Piezoelectric Nanoparticle–Polymer Composite Foams

Piezoelectric polymer composite foams are synthesized using different sugar-templating strategies. By incorporating sugar grains directly into polydimethylsiloxane mixtures containing barium titanate nanoparticles and carbon nanotubes, followed by removal of the sugar after polymer curing, highly co...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:ACS applied materials & interfaces 2014-11, Vol.6 (22), p.19504-19509
Hauptverfasser: McCall, William R, Kim, Kanguk, Heath, Cory, La Pierre, Gina, Sirbuly, Donald J
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page 19509
container_issue 22
container_start_page 19504
container_title ACS applied materials & interfaces
container_volume 6
creator McCall, William R
Kim, Kanguk
Heath, Cory
La Pierre, Gina
Sirbuly, Donald J
description Piezoelectric polymer composite foams are synthesized using different sugar-templating strategies. By incorporating sugar grains directly into polydimethylsiloxane mixtures containing barium titanate nanoparticles and carbon nanotubes, followed by removal of the sugar after polymer curing, highly compliant materials with excellent piezoelectric properties can be fabricated. Porosities and elasticity are tuned by simply adjusting the sugar/polymer mass ratio which gave an upper bound on the porosity of 73% and a lower bound on the elastic coefficient of 32 kPa. The electrical performance of the foams showed a direct relationship between porosity and the piezoelectric outputs, giving piezoelectric coefficient values of ∼112 pC/N and a power output of ∼18 mW/cm3 under a load of 10 N for the highest porosity samples. These novel materials should find exciting use in a variety of applications including energy scavenging platforms, biosensors, and acoustic actuators.
doi_str_mv 10.1021/am506415y
format Article
fullrecord <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_1628527925</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>1628527925</sourcerecordid><originalsourceid>FETCH-LOGICAL-a315t-1e76d7a1581999243a2b28e6f9dcb4d043d1deea751a952ccdb5d32f6f2788d93</originalsourceid><addsrcrecordid>eNptkL1OwzAURi0EoqUw8AKoCxIMAf8m9ogqCkgVdIDZcuwbKVVcBzsZysQ78IY8CUEtnZjuHY6O9B2Ezgm-IZiSW-MFzjkRmwM0JorzTFJBD_c_5yN0ktIK45xRLI7RiAomWC6LMeLLGj4CNGC7WNvps1mH1sSutg18f34tQ7PxEKez4NuQ6g6m82B8OkVHlWkSnO3uBL3N719nj9ni5eFpdrfIDCOiywgUuSsMEZIopShnhpZUQl4pZ0vuMGeOOABTCGKUoNa6UjhGq7yihZROsQm62nrbGN57SJ32dbLQNGYNoU-a5FQKWqhhzgRdb1EbQ0oRKt3G2pu40QTr30h6H2lgL3bavvTg9uRflQG43ALGJr0KfVwPK_8R_QDRIW5f</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>1628527925</pqid></control><display><type>article</type><title>Piezoelectric Nanoparticle–Polymer Composite Foams</title><source>MEDLINE</source><source>American Chemical Society Web Editions</source><creator>McCall, William R ; Kim, Kanguk ; Heath, Cory ; La Pierre, Gina ; Sirbuly, Donald J</creator><creatorcontrib>McCall, William R ; Kim, Kanguk ; Heath, Cory ; La Pierre, Gina ; Sirbuly, Donald J</creatorcontrib><description>Piezoelectric polymer composite foams are synthesized using different sugar-templating strategies. By incorporating sugar grains directly into polydimethylsiloxane mixtures containing barium titanate nanoparticles and carbon nanotubes, followed by removal of the sugar after polymer curing, highly compliant materials with excellent piezoelectric properties can be fabricated. Porosities and elasticity are tuned by simply adjusting the sugar/polymer mass ratio which gave an upper bound on the porosity of 73% and a lower bound on the elastic coefficient of 32 kPa. The electrical performance of the foams showed a direct relationship between porosity and the piezoelectric outputs, giving piezoelectric coefficient values of ∼112 pC/N and a power output of ∼18 mW/cm3 under a load of 10 N for the highest porosity samples. These novel materials should find exciting use in a variety of applications including energy scavenging platforms, biosensors, and acoustic actuators.</description><identifier>ISSN: 1944-8244</identifier><identifier>EISSN: 1944-8252</identifier><identifier>DOI: 10.1021/am506415y</identifier><identifier>PMID: 25353687</identifier><language>eng</language><publisher>United States: American Chemical Society</publisher><subject>Barium Compounds - chemistry ; Biosensing Techniques ; Carbohydrates - chemistry ; Nanoparticles - chemistry ; Polymers - chemistry ; Porosity ; Titanium - chemistry</subject><ispartof>ACS applied materials &amp; interfaces, 2014-11, Vol.6 (22), p.19504-19509</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a315t-1e76d7a1581999243a2b28e6f9dcb4d043d1deea751a952ccdb5d32f6f2788d93</citedby><cites>FETCH-LOGICAL-a315t-1e76d7a1581999243a2b28e6f9dcb4d043d1deea751a952ccdb5d32f6f2788d93</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/am506415y$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/am506415y$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>314,780,784,2765,27076,27924,27925,56738,56788</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/25353687$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>McCall, William R</creatorcontrib><creatorcontrib>Kim, Kanguk</creatorcontrib><creatorcontrib>Heath, Cory</creatorcontrib><creatorcontrib>La Pierre, Gina</creatorcontrib><creatorcontrib>Sirbuly, Donald J</creatorcontrib><title>Piezoelectric Nanoparticle–Polymer Composite Foams</title><title>ACS applied materials &amp; interfaces</title><addtitle>ACS Appl. Mater. Interfaces</addtitle><description>Piezoelectric polymer composite foams are synthesized using different sugar-templating strategies. By incorporating sugar grains directly into polydimethylsiloxane mixtures containing barium titanate nanoparticles and carbon nanotubes, followed by removal of the sugar after polymer curing, highly compliant materials with excellent piezoelectric properties can be fabricated. Porosities and elasticity are tuned by simply adjusting the sugar/polymer mass ratio which gave an upper bound on the porosity of 73% and a lower bound on the elastic coefficient of 32 kPa. The electrical performance of the foams showed a direct relationship between porosity and the piezoelectric outputs, giving piezoelectric coefficient values of ∼112 pC/N and a power output of ∼18 mW/cm3 under a load of 10 N for the highest porosity samples. These novel materials should find exciting use in a variety of applications including energy scavenging platforms, biosensors, and acoustic actuators.</description><subject>Barium Compounds - chemistry</subject><subject>Biosensing Techniques</subject><subject>Carbohydrates - chemistry</subject><subject>Nanoparticles - chemistry</subject><subject>Polymers - chemistry</subject><subject>Porosity</subject><subject>Titanium - chemistry</subject><issn>1944-8244</issn><issn>1944-8252</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2014</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNptkL1OwzAURi0EoqUw8AKoCxIMAf8m9ogqCkgVdIDZcuwbKVVcBzsZysQ78IY8CUEtnZjuHY6O9B2Ezgm-IZiSW-MFzjkRmwM0JorzTFJBD_c_5yN0ktIK45xRLI7RiAomWC6LMeLLGj4CNGC7WNvps1mH1sSutg18f34tQ7PxEKez4NuQ6g6m82B8OkVHlWkSnO3uBL3N719nj9ni5eFpdrfIDCOiywgUuSsMEZIopShnhpZUQl4pZ0vuMGeOOABTCGKUoNa6UjhGq7yihZROsQm62nrbGN57SJ32dbLQNGYNoU-a5FQKWqhhzgRdb1EbQ0oRKt3G2pu40QTr30h6H2lgL3bavvTg9uRflQG43ALGJr0KfVwPK_8R_QDRIW5f</recordid><startdate>20141126</startdate><enddate>20141126</enddate><creator>McCall, William R</creator><creator>Kim, Kanguk</creator><creator>Heath, Cory</creator><creator>La Pierre, Gina</creator><creator>Sirbuly, Donald J</creator><general>American Chemical Society</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope></search><sort><creationdate>20141126</creationdate><title>Piezoelectric Nanoparticle–Polymer Composite Foams</title><author>McCall, William R ; Kim, Kanguk ; Heath, Cory ; La Pierre, Gina ; Sirbuly, Donald J</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a315t-1e76d7a1581999243a2b28e6f9dcb4d043d1deea751a952ccdb5d32f6f2788d93</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2014</creationdate><topic>Barium Compounds - chemistry</topic><topic>Biosensing Techniques</topic><topic>Carbohydrates - chemistry</topic><topic>Nanoparticles - chemistry</topic><topic>Polymers - chemistry</topic><topic>Porosity</topic><topic>Titanium - chemistry</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>McCall, William R</creatorcontrib><creatorcontrib>Kim, Kanguk</creatorcontrib><creatorcontrib>Heath, Cory</creatorcontrib><creatorcontrib>La Pierre, Gina</creatorcontrib><creatorcontrib>Sirbuly, Donald J</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><jtitle>ACS applied materials &amp; interfaces</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>McCall, William R</au><au>Kim, Kanguk</au><au>Heath, Cory</au><au>La Pierre, Gina</au><au>Sirbuly, Donald J</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Piezoelectric Nanoparticle–Polymer Composite Foams</atitle><jtitle>ACS applied materials &amp; interfaces</jtitle><addtitle>ACS Appl. Mater. Interfaces</addtitle><date>2014-11-26</date><risdate>2014</risdate><volume>6</volume><issue>22</issue><spage>19504</spage><epage>19509</epage><pages>19504-19509</pages><issn>1944-8244</issn><eissn>1944-8252</eissn><abstract>Piezoelectric polymer composite foams are synthesized using different sugar-templating strategies. By incorporating sugar grains directly into polydimethylsiloxane mixtures containing barium titanate nanoparticles and carbon nanotubes, followed by removal of the sugar after polymer curing, highly compliant materials with excellent piezoelectric properties can be fabricated. Porosities and elasticity are tuned by simply adjusting the sugar/polymer mass ratio which gave an upper bound on the porosity of 73% and a lower bound on the elastic coefficient of 32 kPa. The electrical performance of the foams showed a direct relationship between porosity and the piezoelectric outputs, giving piezoelectric coefficient values of ∼112 pC/N and a power output of ∼18 mW/cm3 under a load of 10 N for the highest porosity samples. These novel materials should find exciting use in a variety of applications including energy scavenging platforms, biosensors, and acoustic actuators.</abstract><cop>United States</cop><pub>American Chemical Society</pub><pmid>25353687</pmid><doi>10.1021/am506415y</doi><tpages>6</tpages></addata></record>
fulltext fulltext
identifier ISSN: 1944-8244
ispartof ACS applied materials & interfaces, 2014-11, Vol.6 (22), p.19504-19509
issn 1944-8244
1944-8252
language eng
recordid cdi_proquest_miscellaneous_1628527925
source MEDLINE; American Chemical Society Web Editions
subjects Barium Compounds - chemistry
Biosensing Techniques
Carbohydrates - chemistry
Nanoparticles - chemistry
Polymers - chemistry
Porosity
Titanium - chemistry
title Piezoelectric Nanoparticle–Polymer Composite Foams
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-03T17%3A11%3A07IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Piezoelectric%20Nanoparticle%E2%80%93Polymer%20Composite%20Foams&rft.jtitle=ACS%20applied%20materials%20&%20interfaces&rft.au=McCall,%20William%20R&rft.date=2014-11-26&rft.volume=6&rft.issue=22&rft.spage=19504&rft.epage=19509&rft.pages=19504-19509&rft.issn=1944-8244&rft.eissn=1944-8252&rft_id=info:doi/10.1021/am506415y&rft_dat=%3Cproquest_cross%3E1628527925%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=1628527925&rft_id=info:pmid/25353687&rfr_iscdi=true