Emission factors from small scale appliances burning wood and pellets
Four manually fed (6–11 kW) firewood burning and two automatic wood pellets (8.8–25 kW) residential heating appliances were tested under real-world operating conditions in order to determine emission factors (EFs) of macropollutants, i.e., carbon monoxide (CO), nitrogen oxides (NOx), non-methane hyd...
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creator | Ozgen, Senem Caserini, Stefano Galante, Silvia Giugliano, Michele Angelino, Elisabetta Marongiu, Alessandro Hugony, Francesca Migliavacca, Gabriele Morreale, Carmen |
description | Four manually fed (6–11 kW) firewood burning and two automatic wood pellets (8.8–25 kW) residential heating appliances were tested under real-world operating conditions in order to determine emission factors (EFs) of macropollutants, i.e., carbon monoxide (CO), nitrogen oxides (NOx), non-methane hydrocarbons (NMHC), particulate matter (PM) and trace pollutants such as polycyclic aromatic hydrocarbons (PAH) and dioxins. The results were examined for the influence of different factors (i.e., type of wood, appliance and combustion cycle). The experimental EFs were also compared with the values proposed by the European emission inventory guidebook used in the local inventory in order to evaluate their representativeness of real world emissions. The composite macropollutant EFs for manually fed appliances were: for CO 5858 g GJ−1, for NOx 122 g GJ−1, NMHC 542 g GJ−1, PM 254 g GJ−1, whereas emissions were much lower for automatic pellets appliances: CO 219 g GJ−1, for NOx 66 g GJ−1, NMHC 5 g GJ−1, PM 85 g GJ−1. The highest emissions were generally observed for the open fireplace, however traditional and advanced stoves have the highest overall CO EFs. Especially for the advanced stove real-world emissions are far worse than those measured under cycles used for type testing of residential solid fuel appliances. No great difference is observed for different firewood types in batch working appliances, diversely the quality of the pellets is observed to influence directly the emission performance of the automatic appliances. Benzo(b)fluoranthene is the PAH with the highest contribution (110 mg GJ−1 for manual appliances and 2 mg GJ−1 for automatic devices) followed by benzo(a)pyrene (77 mg GJ−1 for manual appliances and 0.8 mg GJ−1 for automatic devices).
•About 300 emission factors for 6 appliances and 5 types of wood were measured.•Emissions in real-world operating conditions and standard cycle are compared.•Real cycles double the CO and NMHC emissions with respect to EN cycle averages.•The highest PAH in emission is Benzo(b)fluoranthene, followed by benzo(a)pyrene.•NMHC, NOx and PAH emission from advanced and traditional stoves are comparable. |
doi_str_mv | 10.1016/j.atmosenv.2014.05.032 |
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•About 300 emission factors for 6 appliances and 5 types of wood were measured.•Emissions in real-world operating conditions and standard cycle are compared.•Real cycles double the CO and NMHC emissions with respect to EN cycle averages.•The highest PAH in emission is Benzo(b)fluoranthene, followed by benzo(a)pyrene.•NMHC, NOx and PAH emission from advanced and traditional stoves are comparable.</description><identifier>ISSN: 1352-2310</identifier><identifier>EISSN: 1873-2844</identifier><identifier>DOI: 10.1016/j.atmosenv.2014.05.032</identifier><language>eng</language><publisher>Kidlington: Elsevier Ltd</publisher><subject>Applied sciences ; Atmospheric pollution ; Combustion and energy production ; Combustion cycle ; Emission factor ; Exact sciences and technology ; Fireplaces ; Pellet ; Pollution ; Pollution sources. Measurement results ; Residential wood combustion ; Stoves</subject><ispartof>Atmospheric environment (1994), 2014-09, Vol.94, p.144-153</ispartof><rights>2014 Elsevier Ltd</rights><rights>2015 INIST-CNRS</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c423t-100b485766f743c080553c8e843cf0d0250eab5be120356857e84e62c4a442823</citedby><cites>FETCH-LOGICAL-c423t-100b485766f743c080553c8e843cf0d0250eab5be120356857e84e62c4a442823</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.atmosenv.2014.05.032$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,780,784,3550,27924,27925,45995</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=28615597$$DView record in Pascal Francis$$Hfree_for_read</backlink></links><search><creatorcontrib>Ozgen, Senem</creatorcontrib><creatorcontrib>Caserini, Stefano</creatorcontrib><creatorcontrib>Galante, Silvia</creatorcontrib><creatorcontrib>Giugliano, Michele</creatorcontrib><creatorcontrib>Angelino, Elisabetta</creatorcontrib><creatorcontrib>Marongiu, Alessandro</creatorcontrib><creatorcontrib>Hugony, Francesca</creatorcontrib><creatorcontrib>Migliavacca, Gabriele</creatorcontrib><creatorcontrib>Morreale, Carmen</creatorcontrib><title>Emission factors from small scale appliances burning wood and pellets</title><title>Atmospheric environment (1994)</title><description>Four manually fed (6–11 kW) firewood burning and two automatic wood pellets (8.8–25 kW) residential heating appliances were tested under real-world operating conditions in order to determine emission factors (EFs) of macropollutants, i.e., carbon monoxide (CO), nitrogen oxides (NOx), non-methane hydrocarbons (NMHC), particulate matter (PM) and trace pollutants such as polycyclic aromatic hydrocarbons (PAH) and dioxins. The results were examined for the influence of different factors (i.e., type of wood, appliance and combustion cycle). The experimental EFs were also compared with the values proposed by the European emission inventory guidebook used in the local inventory in order to evaluate their representativeness of real world emissions. The composite macropollutant EFs for manually fed appliances were: for CO 5858 g GJ−1, for NOx 122 g GJ−1, NMHC 542 g GJ−1, PM 254 g GJ−1, whereas emissions were much lower for automatic pellets appliances: CO 219 g GJ−1, for NOx 66 g GJ−1, NMHC 5 g GJ−1, PM 85 g GJ−1. The highest emissions were generally observed for the open fireplace, however traditional and advanced stoves have the highest overall CO EFs. Especially for the advanced stove real-world emissions are far worse than those measured under cycles used for type testing of residential solid fuel appliances. No great difference is observed for different firewood types in batch working appliances, diversely the quality of the pellets is observed to influence directly the emission performance of the automatic appliances. Benzo(b)fluoranthene is the PAH with the highest contribution (110 mg GJ−1 for manual appliances and 2 mg GJ−1 for automatic devices) followed by benzo(a)pyrene (77 mg GJ−1 for manual appliances and 0.8 mg GJ−1 for automatic devices).
•About 300 emission factors for 6 appliances and 5 types of wood were measured.•Emissions in real-world operating conditions and standard cycle are compared.•Real cycles double the CO and NMHC emissions with respect to EN cycle averages.•The highest PAH in emission is Benzo(b)fluoranthene, followed by benzo(a)pyrene.•NMHC, NOx and PAH emission from advanced and traditional stoves are comparable.</description><subject>Applied sciences</subject><subject>Atmospheric pollution</subject><subject>Combustion and energy production</subject><subject>Combustion cycle</subject><subject>Emission factor</subject><subject>Exact sciences and technology</subject><subject>Fireplaces</subject><subject>Pellet</subject><subject>Pollution</subject><subject>Pollution sources. Measurement results</subject><subject>Residential wood combustion</subject><subject>Stoves</subject><issn>1352-2310</issn><issn>1873-2844</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2014</creationdate><recordtype>article</recordtype><recordid>eNqFkE1r3DAQhk1JoJs0fyHoUsjFzujT2ltL2KSBhV7as9DK46DFtlyNd0P_fbXstteeJDHPaOZ9quqeQ8OBm8d945cxEU7HRgBXDegGpPhQrbhtZS2sUlflLrWoheTwsboh2gOAbNftqtpsxkgU08R6H5aUifU5jYxGPwyMgh-Q-Xkeop8CEtsd8hSnN_aeUsf81LEZhwEX-lRd934gvLuct9XP582Pp2_19vvL69PXbR2UkEvNAXbK6taYvlUygAWtZbBoy6OHDoQG9Du9Qy5AalPIUkIjgvJKCSvkbfVw_nfO6dcBaXFl-1B28BOmAzluRLs2Zm1lQc0ZDTkRZezdnOPo82_HwZ28ub37682dvDnQrngrjZ8vM_wpf59L9Ej_uoU1XOt1W7gvZw5L4GPE7ChELJq6mDEsrkvxf6P-AC10hgg</recordid><startdate>20140901</startdate><enddate>20140901</enddate><creator>Ozgen, Senem</creator><creator>Caserini, Stefano</creator><creator>Galante, Silvia</creator><creator>Giugliano, Michele</creator><creator>Angelino, Elisabetta</creator><creator>Marongiu, Alessandro</creator><creator>Hugony, Francesca</creator><creator>Migliavacca, Gabriele</creator><creator>Morreale, Carmen</creator><general>Elsevier Ltd</general><general>Elsevier</general><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7ST</scope><scope>7TG</scope><scope>7TV</scope><scope>7UA</scope><scope>C1K</scope><scope>F1W</scope><scope>H96</scope><scope>KL.</scope><scope>L.G</scope><scope>SOI</scope></search><sort><creationdate>20140901</creationdate><title>Emission factors from small scale appliances burning wood and pellets</title><author>Ozgen, Senem ; Caserini, Stefano ; Galante, Silvia ; Giugliano, Michele ; Angelino, Elisabetta ; Marongiu, Alessandro ; Hugony, Francesca ; Migliavacca, Gabriele ; Morreale, Carmen</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c423t-100b485766f743c080553c8e843cf0d0250eab5be120356857e84e62c4a442823</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2014</creationdate><topic>Applied sciences</topic><topic>Atmospheric pollution</topic><topic>Combustion and energy production</topic><topic>Combustion cycle</topic><topic>Emission factor</topic><topic>Exact sciences and technology</topic><topic>Fireplaces</topic><topic>Pellet</topic><topic>Pollution</topic><topic>Pollution sources. Measurement results</topic><topic>Residential wood combustion</topic><topic>Stoves</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Ozgen, Senem</creatorcontrib><creatorcontrib>Caserini, Stefano</creatorcontrib><creatorcontrib>Galante, Silvia</creatorcontrib><creatorcontrib>Giugliano, Michele</creatorcontrib><creatorcontrib>Angelino, Elisabetta</creatorcontrib><creatorcontrib>Marongiu, Alessandro</creatorcontrib><creatorcontrib>Hugony, Francesca</creatorcontrib><creatorcontrib>Migliavacca, Gabriele</creatorcontrib><creatorcontrib>Morreale, Carmen</creatorcontrib><collection>Pascal-Francis</collection><collection>CrossRef</collection><collection>Environment Abstracts</collection><collection>Meteorological & Geoastrophysical Abstracts</collection><collection>Pollution Abstracts</collection><collection>Water Resources Abstracts</collection><collection>Environmental Sciences and Pollution Management</collection><collection>ASFA: Aquatic Sciences and Fisheries Abstracts</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) 2: Ocean Technology, Policy & Non-Living Resources</collection><collection>Meteorological & Geoastrophysical Abstracts - Academic</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) Professional</collection><collection>Environment Abstracts</collection><jtitle>Atmospheric environment (1994)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Ozgen, Senem</au><au>Caserini, Stefano</au><au>Galante, Silvia</au><au>Giugliano, Michele</au><au>Angelino, Elisabetta</au><au>Marongiu, Alessandro</au><au>Hugony, Francesca</au><au>Migliavacca, Gabriele</au><au>Morreale, Carmen</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Emission factors from small scale appliances burning wood and pellets</atitle><jtitle>Atmospheric environment (1994)</jtitle><date>2014-09-01</date><risdate>2014</risdate><volume>94</volume><spage>144</spage><epage>153</epage><pages>144-153</pages><issn>1352-2310</issn><eissn>1873-2844</eissn><abstract>Four manually fed (6–11 kW) firewood burning and two automatic wood pellets (8.8–25 kW) residential heating appliances were tested under real-world operating conditions in order to determine emission factors (EFs) of macropollutants, i.e., carbon monoxide (CO), nitrogen oxides (NOx), non-methane hydrocarbons (NMHC), particulate matter (PM) and trace pollutants such as polycyclic aromatic hydrocarbons (PAH) and dioxins. The results were examined for the influence of different factors (i.e., type of wood, appliance and combustion cycle). The experimental EFs were also compared with the values proposed by the European emission inventory guidebook used in the local inventory in order to evaluate their representativeness of real world emissions. The composite macropollutant EFs for manually fed appliances were: for CO 5858 g GJ−1, for NOx 122 g GJ−1, NMHC 542 g GJ−1, PM 254 g GJ−1, whereas emissions were much lower for automatic pellets appliances: CO 219 g GJ−1, for NOx 66 g GJ−1, NMHC 5 g GJ−1, PM 85 g GJ−1. The highest emissions were generally observed for the open fireplace, however traditional and advanced stoves have the highest overall CO EFs. Especially for the advanced stove real-world emissions are far worse than those measured under cycles used for type testing of residential solid fuel appliances. No great difference is observed for different firewood types in batch working appliances, diversely the quality of the pellets is observed to influence directly the emission performance of the automatic appliances. Benzo(b)fluoranthene is the PAH with the highest contribution (110 mg GJ−1 for manual appliances and 2 mg GJ−1 for automatic devices) followed by benzo(a)pyrene (77 mg GJ−1 for manual appliances and 0.8 mg GJ−1 for automatic devices).
•About 300 emission factors for 6 appliances and 5 types of wood were measured.•Emissions in real-world operating conditions and standard cycle are compared.•Real cycles double the CO and NMHC emissions with respect to EN cycle averages.•The highest PAH in emission is Benzo(b)fluoranthene, followed by benzo(a)pyrene.•NMHC, NOx and PAH emission from advanced and traditional stoves are comparable.</abstract><cop>Kidlington</cop><pub>Elsevier Ltd</pub><doi>10.1016/j.atmosenv.2014.05.032</doi><tpages>10</tpages><oa>free_for_read</oa></addata></record> |
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subjects | Applied sciences Atmospheric pollution Combustion and energy production Combustion cycle Emission factor Exact sciences and technology Fireplaces Pellet Pollution Pollution sources. Measurement results Residential wood combustion Stoves |
title | Emission factors from small scale appliances burning wood and pellets |
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