Interfacial interactions between an alkali-free borosilicate viscous sealing glass and aluminized ferritic stainless steel
An alkali-free, alkaline earth borosilicate glass (designated G73) has been developed as a viscous sealant for use with solid oxide fuel cells (SOFC). In this work, the interfacial interactions that occur between this viscous sealant and aluminized ferritic stainless steel (SS441) under SOFC operati...
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| Veröffentlicht in: | Journal of power sources 2014-03, Vol.250, p.236-241 |
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| creator | Hsu, Jen-Hsien Kim, Cheol-Woon Brow, Richard K. |
| description | An alkali-free, alkaline earth borosilicate glass (designated G73) has been developed as a viscous sealant for use with solid oxide fuel cells (SOFC). In this work, the interfacial interactions that occur between this viscous sealant and aluminized ferritic stainless steel (SS441) under SOFC operational conditions are described. YSZ/glass/aluminized SS441 sandwich seals were held at 800 °C in air for up to 1000 h, and the interfaces were analyzed using analytical scanning electron microscopy (ASEM). Interfacial reactions were also characterized by X-ray diffraction (XRD) analyses of heat-treated mixtures of glass and alumina powders. The results show that the glass reacted with aluminum from the steel to form BaAl2Si2O8 crystals at the glass/metal interface and that the aluminum concentration in the aluminized steel was significantly depleted with time. |
| doi_str_mv | 10.1016/j.jpowsour.2013.11.018 |
| format | Article |
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In this work, the interfacial interactions that occur between this viscous sealant and aluminized ferritic stainless steel (SS441) under SOFC operational conditions are described. YSZ/glass/aluminized SS441 sandwich seals were held at 800 °C in air for up to 1000 h, and the interfaces were analyzed using analytical scanning electron microscopy (ASEM). Interfacial reactions were also characterized by X-ray diffraction (XRD) analyses of heat-treated mixtures of glass and alumina powders. The results show that the glass reacted with aluminum from the steel to form BaAl2Si2O8 crystals at the glass/metal interface and that the aluminum concentration in the aluminized steel was significantly depleted with time.</description><identifier>ISSN: 0378-7753</identifier><identifier>EISSN: 1873-2755</identifier><identifier>DOI: 10.1016/j.jpowsour.2013.11.018</identifier><identifier>CODEN: JPSODZ</identifier><language>eng</language><publisher>Amsterdam: Elsevier B.V</publisher><subject>Aluminized stainless steel ; Applied sciences ; Direct energy conversion and energy accumulation ; Electrical engineering. Electrical power engineering ; Electrical power engineering ; Electrochemical conversion: primary and secondary batteries, fuel cells ; Energy ; Energy. Thermal use of fuels ; Equipments for energy generation and conversion: thermal, electrical, mechanical energy, etc ; Exact sciences and technology ; Fuel cells ; Interfacial interaction ; Solid oxide fuel cell ; Viscous sealing glass</subject><ispartof>Journal of power sources, 2014-03, Vol.250, p.236-241</ispartof><rights>2013 Elsevier B.V.</rights><rights>2015 INIST-CNRS</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c416t-84c58db6388c98d880f4e6a10047dcae4029bd3e853d963b3a07a396e221cd193</citedby><cites>FETCH-LOGICAL-c416t-84c58db6388c98d880f4e6a10047dcae4029bd3e853d963b3a07a396e221cd193</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://www.sciencedirect.com/science/article/pii/S0378775313018442$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,776,780,3537,27901,27902,65534</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=28250453$$DView record in Pascal Francis$$Hfree_for_read</backlink></links><search><creatorcontrib>Hsu, Jen-Hsien</creatorcontrib><creatorcontrib>Kim, Cheol-Woon</creatorcontrib><creatorcontrib>Brow, Richard K.</creatorcontrib><title>Interfacial interactions between an alkali-free borosilicate viscous sealing glass and aluminized ferritic stainless steel</title><title>Journal of power sources</title><description>An alkali-free, alkaline earth borosilicate glass (designated G73) has been developed as a viscous sealant for use with solid oxide fuel cells (SOFC). In this work, the interfacial interactions that occur between this viscous sealant and aluminized ferritic stainless steel (SS441) under SOFC operational conditions are described. YSZ/glass/aluminized SS441 sandwich seals were held at 800 °C in air for up to 1000 h, and the interfaces were analyzed using analytical scanning electron microscopy (ASEM). Interfacial reactions were also characterized by X-ray diffraction (XRD) analyses of heat-treated mixtures of glass and alumina powders. The results show that the glass reacted with aluminum from the steel to form BaAl2Si2O8 crystals at the glass/metal interface and that the aluminum concentration in the aluminized steel was significantly depleted with time.</description><subject>Aluminized stainless steel</subject><subject>Applied sciences</subject><subject>Direct energy conversion and energy accumulation</subject><subject>Electrical engineering. Electrical power engineering</subject><subject>Electrical power engineering</subject><subject>Electrochemical conversion: primary and secondary batteries, fuel cells</subject><subject>Energy</subject><subject>Energy. Thermal use of fuels</subject><subject>Equipments for energy generation and conversion: thermal, electrical, mechanical energy, etc</subject><subject>Exact sciences and technology</subject><subject>Fuel cells</subject><subject>Interfacial interaction</subject><subject>Solid oxide fuel cell</subject><subject>Viscous sealing glass</subject><issn>0378-7753</issn><issn>1873-2755</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2014</creationdate><recordtype>article</recordtype><recordid>eNqFUE1rHDEMNaWBbpP-heJLoZeZWPZ8eG4toWkDgV6as_HYmuCt17O1vAnNr4-XTXsNCCTQe3pPj7GPIFoQMFxu2-1-faT1kFspQLUArQD9hm1Aj6qRY9-_ZRuhRt2MY6_esfdEWyEEwCg27OkmFcyLdcFGHo6zdSWsifiM5RExcVsr_rYxNEtG5POaVwoxOFuQPwRy64E4Yd2ne34fLVFl-Eo57EIKT-j5gjmHEhynYkOKWBFUEOMFO1tsJPzw0s_Z3fW3X1c_mtuf32-uvt42roOhNLpzvfbzoLR2k_Zai6XDwYIQ3eidxU7IafYKda_8NKhZWTFaNQ0oJTgPkzpnn09393n9c0AqZldtY4w2YTVvoJedmiYpVIUOJ6irT1LGxexz2Nn814Awx7DN1vwL2xzDNgCmhl2Jn140LDkbl2yTC_SfLbXsRdcfBb6ccFgffgiYDbmAyaEPGV0xfg2vST0DgkicHA</recordid><startdate>20140315</startdate><enddate>20140315</enddate><creator>Hsu, Jen-Hsien</creator><creator>Kim, Cheol-Woon</creator><creator>Brow, Richard K.</creator><general>Elsevier B.V</general><general>Elsevier</general><scope>IQODW</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7ST</scope><scope>C1K</scope><scope>SOI</scope></search><sort><creationdate>20140315</creationdate><title>Interfacial interactions between an alkali-free borosilicate viscous sealing glass and aluminized ferritic stainless steel</title><author>Hsu, Jen-Hsien ; Kim, Cheol-Woon ; Brow, Richard K.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c416t-84c58db6388c98d880f4e6a10047dcae4029bd3e853d963b3a07a396e221cd193</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2014</creationdate><topic>Aluminized stainless steel</topic><topic>Applied sciences</topic><topic>Direct energy conversion and energy accumulation</topic><topic>Electrical engineering. Electrical power engineering</topic><topic>Electrical power engineering</topic><topic>Electrochemical conversion: primary and secondary batteries, fuel cells</topic><topic>Energy</topic><topic>Energy. Thermal use of fuels</topic><topic>Equipments for energy generation and conversion: thermal, electrical, mechanical energy, etc</topic><topic>Exact sciences and technology</topic><topic>Fuel cells</topic><topic>Interfacial interaction</topic><topic>Solid oxide fuel cell</topic><topic>Viscous sealing glass</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Hsu, Jen-Hsien</creatorcontrib><creatorcontrib>Kim, Cheol-Woon</creatorcontrib><creatorcontrib>Brow, Richard K.</creatorcontrib><collection>Pascal-Francis</collection><collection>CrossRef</collection><collection>Environment Abstracts</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Environment Abstracts</collection><jtitle>Journal of power sources</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Hsu, Jen-Hsien</au><au>Kim, Cheol-Woon</au><au>Brow, Richard K.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Interfacial interactions between an alkali-free borosilicate viscous sealing glass and aluminized ferritic stainless steel</atitle><jtitle>Journal of power sources</jtitle><date>2014-03-15</date><risdate>2014</risdate><volume>250</volume><spage>236</spage><epage>241</epage><pages>236-241</pages><issn>0378-7753</issn><eissn>1873-2755</eissn><coden>JPSODZ</coden><abstract>An alkali-free, alkaline earth borosilicate glass (designated G73) has been developed as a viscous sealant for use with solid oxide fuel cells (SOFC). In this work, the interfacial interactions that occur between this viscous sealant and aluminized ferritic stainless steel (SS441) under SOFC operational conditions are described. YSZ/glass/aluminized SS441 sandwich seals were held at 800 °C in air for up to 1000 h, and the interfaces were analyzed using analytical scanning electron microscopy (ASEM). Interfacial reactions were also characterized by X-ray diffraction (XRD) analyses of heat-treated mixtures of glass and alumina powders. The results show that the glass reacted with aluminum from the steel to form BaAl2Si2O8 crystals at the glass/metal interface and that the aluminum concentration in the aluminized steel was significantly depleted with time.</abstract><cop>Amsterdam</cop><pub>Elsevier B.V</pub><doi>10.1016/j.jpowsour.2013.11.018</doi><tpages>6</tpages></addata></record> |
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| identifier | ISSN: 0378-7753 |
| ispartof | Journal of power sources, 2014-03, Vol.250, p.236-241 |
| issn | 0378-7753 1873-2755 |
| language | eng |
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| source | Elsevier ScienceDirect Journals Complete |
| subjects | Aluminized stainless steel Applied sciences Direct energy conversion and energy accumulation Electrical engineering. Electrical power engineering Electrical power engineering Electrochemical conversion: primary and secondary batteries, fuel cells Energy Energy. Thermal use of fuels Equipments for energy generation and conversion: thermal, electrical, mechanical energy, etc Exact sciences and technology Fuel cells Interfacial interaction Solid oxide fuel cell Viscous sealing glass |
| title | Interfacial interactions between an alkali-free borosilicate viscous sealing glass and aluminized ferritic stainless steel |
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