Beyond the Active Site: The Impact of the Outer Coordination Sphere on Electrocatalysts for Hydrogen Production and Oxidation

Conspectus Redox active metalloenzymes play a major role in energy transformation reactions in biological systems. Examples include formate dehydrogenases, nitrogenases, CO dehydrogenase, and hydrogenases. Many of these reactions are also of interest to humans as potential energy storage or utilizat...

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Veröffentlicht in:	Accounts of Chemical Research 2014-08, Vol.47 (8), p.2621-2630
Hauptverfasser:	Ginovska-Pangovska, Bojana, Dutta, Arnab, Reback, Matthew L, Linehan, John C, Shaw, Wendy J
Format:	Artikel
Sprache:	eng
Schlagworte:	Amino Acids - chemistry Biocompatible Materials - chemistry Catalysis catalysis (homogeneous), catalysis (heterogeneous), solar (fuels), bio-inspired, energy storage (including batteries and capacitors), hydrogen and fuel cells, charge transport, materials and chemistry by design, synthesis (novel materials) Catalytic Domain Coordination Complexes - chemistry Crystallography, X-Ray Hydrogen - chemistry Hydrogen - metabolism Hydrogen-Ion Concentration Molecular Conformation Nickel - chemistry Oxidation-Reduction Oxidoreductases - chemistry Oxidoreductases - metabolism Protons
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