Pilot-scale study on the acid-catalyzed steam explosion of rice straw using a continuous pretreatment system
► A pilot-scale continuous pretreatment system was successfully developed. ► The pretreatment system shows good operational stability and durability. ► 73% of the total saccharification yield was obtained. ► The system can be used for the production of bioethanol and bio-based chemicals. ► The total...
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Veröffentlicht in: | Bioresource technology 2013-01, Vol.128, p.297-304 |
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creator | Chen, Wen-Hua Tsai, Chia-Chin Lin, Chih-Feng Tsai, Pei-Yuan Hwang, Wen-Song |
description | ► A pilot-scale continuous pretreatment system was successfully developed. ► The pretreatment system shows good operational stability and durability. ► 73% of the total saccharification yield was obtained. ► The system can be used for the production of bioethanol and bio-based chemicals. ► The total sugar yield of rice straw in different scale system was compared.
A continuous acid-catalyzed steam explosion pretreatment process and system to produce cellulosic ethanol was developed at the pilot-scale. The effects of the following parameters on the pretreatment efficiency of rice straw feedstocks were investigated: the acid concentration, the reaction temperature, the residence time, the feedstock size, the explosion pressure and the screw speed. The optimal presteaming horizontal reactor conditions for the pretreatment process are as follows: 1.7rpm and 100–110°C with an acid concentration of 1.3% (w/w). An acid-catalyzed steam explosion is then performed in the vertical reactor at 185°C for 2min. Approximately 73% of the total saccharification yield was obtained after the rice straw was pretreated under optimal conditions and subsequent enzymatic hydrolysis at a combined severity factor of 0.4–0.7. Moreover, good long-term stability and durability of the pretreatment system under continuous operation was observed. |
doi_str_mv | 10.1016/j.biortech.2012.10.111 |
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A continuous acid-catalyzed steam explosion pretreatment process and system to produce cellulosic ethanol was developed at the pilot-scale. The effects of the following parameters on the pretreatment efficiency of rice straw feedstocks were investigated: the acid concentration, the reaction temperature, the residence time, the feedstock size, the explosion pressure and the screw speed. The optimal presteaming horizontal reactor conditions for the pretreatment process are as follows: 1.7rpm and 100–110°C with an acid concentration of 1.3% (w/w). An acid-catalyzed steam explosion is then performed in the vertical reactor at 185°C for 2min. Approximately 73% of the total saccharification yield was obtained after the rice straw was pretreated under optimal conditions and subsequent enzymatic hydrolysis at a combined severity factor of 0.4–0.7. Moreover, good long-term stability and durability of the pretreatment system under continuous operation was observed.</description><identifier>ISSN: 0960-8524</identifier><identifier>EISSN: 1873-2976</identifier><identifier>DOI: 10.1016/j.biortech.2012.10.111</identifier><identifier>PMID: 23201511</identifier><language>eng</language><publisher>Kidlington: Elsevier Ltd</publisher><subject>Acid-catalyzed steam explosion ; Biological and medical sciences ; Carbohydrates - chemical synthesis ; Catalysis ; Cellulase - chemistry ; Cellulose - chemistry ; Cellulose - isolation & purification ; Ethanol - chemical synthesis ; Ethyl alcohol ; Feedstock ; Food industries ; Fundamental and applied biological sciences. Psychology ; Optimization ; Oryza - chemistry ; Pilot Projects ; Pilot-scale ; Plant Components, Aerial - chemistry ; Pretreatment ; Reactors ; Rice ; Rice straw ; Steam ; Steam explosions ; Straw ; Use and upgrading of agricultural and food by-products. Biotechnology</subject><ispartof>Bioresource technology, 2013-01, Vol.128, p.297-304</ispartof><rights>2012 Elsevier Ltd</rights><rights>2014 INIST-CNRS</rights><rights>Copyright © 2012 Elsevier Ltd. All rights reserved.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c431t-7dd554a3936b873754e8dc05ffdfca25e11ad434659eacb4980ed9a06250c0333</citedby><cites>FETCH-LOGICAL-c431t-7dd554a3936b873754e8dc05ffdfca25e11ad434659eacb4980ed9a06250c0333</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktohtml>$$Uhttps://dx.doi.org/10.1016/j.biortech.2012.10.111$$EHTML$$P50$$Gelsevier$$H</linktohtml><link.rule.ids>314,780,784,3548,4021,27921,27922,27923,45993</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=27081582$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/23201511$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Chen, Wen-Hua</creatorcontrib><creatorcontrib>Tsai, Chia-Chin</creatorcontrib><creatorcontrib>Lin, Chih-Feng</creatorcontrib><creatorcontrib>Tsai, Pei-Yuan</creatorcontrib><creatorcontrib>Hwang, Wen-Song</creatorcontrib><title>Pilot-scale study on the acid-catalyzed steam explosion of rice straw using a continuous pretreatment system</title><title>Bioresource technology</title><addtitle>Bioresour Technol</addtitle><description>► A pilot-scale continuous pretreatment system was successfully developed. ► The pretreatment system shows good operational stability and durability. ► 73% of the total saccharification yield was obtained. ► The system can be used for the production of bioethanol and bio-based chemicals. ► The total sugar yield of rice straw in different scale system was compared.
A continuous acid-catalyzed steam explosion pretreatment process and system to produce cellulosic ethanol was developed at the pilot-scale. The effects of the following parameters on the pretreatment efficiency of rice straw feedstocks were investigated: the acid concentration, the reaction temperature, the residence time, the feedstock size, the explosion pressure and the screw speed. The optimal presteaming horizontal reactor conditions for the pretreatment process are as follows: 1.7rpm and 100–110°C with an acid concentration of 1.3% (w/w). An acid-catalyzed steam explosion is then performed in the vertical reactor at 185°C for 2min. Approximately 73% of the total saccharification yield was obtained after the rice straw was pretreated under optimal conditions and subsequent enzymatic hydrolysis at a combined severity factor of 0.4–0.7. Moreover, good long-term stability and durability of the pretreatment system under continuous operation was observed.</description><subject>Acid-catalyzed steam explosion</subject><subject>Biological and medical sciences</subject><subject>Carbohydrates - chemical synthesis</subject><subject>Catalysis</subject><subject>Cellulase - chemistry</subject><subject>Cellulose - chemistry</subject><subject>Cellulose - isolation & purification</subject><subject>Ethanol - chemical synthesis</subject><subject>Ethyl alcohol</subject><subject>Feedstock</subject><subject>Food industries</subject><subject>Fundamental and applied biological sciences. Psychology</subject><subject>Optimization</subject><subject>Oryza - chemistry</subject><subject>Pilot Projects</subject><subject>Pilot-scale</subject><subject>Plant Components, Aerial - chemistry</subject><subject>Pretreatment</subject><subject>Reactors</subject><subject>Rice</subject><subject>Rice straw</subject><subject>Steam</subject><subject>Steam explosions</subject><subject>Straw</subject><subject>Use and upgrading of agricultural and food by-products. Biotechnology</subject><issn>0960-8524</issn><issn>1873-2976</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2013</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqFkU1v1DAQhi0EokvhL1S-IHHJ4vFHnNxAFV9SJTjA2fLaE-pVEi-2Q1l-PQ67hWNPlsbPa8_MQ8gVsC0waF_vt7sQU0F3u-UM-HatAzwiG-i0aHiv28dkw_qWNZ3i8oI8y3nPGBOg-VNywUUNKYANGb-EMZYmOzsizWXxRxpnWm6RWhd842yx4_E3-nqHdqL46zDGHCoSB5qCWzPJ3tElh_k7tdTFuYR5iUumh4QloS0TzoXmY81Pz8mTwY4ZX5zPS_Lt_buv1x-bm88fPl2_vWmcFFAa7b1S0opetLs6jVYSO--YGgY_OMsVAlgvhWxVj9btZN8x9L1lLVfMMSHEJXl1eveQ4o8FczFTyA7H0c5YWzOgGNOagewfRnknedf2Sle0PaEuxZwTDuaQwmTT0QAzqxSzN_dSzCrlbx2gBq_Ofyy7Cf2_2L2FCrw8A3YVMSQ7u5D_c5p1oDpeuTcnDuvyfgZMJruAs0MfErpifAwP9fIHTYmvFg</recordid><startdate>201301</startdate><enddate>201301</enddate><creator>Chen, Wen-Hua</creator><creator>Tsai, Chia-Chin</creator><creator>Lin, Chih-Feng</creator><creator>Tsai, Pei-Yuan</creator><creator>Hwang, Wen-Song</creator><general>Elsevier Ltd</general><general>Elsevier</general><scope>IQODW</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>7SU</scope><scope>7TB</scope><scope>8FD</scope><scope>C1K</scope><scope>FR3</scope><scope>KR7</scope></search><sort><creationdate>201301</creationdate><title>Pilot-scale study on the acid-catalyzed steam explosion of rice straw using a continuous pretreatment system</title><author>Chen, Wen-Hua ; Tsai, Chia-Chin ; Lin, Chih-Feng ; Tsai, Pei-Yuan ; Hwang, Wen-Song</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c431t-7dd554a3936b873754e8dc05ffdfca25e11ad434659eacb4980ed9a06250c0333</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2013</creationdate><topic>Acid-catalyzed steam explosion</topic><topic>Biological and medical sciences</topic><topic>Carbohydrates - chemical synthesis</topic><topic>Catalysis</topic><topic>Cellulase - chemistry</topic><topic>Cellulose - chemistry</topic><topic>Cellulose - isolation & purification</topic><topic>Ethanol - chemical synthesis</topic><topic>Ethyl alcohol</topic><topic>Feedstock</topic><topic>Food industries</topic><topic>Fundamental and applied biological sciences. Psychology</topic><topic>Optimization</topic><topic>Oryza - chemistry</topic><topic>Pilot Projects</topic><topic>Pilot-scale</topic><topic>Plant Components, Aerial - chemistry</topic><topic>Pretreatment</topic><topic>Reactors</topic><topic>Rice</topic><topic>Rice straw</topic><topic>Steam</topic><topic>Steam explosions</topic><topic>Straw</topic><topic>Use and upgrading of agricultural and food by-products. Biotechnology</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Chen, Wen-Hua</creatorcontrib><creatorcontrib>Tsai, Chia-Chin</creatorcontrib><creatorcontrib>Lin, Chih-Feng</creatorcontrib><creatorcontrib>Tsai, Pei-Yuan</creatorcontrib><creatorcontrib>Hwang, Wen-Song</creatorcontrib><collection>Pascal-Francis</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>Environmental Engineering Abstracts</collection><collection>Mechanical & Transportation Engineering Abstracts</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Engineering Research Database</collection><collection>Civil Engineering Abstracts</collection><jtitle>Bioresource technology</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Chen, Wen-Hua</au><au>Tsai, Chia-Chin</au><au>Lin, Chih-Feng</au><au>Tsai, Pei-Yuan</au><au>Hwang, Wen-Song</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Pilot-scale study on the acid-catalyzed steam explosion of rice straw using a continuous pretreatment system</atitle><jtitle>Bioresource technology</jtitle><addtitle>Bioresour Technol</addtitle><date>2013-01</date><risdate>2013</risdate><volume>128</volume><spage>297</spage><epage>304</epage><pages>297-304</pages><issn>0960-8524</issn><eissn>1873-2976</eissn><abstract>► A pilot-scale continuous pretreatment system was successfully developed. ► The pretreatment system shows good operational stability and durability. ► 73% of the total saccharification yield was obtained. ► The system can be used for the production of bioethanol and bio-based chemicals. ► The total sugar yield of rice straw in different scale system was compared.
A continuous acid-catalyzed steam explosion pretreatment process and system to produce cellulosic ethanol was developed at the pilot-scale. The effects of the following parameters on the pretreatment efficiency of rice straw feedstocks were investigated: the acid concentration, the reaction temperature, the residence time, the feedstock size, the explosion pressure and the screw speed. The optimal presteaming horizontal reactor conditions for the pretreatment process are as follows: 1.7rpm and 100–110°C with an acid concentration of 1.3% (w/w). An acid-catalyzed steam explosion is then performed in the vertical reactor at 185°C for 2min. Approximately 73% of the total saccharification yield was obtained after the rice straw was pretreated under optimal conditions and subsequent enzymatic hydrolysis at a combined severity factor of 0.4–0.7. Moreover, good long-term stability and durability of the pretreatment system under continuous operation was observed.</abstract><cop>Kidlington</cop><pub>Elsevier Ltd</pub><pmid>23201511</pmid><doi>10.1016/j.biortech.2012.10.111</doi><tpages>8</tpages></addata></record> |
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subjects | Acid-catalyzed steam explosion Biological and medical sciences Carbohydrates - chemical synthesis Catalysis Cellulase - chemistry Cellulose - chemistry Cellulose - isolation & purification Ethanol - chemical synthesis Ethyl alcohol Feedstock Food industries Fundamental and applied biological sciences. Psychology Optimization Oryza - chemistry Pilot Projects Pilot-scale Plant Components, Aerial - chemistry Pretreatment Reactors Rice Rice straw Steam Steam explosions Straw Use and upgrading of agricultural and food by-products. Biotechnology |
title | Pilot-scale study on the acid-catalyzed steam explosion of rice straw using a continuous pretreatment system |
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