Aqueous-Solution Route to Zinc Telluride Films for Application to CO2 Reduction
As a photocathode for CO2 reduction, zinc‐blende zinc telluride (ZnTe) was directly formed on a Zn/ZnO nanowire substrate by a simple dissolution–recrystallization mechanism without any surfactant. With the most negative conduction‐band edge among p‐type semiconductors, this new photocatalyst showed...
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| Veröffentlicht in: | Angewandte Chemie International Edition 2014-06, Vol.53 (23), p.5852-5857 |
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| container_issue | 23 |
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| container_title | Angewandte Chemie International Edition |
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| creator | Jang, Ji-Wook Cho, Seungho Magesh, Ganesan Jang, Youn Jeong Kim, Jae Young Kim, Won Yong Seo, Jeong Kon Kim, Sungjee Lee, Kun-Hong Lee, Jae Sung |
| description | As a photocathode for CO2 reduction, zinc‐blende zinc telluride (ZnTe) was directly formed on a Zn/ZnO nanowire substrate by a simple dissolution–recrystallization mechanism without any surfactant. With the most negative conduction‐band edge among p‐type semiconductors, this new photocatalyst showed efficient and stable CO formation in photoelectrochemical CO2 reduction at −0.2–−0.7 V versus RHE without a sacrificial reagent.
High performance without sacrifice: Zinc‐blende zinc telluride (ZnTe) was directly formed on a Zn/ZnO‐nanowire substrate by a simple dissolution–recrystallization mechanism without a surfactant. The ZnTe electrode was applied as a photocathode for CO2 reduction (see picture) and showed efficient and stable CO formation at −0.2–−0.7 V versus the reversible hydrogen electrode (RHE) without a sacrificial reagent. |
| doi_str_mv | 10.1002/anie.201310461 |
| format | Article |
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High performance without sacrifice: Zinc‐blende zinc telluride (ZnTe) was directly formed on a Zn/ZnO‐nanowire substrate by a simple dissolution–recrystallization mechanism without a surfactant. The ZnTe electrode was applied as a photocathode for CO2 reduction (see picture) and showed efficient and stable CO formation at −0.2–−0.7 V versus the reversible hydrogen electrode (RHE) without a sacrificial reagent.</description><edition>International ed. in English</edition><identifier>ISSN: 1433-7851</identifier><identifier>EISSN: 1521-3773</identifier><identifier>DOI: 10.1002/anie.201310461</identifier><identifier>PMID: 24740478</identifier><identifier>CODEN: ACIEAY</identifier><language>eng</language><publisher>Weinheim: WILEY-VCH Verlag</publisher><subject>artificial photosynthesis ; photocathodes ; photoelectrochemical CO2 reduction ; Semiconductors ; solution synthesis ; Zinc telluride</subject><ispartof>Angewandte Chemie International Edition, 2014-06, Vol.53 (23), p.5852-5857</ispartof><rights>2014 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim</rights><rights>2014 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.</rights><rights>2014 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1002%2Fanie.201310461$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1002%2Fanie.201310461$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>314,776,780,1411,27901,27902,45550,45551</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/24740478$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Jang, Ji-Wook</creatorcontrib><creatorcontrib>Cho, Seungho</creatorcontrib><creatorcontrib>Magesh, Ganesan</creatorcontrib><creatorcontrib>Jang, Youn Jeong</creatorcontrib><creatorcontrib>Kim, Jae Young</creatorcontrib><creatorcontrib>Kim, Won Yong</creatorcontrib><creatorcontrib>Seo, Jeong Kon</creatorcontrib><creatorcontrib>Kim, Sungjee</creatorcontrib><creatorcontrib>Lee, Kun-Hong</creatorcontrib><creatorcontrib>Lee, Jae Sung</creatorcontrib><title>Aqueous-Solution Route to Zinc Telluride Films for Application to CO2 Reduction</title><title>Angewandte Chemie International Edition</title><addtitle>Angew. Chem. Int. Ed</addtitle><description>As a photocathode for CO2 reduction, zinc‐blende zinc telluride (ZnTe) was directly formed on a Zn/ZnO nanowire substrate by a simple dissolution–recrystallization mechanism without any surfactant. With the most negative conduction‐band edge among p‐type semiconductors, this new photocatalyst showed efficient and stable CO formation in photoelectrochemical CO2 reduction at −0.2–−0.7 V versus RHE without a sacrificial reagent.
High performance without sacrifice: Zinc‐blende zinc telluride (ZnTe) was directly formed on a Zn/ZnO‐nanowire substrate by a simple dissolution–recrystallization mechanism without a surfactant. The ZnTe electrode was applied as a photocathode for CO2 reduction (see picture) and showed efficient and stable CO formation at −0.2–−0.7 V versus the reversible hydrogen electrode (RHE) without a sacrificial reagent.</description><subject>artificial photosynthesis</subject><subject>photocathodes</subject><subject>photoelectrochemical CO2 reduction</subject><subject>Semiconductors</subject><subject>solution synthesis</subject><subject>Zinc telluride</subject><issn>1433-7851</issn><issn>1521-3773</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2014</creationdate><recordtype>article</recordtype><recordid>eNpdkUlPwzAQhS0EolC4ckSRuHBJGW-xe4xCN6lqpVKE1IvlpA5ySZOSRdB_j0NLD5xsj783mjcPoTsMPQxAnnRuTY8AphhYgM_QFeYE-1QIeu7ujFJfSI476LqqNo6XEoJL1CFMMGBCXqF5-NmYoqn8lyJralvk3qJoauPVhbeyeeItTZY1pV0bb2izbeWlRemFu11mE_1LOy6aE29h1k3SFm7QRaqzytwezy56HQ6W0difzkeTKJz67zQA7PM0jhMB0hihieCGg5CxjiUJBHUAYCYli4GsCddpyhhgiMFQHjPDGROEdtHjoe-uLJyDqlZbWyVuWJ23dhTm1JmUTIBDH_6hm6IpczddSwEJ-lK2De-PVBNvzVrtSrvV5V79rcoB_QPwZTOzP_1jUG0Qqg1CnYJQ4WwyOL2c1j9obVWb75NWlx_KGRZcvc1GKuLj0fK5v1JAfwBQLohK</recordid><startdate>20140602</startdate><enddate>20140602</enddate><creator>Jang, Ji-Wook</creator><creator>Cho, Seungho</creator><creator>Magesh, Ganesan</creator><creator>Jang, Youn Jeong</creator><creator>Kim, Jae Young</creator><creator>Kim, Won Yong</creator><creator>Seo, Jeong Kon</creator><creator>Kim, Sungjee</creator><creator>Lee, Kun-Hong</creator><creator>Lee, Jae Sung</creator><general>WILEY-VCH Verlag</general><general>WILEY‐VCH Verlag</general><general>Wiley Subscription Services, Inc</general><scope>BSCLL</scope><scope>NPM</scope><scope>7TM</scope><scope>K9.</scope><scope>7X8</scope></search><sort><creationdate>20140602</creationdate><title>Aqueous-Solution Route to Zinc Telluride Films for Application to CO2 Reduction</title><author>Jang, Ji-Wook ; Cho, Seungho ; Magesh, Ganesan ; Jang, Youn Jeong ; Kim, Jae Young ; Kim, Won Yong ; Seo, Jeong Kon ; Kim, Sungjee ; Lee, Kun-Hong ; Lee, Jae Sung</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-g3601-5fbbc708ee7a275e5078bab82673360014884b02d25aff44010b0e35b4e544723</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2014</creationdate><topic>artificial photosynthesis</topic><topic>photocathodes</topic><topic>photoelectrochemical CO2 reduction</topic><topic>Semiconductors</topic><topic>solution synthesis</topic><topic>Zinc telluride</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Jang, Ji-Wook</creatorcontrib><creatorcontrib>Cho, Seungho</creatorcontrib><creatorcontrib>Magesh, Ganesan</creatorcontrib><creatorcontrib>Jang, Youn Jeong</creatorcontrib><creatorcontrib>Kim, Jae Young</creatorcontrib><creatorcontrib>Kim, Won Yong</creatorcontrib><creatorcontrib>Seo, Jeong Kon</creatorcontrib><creatorcontrib>Kim, Sungjee</creatorcontrib><creatorcontrib>Lee, Kun-Hong</creatorcontrib><creatorcontrib>Lee, Jae Sung</creatorcontrib><collection>Istex</collection><collection>PubMed</collection><collection>Nucleic Acids Abstracts</collection><collection>ProQuest Health & Medical Complete (Alumni)</collection><collection>MEDLINE - Academic</collection><jtitle>Angewandte Chemie International Edition</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Jang, Ji-Wook</au><au>Cho, Seungho</au><au>Magesh, Ganesan</au><au>Jang, Youn Jeong</au><au>Kim, Jae Young</au><au>Kim, Won Yong</au><au>Seo, Jeong Kon</au><au>Kim, Sungjee</au><au>Lee, Kun-Hong</au><au>Lee, Jae Sung</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Aqueous-Solution Route to Zinc Telluride Films for Application to CO2 Reduction</atitle><jtitle>Angewandte Chemie International Edition</jtitle><addtitle>Angew. Chem. Int. Ed</addtitle><date>2014-06-02</date><risdate>2014</risdate><volume>53</volume><issue>23</issue><spage>5852</spage><epage>5857</epage><pages>5852-5857</pages><issn>1433-7851</issn><eissn>1521-3773</eissn><coden>ACIEAY</coden><abstract>As a photocathode for CO2 reduction, zinc‐blende zinc telluride (ZnTe) was directly formed on a Zn/ZnO nanowire substrate by a simple dissolution–recrystallization mechanism without any surfactant. With the most negative conduction‐band edge among p‐type semiconductors, this new photocatalyst showed efficient and stable CO formation in photoelectrochemical CO2 reduction at −0.2–−0.7 V versus RHE without a sacrificial reagent.
High performance without sacrifice: Zinc‐blende zinc telluride (ZnTe) was directly formed on a Zn/ZnO‐nanowire substrate by a simple dissolution–recrystallization mechanism without a surfactant. The ZnTe electrode was applied as a photocathode for CO2 reduction (see picture) and showed efficient and stable CO formation at −0.2–−0.7 V versus the reversible hydrogen electrode (RHE) without a sacrificial reagent.</abstract><cop>Weinheim</cop><pub>WILEY-VCH Verlag</pub><pmid>24740478</pmid><doi>10.1002/anie.201310461</doi><tpages>6</tpages><edition>International ed. in English</edition></addata></record> |
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| subjects | artificial photosynthesis photocathodes photoelectrochemical CO2 reduction Semiconductors solution synthesis Zinc telluride |
| title | Aqueous-Solution Route to Zinc Telluride Films for Application to CO2 Reduction |
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