulphur contents have insignificant impacts on carbonyl compounds emission.•MIR of emitted carbonyls decreases in the following order: B100, diesel, B50.
The study found that B50 resulted in lower total carbonyl emission rates and ozone formation potential resultant from these compounds, whereas both increased with B100.</description><identifier>ISSN: 0269-7491</identifier><identifier>EISSN: 1873-6424</identifier><identifier>DOI: 10.1016/j.envpol.2013.03.021</identifier><identifier>PMID: 23583671</identifier><identifier>CODEN: ENVPAF</identifier><language>eng</language><publisher>Kidlington: Elsevier Ltd</publisher><subject>acetaldehyde ; acrolein ; Air Pollutants - analysis ; Air Pollution - statistics & numerical data ; Applied sciences ; Atmospheric pollution ; Biodiesel ; Biofuels ; Blends ; Carbonyl compounds ; Diesel ; diesel fuel ; Diesel fuels ; Electric Power Supplies ; emissions ; Environmental Monitoring ; Exact sciences and technology ; formaldehyde ; Generators ; generators (equipment) ; Maximum incremental reactivity (MIR) ; Non-road engine ; ozone ; Ozone - analysis ; Ozone formation potential ; Pollution ; Pollution sources. Measurement results ; Polymer blends ; Power Plants ; sulfur ; Transports</subject><ispartof>Environmental pollution (1987), 2013-07, Vol.178, p.159-165</ispartof><rights>2013 Elsevier Ltd</rights><rights>2014 INIST-CNRS</rights><rights>Copyright © 2013 Elsevier Ltd. All rights reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c482t-c1791ea8535ef28b679fe0f9a425b7efae05381d9c59a0e09f69a091fad6cef83</citedby><cites>FETCH-LOGICAL-c482t-c1791ea8535ef28b679fe0f9a425b7efae05381d9c59a0e09f69a091fad6cef83</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.envpol.2013.03.021$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,780,784,3548,27923,27924,45994</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=27398124$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/23583671$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Chai, Ming</creatorcontrib><creatorcontrib>Lu, Mingming</creatorcontrib><creatorcontrib>Liang, Fuyan</creatorcontrib><creatorcontrib>Tzillah, Aisha</creatorcontrib><creatorcontrib>Dendramis, Nancy</creatorcontrib><creatorcontrib>Watson, Libya</creatorcontrib><title>The use of biodiesel blends on a non-road generator and its impacts on ozone formation potentials based on carbonyl emissions</title><title>Environmental pollution (1987)</title><addtitle>Environ Pollut</addtitle><description>In this study, emissions of carbonyl compounds from the use B50 and B100 were measured with a non-road diesel generator. A total of 25 carbonyl compounds were identified in the exhaust, including 10 with laboratory-synthesized standards. Formaldehyde, acetaldehyde, and acrolein were found as the most abundant carbonyl compounds emitted for both diesel and biodiesel. The sulphur content of diesel fuels and the source of biodiesel fuels were not found to have a significant impact on the emission of carbonyl compounds. The overall maximum incremental reactivity (MIR) was the highest at 0 kW and slightly increased from 25 to 75 kW. The MIR of B100 was the highest, followed by diesel and B50, which is consistent with the emission rates of total carbonyl compounds. This suggests that the use of biodiesel blends may be more beneficial to the environment than using pure biodiesel.
•Carbonyl compound emission from biodiesel blends combustion on a non-road generator.•25 compounds were identified, including 10 by laboratory-synthesized standards.•Sources of biodiesel have insignificant impacts on carbonyl compounds emission.•Sulphur contents have insignificant impacts on carbonyl compounds emission.•MIR of emitted carbonyls decreases in the following order: B100, diesel, B50.
The study found that B50 resulted in lower total carbonyl emission rates and ozone formation potential resultant from these compounds, whereas both increased with B100.</description><subject>acetaldehyde</subject><subject>acrolein</subject><subject>Air Pollutants - analysis</subject><subject>Air Pollution - statistics & numerical data</subject><subject>Applied sciences</subject><subject>Atmospheric pollution</subject><subject>Biodiesel</subject><subject>Biofuels</subject><subject>Blends</subject><subject>Carbonyl compounds</subject><subject>Diesel</subject><subject>diesel fuel</subject><subject>Diesel fuels</subject><subject>Electric Power Supplies</subject><subject>emissions</subject><subject>Environmental Monitoring</subject><subject>Exact sciences and technology</subject><subject>formaldehyde</subject><subject>Generators</subject><subject>generators (equipment)</subject><subject>Maximum incremental reactivity (MIR)</subject><subject>Non-road engine</subject><subject>ozone</subject><subject>Ozone - analysis</subject><subject>Ozone formation potential</subject><subject>Pollution</subject><subject>Pollution sources. Measurement results</subject><subject>Polymer blends</subject><subject>Power Plants</subject><subject>sulfur</subject><subject>Transports</subject><issn>0269-7491</issn><issn>1873-6424</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2013</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqN0l2L1TAQBuAiintc_QeiuRG86TEfTdrcCLL4BQteuHsdpulkzaFNatKzsIL_3dQe9U6FwBB4ZjLwpqqeMrpnlKlXhz2G2zmOe06Z2NNyOLtX7VjXilo1vLlf7ShXum4bzc6qRzkfKKWNEOJhdcaF7IRq2a76fvUFyTEjiY70Pg4eM46kHzEMmcRAgIQY6hRhIDcYMMESE4EwEL9k4qcZ7PLTxW8xIHExTbD4cp_jgmHxMGbSQ8ZhNRZSH8PdSHDyOReVH1cPXCH45FTPq-t3b68uPtSXn95_vHhzWdum40ttWasZQieFRMe7XrXaIXUaGi77Fh0glaJjg7ZSA0WqnSpVMweDsug6cV693ObOKX49Yl5M2cDiOELAeMyGKcmElpyq_6BCUi540_ybCil0J6VapzYbtSnmnNCZOfkJ0p1h1KxxmoPZ4jRrnIaWw1lpe3Z64dhPOPxu-pVfAS9OALKF0SUI1uc_ri0LML6u-nxzDqKBm1TM9efykix_gnHe8CJebwJLDrcek8nWY7A4-IR2MUP0f9_1B-FqyfM</recordid><startdate>20130701</startdate><enddate>20130701</enddate><creator>Chai, Ming</creator><creator>Lu, Mingming</creator><creator>Liang, Fuyan</creator><creator>Tzillah, Aisha</creator><creator>Dendramis, Nancy</creator><creator>Watson, Libya</creator><general>Elsevier Ltd</general><general>Elsevier</general><scope>FBQ</scope><scope>IQODW</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>7ST</scope><scope>7TG</scope><scope>7TV</scope><scope>7U7</scope><scope>C1K</scope><scope>KL.</scope><scope>SOI</scope><scope>7SU</scope><scope>7TB</scope><scope>8FD</scope><scope>FR3</scope><scope>KR7</scope></search><sort><creationdate>20130701</creationdate><title>The use of biodiesel blends on a non-road generator and its impacts on ozone formation potentials based on carbonyl emissions</title><author>Chai, Ming ; Lu, Mingming ; Liang, Fuyan ; Tzillah, Aisha ; Dendramis, Nancy ; Watson, Libya</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c482t-c1791ea8535ef28b679fe0f9a425b7efae05381d9c59a0e09f69a091fad6cef83</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2013</creationdate><topic>acetaldehyde</topic><topic>acrolein</topic><topic>Air Pollutants - analysis</topic><topic>Air Pollution - statistics & numerical data</topic><topic>Applied sciences</topic><topic>Atmospheric pollution</topic><topic>Biodiesel</topic><topic>Biofuels</topic><topic>Blends</topic><topic>Carbonyl compounds</topic><topic>Diesel</topic><topic>diesel fuel</topic><topic>Diesel fuels</topic><topic>Electric Power Supplies</topic><topic>emissions</topic><topic>Environmental Monitoring</topic><topic>Exact sciences and technology</topic><topic>formaldehyde</topic><topic>Generators</topic><topic>generators (equipment)</topic><topic>Maximum incremental reactivity (MIR)</topic><topic>Non-road engine</topic><topic>ozone</topic><topic>Ozone - analysis</topic><topic>Ozone formation potential</topic><topic>Pollution</topic><topic>Pollution sources. Measurement results</topic><topic>Polymer blends</topic><topic>Power Plants</topic><topic>sulfur</topic><topic>Transports</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Chai, Ming</creatorcontrib><creatorcontrib>Lu, Mingming</creatorcontrib><creatorcontrib>Liang, Fuyan</creatorcontrib><creatorcontrib>Tzillah, Aisha</creatorcontrib><creatorcontrib>Dendramis, Nancy</creatorcontrib><creatorcontrib>Watson, Libya</creatorcontrib><collection>AGRIS</collection><collection>Pascal-Francis</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>Environment Abstracts</collection><collection>Meteorological & Geoastrophysical Abstracts</collection><collection>Pollution Abstracts</collection><collection>Toxicology Abstracts</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Meteorological & Geoastrophysical Abstracts - Academic</collection><collection>Environment Abstracts</collection><collection>Environmental Engineering Abstracts</collection><collection>Mechanical & Transportation Engineering Abstracts</collection><collection>Technology Research Database</collection><collection>Engineering Research Database</collection><collection>Civil Engineering Abstracts</collection><jtitle>Environmental pollution (1987)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Chai, Ming</au><au>Lu, Mingming</au><au>Liang, Fuyan</au><au>Tzillah, Aisha</au><au>Dendramis, Nancy</au><au>Watson, Libya</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>The use of biodiesel blends on a non-road generator and its impacts on ozone formation potentials based on carbonyl emissions</atitle><jtitle>Environmental pollution (1987)</jtitle><addtitle>Environ Pollut</addtitle><date>2013-07-01</date><risdate>2013</risdate><volume>178</volume><spage>159</spage><epage>165</epage><pages>159-165</pages><issn>0269-7491</issn><eissn>1873-6424</eissn><coden>ENVPAF</coden><abstract>In this study, emissions of carbonyl compounds from the use B50 and B100 were measured with a non-road diesel generator. A total of 25 carbonyl compounds were identified in the exhaust, including 10 with laboratory-synthesized standards. Formaldehyde, acetaldehyde, and acrolein were found as the most abundant carbonyl compounds emitted for both diesel and biodiesel. The sulphur content of diesel fuels and the source of biodiesel fuels were not found to have a significant impact on the emission of carbonyl compounds. The overall maximum incremental reactivity (MIR) was the highest at 0 kW and slightly increased from 25 to 75 kW. The MIR of B100 was the highest, followed by diesel and B50, which is consistent with the emission rates of total carbonyl compounds. This suggests that the use of biodiesel blends may be more beneficial to the environment than using pure biodiesel.
•Carbonyl compound emission from biodiesel blends combustion on a non-road generator.•25 compounds were identified, including 10 by laboratory-synthesized standards.•Sources of biodiesel have insignificant impacts on carbonyl compounds emission.•Sulphur contents have insignificant impacts on carbonyl compounds emission.•MIR of emitted carbonyls decreases in the following order: B100, diesel, B50.
The study found that B50 resulted in lower total carbonyl emission rates and ozone formation potential resultant from these compounds, whereas both increased with B100.</abstract><cop>Kidlington</cop><pub>Elsevier Ltd</pub><pmid>23583671</pmid><doi>10.1016/j.envpol.2013.03.021</doi><tpages>7</tpages></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0269-7491 |
| ispartof | Environmental pollution (1987), 2013-07, Vol.178, p.159-165 |
| issn | 0269-7491 1873-6424 |
| language | eng |
| recordid | cdi_proquest_miscellaneous_1651395206 |
| source | MEDLINE; ScienceDirect Journals (5 years ago - present) |
| subjects | acetaldehyde acrolein Air Pollutants - analysis Air Pollution - statistics & numerical data Applied sciences Atmospheric pollution Biodiesel Biofuels Blends Carbonyl compounds Diesel diesel fuel Diesel fuels Electric Power Supplies emissions Environmental Monitoring Exact sciences and technology formaldehyde Generators generators (equipment) Maximum incremental reactivity (MIR) Non-road engine ozone Ozone - analysis Ozone formation potential Pollution Pollution sources. Measurement results Polymer blends Power Plants sulfur Transports |
| title | The use of biodiesel blends on a non-road generator and its impacts on ozone formation potentials based on carbonyl emissions |
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