Two-pulse field-free orientation reveals anisotropy of molecular shape resonance

We report the observation of macroscopic field-free orientation, i.e., more than 73% of CO molecules pointing in the same direction. This is achieved through an all-optical scheme operating at high particle densities (>10(17)  cm(-3)) that combines one-color (ω) and two-color (ω+2ω) nonresonant f...

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Veröffentlicht in:	Physical review letters 2014-07, Vol.113 (2), p.023001-023001, Article 023001
Hauptverfasser:	Kraus, P M, Baykusheva, D, Wörner, H J
Format:	Artikel
Sprache:	eng
Online-Zugang:	Volltext
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