Quantum Plasmon Resonances Controlled by Molecular Tunnel Junctions
Quantum tunneling between two plasmonic resonators links nonlinear quantum optics with terahertz nanoelectronics. We describe the direct observation of and control over quantum plasmon resonances at length scales in the range 0.4 to 1.3 nanometers across molecular tunnel junctions made of two plasmo...
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| Veröffentlicht in: | Science (American Association for the Advancement of Science) 2014-03, Vol.343 (6178), p.1496-1499 |
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| container_title | Science (American Association for the Advancement of Science) |
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| creator | Tan, Shu Fen Wu, Lin Yang, Joel K.W. Bai, Ping Bosman, Michel Nijhuis, Christian A. |
| description | Quantum tunneling between two plasmonic resonators links nonlinear quantum optics with terahertz nanoelectronics. We describe the direct observation of and control over quantum plasmon resonances at length scales in the range 0.4 to 1.3 nanometers across molecular tunnel junctions made of two plasmonic resonators bridged by self-assembled monolayers (SAMs). The tunnel barrier width and height are controlled by the properties of the molecules. Using electron energy-loss spectroscopy, we directly observe a plasmon mode, the tunneling charge transfer plasmon, whose frequency (ranging from 140 to 245 terahertz) is dependent on the molecules bridging the gaps. |
| doi_str_mv | 10.1126/science.1248797 |
| format | Article |
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| source | Science Magazine; JSTOR Archive Collection A-Z Listing |
| subjects | Broadband transmission Dimers Electrons Molecules Nanoparticles Nanotechnology Optics Plasma spectra Plasmons Quantum physics Quantum tunneling Resonators Tunnel junctions Wave propagation |
| title | Quantum Plasmon Resonances Controlled by Molecular Tunnel Junctions |
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