Simultaneous two and three photon resonant enhancement of third-order NLO susceptibility in an azo-dye functionalized polymer film
We report the observation of simultaneous two and three photon resonances, enhancing the third-order NLO susceptibility in a thin film of an azo-dye polymer. The possibility of 2-3 orders of magnitude increase in χ((3)) susceptibility is sustained by quantum mechanical calculations. This improves th...
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Veröffentlicht in: | Physical chemistry chemical physics : PCCP 2013-01, Vol.15 (19), p.7060-7063 |
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container_title | Physical chemistry chemical physics : PCCP |
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creator | JERCA, Florica Adriana JERCA, Valentin Victor KAJZAR, Francois MANEA, Ana Maria RAU, Ileana MIRCEA VULUGA, Dumitru |
description | We report the observation of simultaneous two and three photon resonances, enhancing the third-order NLO susceptibility in a thin film of an azo-dye polymer. The possibility of 2-3 orders of magnitude increase in χ((3)) susceptibility is sustained by quantum mechanical calculations. This improves the applications of azo-polymers in all optical signal processing as well as in nonlinear optical imaging. |
doi_str_mv | 10.1039/c3cp50547b |
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The possibility of 2-3 orders of magnitude increase in χ((3)) susceptibility is sustained by quantum mechanical calculations. 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The possibility of 2-3 orders of magnitude increase in χ((3)) susceptibility is sustained by quantum mechanical calculations. This improves the applications of azo-polymers in all optical signal processing as well as in nonlinear optical imaging.</abstract><cop>Cambridge</cop><pub>Royal Society of Chemistry</pub><pmid>23576205</pmid><doi>10.1039/c3cp50547b</doi><tpages>4</tpages></addata></record> |
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source | Royal Society Of Chemistry Journals 2008-; Alma/SFX Local Collection |
subjects | Applied sciences Exact sciences and technology Forms of application and semi-finished materials Mathematical analysis Nonlinearity Optical data processing Photons Physical chemistry Polymer industry, paints, wood Polymeric films Quantum mechanics Sheets and films Technology of polymers Thin films |
title | Simultaneous two and three photon resonant enhancement of third-order NLO susceptibility in an azo-dye functionalized polymer film |
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