Occurrence of Polychlorinated Diphenyl Sulfides (PCDPSs) in Surface Sediments and Surface Water from the Nanjing Section of the Yangtze River
Polychlorinated diphenyl sulfides (PCDPSs) are dioxin-like compounds that could induce various adverse effects to organisms. However, little is known about the occurrence of PCDPSs in the riverine environment. In the present study, the concentrations of twenty-one types of PCDPSs in the surface sedi...
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| Veröffentlicht in: | Environmental science & technology 2014-10, Vol.48 (19), p.11429-11436 |
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| creator | Zhang, Xuesheng Qin, Li Qu, Ruijuan Feng, Mingbao Wei, Zhongbo Wang, Liansheng Wang, Zunyao |
| description | Polychlorinated diphenyl sulfides (PCDPSs) are dioxin-like compounds that could induce various adverse effects to organisms. However, little is known about the occurrence of PCDPSs in the riverine environment. In the present study, the concentrations of twenty-one types of PCDPSs in the surface sediments and in surface water from the Nanjing section of the Yangtze River were examined. A total of 19 types of PCDPSs were detected and ∑PCDPSs concentrations in surface sediment and surface water ranged from 0.10 to 6.90 ng/g and 0.18 to 2.03 ng/L, respectively. The 2,2′,4,4′,5-penta-CDPS was the dominant congener in sediment (19.9%) and 2,2′,3,3′-tetra-CDPS was the most abundant congener in water (12.2%). The tetra-CDPSs were the dominant congeners both in sediment and in water. Compared with sediment, the percentage of lower chlorinated PCDPSs in water increased distinctly. Source analysis revealed that the PCDPSs in the sediment and in the water mainly came from chemical wastewater rather than domestic sewage. There was a significant linear correlation between ∑PCDPS concentrations and sediment TOC contents, while no linear correlation existed between ∑PCDPS concentrations and water DOC contents. This study demonstrated the prevalent contamination by PCDPSs in sediments and in water from the Nanjing section of the Yangtze River. |
| doi_str_mv | 10.1021/es502197b |
| format | Article |
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However, little is known about the occurrence of PCDPSs in the riverine environment. In the present study, the concentrations of twenty-one types of PCDPSs in the surface sediments and in surface water from the Nanjing section of the Yangtze River were examined. A total of 19 types of PCDPSs were detected and ∑PCDPSs concentrations in surface sediment and surface water ranged from 0.10 to 6.90 ng/g and 0.18 to 2.03 ng/L, respectively. The 2,2′,4,4′,5-penta-CDPS was the dominant congener in sediment (19.9%) and 2,2′,3,3′-tetra-CDPS was the most abundant congener in water (12.2%). The tetra-CDPSs were the dominant congeners both in sediment and in water. Compared with sediment, the percentage of lower chlorinated PCDPSs in water increased distinctly. Source analysis revealed that the PCDPSs in the sediment and in the water mainly came from chemical wastewater rather than domestic sewage. There was a significant linear correlation between ∑PCDPS concentrations and sediment TOC contents, while no linear correlation existed between ∑PCDPS concentrations and water DOC contents. This study demonstrated the prevalent contamination by PCDPSs in sediments and in water from the Nanjing section of the Yangtze River.</description><identifier>ISSN: 0013-936X</identifier><identifier>EISSN: 1520-5851</identifier><identifier>DOI: 10.1021/es502197b</identifier><identifier>PMID: 25168171</identifier><identifier>CODEN: ESTHAG</identifier><language>eng</language><publisher>Washington, DC: American Chemical Society</publisher><subject>Analytical chemistry ; Applied sciences ; Chemical compounds ; China ; Comparative analysis ; Contamination ; Continental surface waters ; Earth sciences ; Earth, ocean, space ; Engineering and environment geology. Geothermics ; Environmental Monitoring ; Exact sciences and technology ; Geologic Sediments - analysis ; Natural water pollution ; Pollution ; Pollution, environment geology ; Rivers - chemistry ; Sediment transport ; Sediments ; Sulfides - analysis ; Surface water ; Waste Water ; Water Pollutants, Chemical - analysis ; Water treatment ; Water treatment and pollution</subject><ispartof>Environmental science & technology, 2014-10, Vol.48 (19), p.11429-11436</ispartof><rights>2015 INIST-CNRS</rights><rights>Copyright American Chemical Society Oct 7, 2014</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a406t-1664ad57969f1cd72840b9050dc2399c040b0a294e29f3f91e11c65ac3f288623</citedby><cites>FETCH-LOGICAL-a406t-1664ad57969f1cd72840b9050dc2399c040b0a294e29f3f91e11c65ac3f288623</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/es502197b$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/es502197b$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>314,780,784,2756,27067,27915,27916,56729,56779</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=28919802$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/25168171$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Zhang, Xuesheng</creatorcontrib><creatorcontrib>Qin, Li</creatorcontrib><creatorcontrib>Qu, Ruijuan</creatorcontrib><creatorcontrib>Feng, Mingbao</creatorcontrib><creatorcontrib>Wei, Zhongbo</creatorcontrib><creatorcontrib>Wang, Liansheng</creatorcontrib><creatorcontrib>Wang, Zunyao</creatorcontrib><title>Occurrence of Polychlorinated Diphenyl Sulfides (PCDPSs) in Surface Sediments and Surface Water from the Nanjing Section of the Yangtze River</title><title>Environmental science & technology</title><addtitle>Environ. Sci. Technol</addtitle><description>Polychlorinated diphenyl sulfides (PCDPSs) are dioxin-like compounds that could induce various adverse effects to organisms. However, little is known about the occurrence of PCDPSs in the riverine environment. In the present study, the concentrations of twenty-one types of PCDPSs in the surface sediments and in surface water from the Nanjing section of the Yangtze River were examined. A total of 19 types of PCDPSs were detected and ∑PCDPSs concentrations in surface sediment and surface water ranged from 0.10 to 6.90 ng/g and 0.18 to 2.03 ng/L, respectively. The 2,2′,4,4′,5-penta-CDPS was the dominant congener in sediment (19.9%) and 2,2′,3,3′-tetra-CDPS was the most abundant congener in water (12.2%). The tetra-CDPSs were the dominant congeners both in sediment and in water. Compared with sediment, the percentage of lower chlorinated PCDPSs in water increased distinctly. Source analysis revealed that the PCDPSs in the sediment and in the water mainly came from chemical wastewater rather than domestic sewage. There was a significant linear correlation between ∑PCDPS concentrations and sediment TOC contents, while no linear correlation existed between ∑PCDPS concentrations and water DOC contents. This study demonstrated the prevalent contamination by PCDPSs in sediments and in water from the Nanjing section of the Yangtze River.</description><subject>Analytical chemistry</subject><subject>Applied sciences</subject><subject>Chemical compounds</subject><subject>China</subject><subject>Comparative analysis</subject><subject>Contamination</subject><subject>Continental surface waters</subject><subject>Earth sciences</subject><subject>Earth, ocean, space</subject><subject>Engineering and environment geology. Geothermics</subject><subject>Environmental Monitoring</subject><subject>Exact sciences and technology</subject><subject>Geologic Sediments - analysis</subject><subject>Natural water pollution</subject><subject>Pollution</subject><subject>Pollution, environment geology</subject><subject>Rivers - chemistry</subject><subject>Sediment transport</subject><subject>Sediments</subject><subject>Sulfides - analysis</subject><subject>Surface water</subject><subject>Waste Water</subject><subject>Water Pollutants, Chemical - analysis</subject><subject>Water treatment</subject><subject>Water treatment and pollution</subject><issn>0013-936X</issn><issn>1520-5851</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2014</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqN0c2O0zAQB3ALgdiycOAFkCWEtHsIzDiJEx9Rly9pxVYUBJwi1xlvXaVOsROk8g68M462dBFcOI08-nnG1p-xxwjPEQS-oFimoqrVHTbDUkBW1iXeZTMAzDOVyy8n7EGMGwAQOdT32YkoUdZY4Yz9vDJmDIG8Id5bvui7vVl3fXBeD9TyC7dbk993fDl21rUU-dlifrFYxnPufGoGq9PFJbVuS36IXPv22P2cJgRuQ7_lw5r4e-03zl8nbAbX-2nb1P6q_fXwg_gH953CQ3bP6i7So0M9ZZ9ev_o4f5tdXr15N395mekC5JChlIVuy0pJZdG0lagLWCkooTUiV8pAOoIWqiChbG4VEqKRpTa5FXUtRX7Kzm7m7kL_baQ4NFsXDXWd9tSPsUEphIRSFfAfFFQOssKJPv2Lbvox-PSRpLCoZSVhUuc3yoQ-xkC22QW31WHfIDRTnM0xzmSfHCaOqy21R_k7vwSeHYCORnc2aG9cvHW1QlWDuHXaxD9e9c_CX1TnsWk</recordid><startdate>20141007</startdate><enddate>20141007</enddate><creator>Zhang, Xuesheng</creator><creator>Qin, Li</creator><creator>Qu, Ruijuan</creator><creator>Feng, Mingbao</creator><creator>Wei, Zhongbo</creator><creator>Wang, Liansheng</creator><creator>Wang, Zunyao</creator><general>American Chemical Society</general><scope>IQODW</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7QO</scope><scope>7ST</scope><scope>7T7</scope><scope>7U7</scope><scope>8FD</scope><scope>C1K</scope><scope>FR3</scope><scope>P64</scope><scope>SOI</scope><scope>7X8</scope><scope>7QH</scope><scope>7TG</scope><scope>7UA</scope><scope>F1W</scope><scope>H97</scope><scope>KL.</scope><scope>L.G</scope></search><sort><creationdate>20141007</creationdate><title>Occurrence of Polychlorinated Diphenyl Sulfides (PCDPSs) in Surface Sediments and Surface Water from the Nanjing Section of the Yangtze River</title><author>Zhang, Xuesheng ; Qin, Li ; Qu, Ruijuan ; Feng, Mingbao ; Wei, Zhongbo ; Wang, Liansheng ; Wang, Zunyao</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a406t-1664ad57969f1cd72840b9050dc2399c040b0a294e29f3f91e11c65ac3f288623</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2014</creationdate><topic>Analytical chemistry</topic><topic>Applied sciences</topic><topic>Chemical compounds</topic><topic>China</topic><topic>Comparative analysis</topic><topic>Contamination</topic><topic>Continental surface waters</topic><topic>Earth sciences</topic><topic>Earth, ocean, space</topic><topic>Engineering and environment geology. Geothermics</topic><topic>Environmental Monitoring</topic><topic>Exact sciences and technology</topic><topic>Geologic Sediments - analysis</topic><topic>Natural water pollution</topic><topic>Pollution</topic><topic>Pollution, environment geology</topic><topic>Rivers - chemistry</topic><topic>Sediment transport</topic><topic>Sediments</topic><topic>Sulfides - analysis</topic><topic>Surface water</topic><topic>Waste Water</topic><topic>Water Pollutants, Chemical - analysis</topic><topic>Water treatment</topic><topic>Water treatment and pollution</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhang, Xuesheng</creatorcontrib><creatorcontrib>Qin, Li</creatorcontrib><creatorcontrib>Qu, Ruijuan</creatorcontrib><creatorcontrib>Feng, Mingbao</creatorcontrib><creatorcontrib>Wei, Zhongbo</creatorcontrib><creatorcontrib>Wang, Liansheng</creatorcontrib><creatorcontrib>Wang, Zunyao</creatorcontrib><collection>Pascal-Francis</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>Biotechnology Research Abstracts</collection><collection>Environment Abstracts</collection><collection>Industrial and Applied Microbiology Abstracts (Microbiology A)</collection><collection>Toxicology Abstracts</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Engineering Research Database</collection><collection>Biotechnology and BioEngineering Abstracts</collection><collection>Environment Abstracts</collection><collection>MEDLINE - Academic</collection><collection>Aqualine</collection><collection>Meteorological & Geoastrophysical Abstracts</collection><collection>Water Resources Abstracts</collection><collection>ASFA: Aquatic Sciences and Fisheries Abstracts</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) 3: Aquatic Pollution & Environmental Quality</collection><collection>Meteorological & Geoastrophysical Abstracts - Academic</collection><collection>Aquatic Science & Fisheries Abstracts (ASFA) Professional</collection><jtitle>Environmental science & technology</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zhang, Xuesheng</au><au>Qin, Li</au><au>Qu, Ruijuan</au><au>Feng, Mingbao</au><au>Wei, Zhongbo</au><au>Wang, Liansheng</au><au>Wang, Zunyao</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Occurrence of Polychlorinated Diphenyl Sulfides (PCDPSs) in Surface Sediments and Surface Water from the Nanjing Section of the Yangtze River</atitle><jtitle>Environmental science & technology</jtitle><addtitle>Environ. Sci. Technol</addtitle><date>2014-10-07</date><risdate>2014</risdate><volume>48</volume><issue>19</issue><spage>11429</spage><epage>11436</epage><pages>11429-11436</pages><issn>0013-936X</issn><eissn>1520-5851</eissn><coden>ESTHAG</coden><abstract>Polychlorinated diphenyl sulfides (PCDPSs) are dioxin-like compounds that could induce various adverse effects to organisms. However, little is known about the occurrence of PCDPSs in the riverine environment. In the present study, the concentrations of twenty-one types of PCDPSs in the surface sediments and in surface water from the Nanjing section of the Yangtze River were examined. A total of 19 types of PCDPSs were detected and ∑PCDPSs concentrations in surface sediment and surface water ranged from 0.10 to 6.90 ng/g and 0.18 to 2.03 ng/L, respectively. The 2,2′,4,4′,5-penta-CDPS was the dominant congener in sediment (19.9%) and 2,2′,3,3′-tetra-CDPS was the most abundant congener in water (12.2%). The tetra-CDPSs were the dominant congeners both in sediment and in water. Compared with sediment, the percentage of lower chlorinated PCDPSs in water increased distinctly. Source analysis revealed that the PCDPSs in the sediment and in the water mainly came from chemical wastewater rather than domestic sewage. There was a significant linear correlation between ∑PCDPS concentrations and sediment TOC contents, while no linear correlation existed between ∑PCDPS concentrations and water DOC contents. This study demonstrated the prevalent contamination by PCDPSs in sediments and in water from the Nanjing section of the Yangtze River.</abstract><cop>Washington, DC</cop><pub>American Chemical Society</pub><pmid>25168171</pmid><doi>10.1021/es502197b</doi><tpages>8</tpages></addata></record> |
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| ispartof | Environmental science & technology, 2014-10, Vol.48 (19), p.11429-11436 |
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| subjects | Analytical chemistry Applied sciences Chemical compounds China Comparative analysis Contamination Continental surface waters Earth sciences Earth, ocean, space Engineering and environment geology. Geothermics Environmental Monitoring Exact sciences and technology Geologic Sediments - analysis Natural water pollution Pollution Pollution, environment geology Rivers - chemistry Sediment transport Sediments Sulfides - analysis Surface water Waste Water Water Pollutants, Chemical - analysis Water treatment Water treatment and pollution |
| title | Occurrence of Polychlorinated Diphenyl Sulfides (PCDPSs) in Surface Sediments and Surface Water from the Nanjing Section of the Yangtze River |
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